Related papers: Tunneling Splittings in Mn12-Acetate Single Crysta…
The term in spin Hamiltonian, which determines the quantum tunneling rate in Mn12, is measured with neutron scattering. It is much smaller than previously reported values. This may imply that other mechanisms such as hyperfine fields may be…
The dynamical theory of thermally activated resonant magnetization tunneling in uniaxially anisotropic magnetic molecules such as Mn_12Ac (S=10) is developed.The observed slow dynamics of the system is described by master equations for the…
Inelastic tunneling through magnetically anisotropic molecules is studied theoretically in the presence of a strong magnetic field. Since the molecular orientation is not well controlled in tunneling experiments, we consider arbitrary…
We investigate the macroscopic quantum coherence of a spin-1 Rb condensate confined in an anisotropic potential. Under the single-mode approximation, we show that the system can be modeled as a biaxial quantum magnet due to the interplay…
Ramsey et al. [Nature Phys. 4, 277-281 (2008)] report the observation of quantum interference associated with tunnelling trajectories between states of different total spin length in a dimeric molecular nanomagnet. They argue that the…
We performed high resolution diffraction and inelastic neutron scattering measurements of Mn_{12}-acetate. Using a very high energy resolution, we could separate the energy levels corresponding to the splitting of the lowest S multiplet.…
Application of strong dc electric field to an insulator leads to quantum tunneling of electrons from the valence band to the conduction band, which is a famous nonlinear response known as Landau-Zener tunneling. One of the growing interests…
Using a simple model for nonlinear Landau-Zener tunneling between two energy bands of a Bose-Einstein condensate in a periodic potential, we find that the tunneling rates for the two directions of tunneling are not the same. Tunneling from…
We present a detailed analysis of the Landau-Zener problem for an interacting Bose-Einstein condensate in a time-varying double-well trap, especially focussing on the relation between the full many-particle problem and the mean-field…
Decoherence processes in crystals of molecular magnets are prototypical for interacting electronic spin systems. We analyze the Landau-Zener dynamics of the archetypical TbPc$_2$ complex diluted in a diamagnetic monocrystal. The dependence…
Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a…
We compute the width and shape of the EPR and tunneling resonances due to dislocations in Mn-12 acetate crystals. Uncorrelated dislocations produce the Gaussian shape of resonances while dislocations bound in pairs produce the Lorentzian…
A simple mechanical analog describing Landau-Zener tunneling effect is proposed using two weakly coupled chains of nonlinear oscillators with gradually decreasing (first chain) and increasing (second chain) masses. The model allows to…
We consider momentum resolved tunneling between a Luttinger liquid and a two dimensional electron gas as a function of transverse magnetic field. We include the effects of an anomalous exponent and Zeeman splitting on both the Luttinger…
We report synthesis, structural characterization, and magnetic measurements of amorphous Mn$_{12}$-acetate ribbons with a triclinic short-range crystal order not previously seen in experiment. The ribbons exhibit the same structure of…
It has been shown within density-functional theory that in Mn$_{12}$-acetate there are effects due to disorder by solvent molecules and a coupling between vibrational and electronic degrees of freedom. We calculate the in-plane principal…
The symmetry of single-molecule magnets dictates their spin quantum dynamics, influencing how such systems relax via quantum tunneling of magnetization (QTM). By reducing a system's symmetry, through the application of a magnetic field or…
We calculate the tunneling splittings in a Mn$_{12}$ magnetic molecule taking into account its internal many-spin structure. We discuss the precision and reliability of these calculations and show that restricting the basis (limiting the…
We consider a large spin \bf S in the magnetic field parallel to the uniaxial crystal field, interacting with N >> 1 nuclear spins \bf I_i via Hamiltonian \cal H = -DS_z^2 - H_zS_z+ A{\bf S}\cdot \sum_{i=1}^N {\bf I}_i with A << D, at…
We present a method for precisely measuring the tunnel splitting in single-molecule magnets using electron-spin resonance, and use these measurements to precisely and independently determine the underlying transverse anisotropy parameter,…