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We study the temperature dependence as well as anisotropy of optical conductivity ($\sigma_1$) in the pseudocubic single crystal Pr$_{0.5}$Ca$_{1.5}$MnO$_{4}$ using spectrocopic ellipsometry. Three transition temperatures are observed and…

Symmetry arguments are used to develop a spin Hamiltonian for the description of the complex magnetic ordering in HoMnO$_3$. Using a novel application of the Landau Lifshitz Gilbert dynamic torque equations to this model of the frustrated…

Strongly Correlated Electrons · Physics 2012-02-13 S. G. Condran , M. L. Plumer

Calcium vanadate CaV$_2$O$_4$ has a crystal structure of quasi-one-dimensional zigzag chains composed of orbital-active V$^{3+}$ ions and undergoes successive structural and antiferromagnetic phase transitions at $T_s\sim 140$ K and $T_N…

Strongly Correlated Electrons · Physics 2020-06-17 T. Watanabe , S. Kobayashi , Y. Hara , J. Xu , B. Lake , J. -Q. Yan , A. Niazi , D. C. Johnston

The origin of the cooperative Jahn-Teller distortion and orbital-order in LaMnO3 is central to the physics of the manganites. The question is complicated by the simultaneous presence of tetragonal and GdFeO3-type distortions and the strong…

Strongly Correlated Electrons · Physics 2013-05-29 Eva Pavarini , Erik Koch

In $A_{3}$Cr$_{2}$O$_{8}$, where $A$ = Sr or Ba, the Cr$^{5+}$ ions surrounded by oxygen ions in a tetrahedral coordination are Jahn-Teller active. The Jahn-Teller distortion leads to a structural transition and a related emergence of three…

We investigated the electronic response of the quasi-two-dimensional spin gap compound La4Ru2O10 using optical spectroscopy. We observed drastic changes in the optical spectra as the temperature decreased, resulting in anisotropy in the…

Strongly Correlated Electrons · Physics 2009-11-13 S. J. Moon , W. S. Choi , S. J. Kim , Y. S. Lee , P. G. Khalifah , D. Mandrus , T. W. Noh

Basic mechanisms controlling orbital order and orbital fluctuations in transition metal oxides are discussed. The lattice driven classical orbital picture, e.g. like in manganites LaMnO$_3$, is contrasted to the quantum behavior of orbitals…

Strongly Correlated Electrons · Physics 2009-11-11 Giniyat Khaliullin

The functional properties of transition metal perovskite oxides are known to result from a complex interplay of magnetism, polarization, strain, and stoichiometry. Here, we show that for materials with a cooperative Jahn-Teller distortion,…

Materials Science · Physics 2021-01-04 Chiara Ricca , Nicolas Niederhauser , Ulrich Aschauer

Crystal and magnetic structures of the high-pressure stabilized perovskite phase of TlMnO3 have been studied by neutron powder diffraction. The crystal structure involves two types of primary structural distortions: a+b-b-octahedral tilting…

Strongly Correlated Electrons · Physics 2019-03-07 Dmitry D. Khalyavin , Pascal Manuel , Wei Yi , Alexei A. Belik

Starting from the Mott insulator picture for cubic vanadates, we derive and investigate the model of superexchange interactions between V$^{3+}$ ions, with nearly degenerate $t_{2g}$ orbitals occupied by two electrons each. The…

Strongly Correlated Electrons · Physics 2007-06-19 Andrzej M. Oles , Peter Horsch , Giniyat Khaliullin

The longitudinal ultrasonic sound velocity and attenuation, the resistivity, and lattice parameters were studied as a function of temperature from 30 K to 300 K in La1-xCaxMnO3 (0.5<x<0.9). For all the samples, a dramatic stiffening of the…

Strongly Correlated Electrons · Physics 2009-11-07 X. G. Li , R. K. Zheng , G. Li , H. D. Zhou , R. X. Huang , J. Q. Xie , Z. D. Wang

The prototypical Mott-Hubbard insulator LaVO3 undergoes a structural phase transition accompanied by the onset of spin and orbital ordering below 140 K. By combining ultrafast optical pump-probe spectroscopy and two-dimensional electronic…

The properties of Mott insulators with orbital degrees of freedom are described by spin-orbital superexchange models, which provide a theoretical framework for understanding their magnetic and optical properties. We introduce such a model…

Strongly Correlated Electrons · Physics 2015-05-19 Andrzej M. Oleś , Peter Horsch

The Jahn-Teller distortion and the resulting orbital order usually cause some fascinating correlated electronic behaviors, and generally lead to antiferromagnetism in perovskite bulks. Here we demonstrate that the Jahn-Teller distortion…

Materials Science · Physics 2023-05-03 Ke Ji , Zongshuo Wu , Xiaofan Shen , Jianli Wang , Junting Zhang

We investigated the spin-lattice coupling in orthorhombic pseudobrookite FeTi2O5 single crystal with highly ordered $ Fe^{2+} / Ti^{4+}$ occupation, which consists of quasi-1D S=2 chains running along a-axis. Both the magnetization and…

Strongly Correlated Electrons · Physics 2024-05-31 Hao-Hang Xu , Jian Liu , L. L. Tao , Xian-Jie Wang , Sergey V. Streltsov , Yu Sui

We report on a dynamical mean-field theoretical analysis of emerging low-temperature phases in multicomponent gases of fermionic alkaline-earth(-like) atoms in state-dependent optical lattices. Using the example of $^{173}$Yb atoms, we show…

Quantum Gases · Physics 2020-05-21 Andrii Sotnikov , Nelson Darkwah Oppong , Yeimer Zambrano , Agnieszka Cichy

Ultrasound velocity measurements of cubic spinel GeCo$_2$O$_4$ in single crystal were performed for the investigation of shear and compression moduli. The shear moduli in the paramagnetic state reveal an absence of Jahn-Teller activity…

Strongly Correlated Electrons · Physics 2009-11-13 Tadataka Watanabe , Shigeo Hara , Shin-Ichi Ikeda

Motivated by recent interest in quasi-one-dimensional compound CaV2O4, we study the ground states of a spin-orbital chain characterized by an Ising-like orbital Hamiltonian and frustrated interactions between S=1 spins. The on-site…

Strongly Correlated Electrons · Physics 2010-07-13 Gia-Wei Chern , Natalia Perkins

In a two orbital double exchange model we formulate Jahn-Teller coupled charge density wave in one electron per lattice site limit. Softening of Jahn-Teller phonons corresponding to distortion modes $Q_2$ or $Q_3$ associated with perfect…

Strongly Correlated Electrons · Physics 2016-08-31 Manidipa Mitra

In this work we study the complex entanglement between spin interactions, electron correlation and Janh-Teller structural instabilities in the 5d$^1$ $J_{eff}=\frac{3}{2}$ spin-orbit coupled double perovskite $\rm Ba_2NaOsO_6$ using first…

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