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Double perovskites like Sr$_2$FeMoO$_6$ are materials with half-metallic ground states and ferrimagnetic T$_{\rm{c}}$'s well above room temperature. This paper is the second of our comprehensive theory for half metallic double perovskites.…

Strongly Correlated Electrons · Physics 2013-04-08 Onur Erten , O. Nganba Meetei , Anamitra Mukherjee , Mohit Randeria , Nandini Trivedi , Patrick Woodward

We present a comprehensive theory of the temperature- and disorder-dependence of half-metallic ferrimagnetism in the double perovskite Sr$_2$FeMoO$_6$ (SFMO) with $T_c$ above room temperature. We show that the magnetization $M(T)$ and…

Strongly Correlated Electrons · Physics 2015-05-28 Onur Erten , O. Nganba Meetei , Anamitra Mukherjee , Mohit Randeria , Nandini Trivedi , Patrick Woodward

We consider a model of the double perovskite Ba2FeReO6, a room temperature ferrimagnet with correlated and spin-orbit coupled Re t2g electrons moving in the background of Fe moments stabilized by Hund's coupling. We show that for such 3d/5d…

Strongly Correlated Electrons · Physics 2015-06-16 A. M. Cook , A. Paramekanti

Sr$_{2}$FeMoO$_6$ is a double perovskite compound, known for its high temperature behavior. Combining different magnetic and spectroscopic tools, we show that this compound can be driven to rare example of antiferromagnetic metallic state…

We formulate a superexchange theory of insulating double-perovskite compounds such as Sr$_2$FeWO$_6$. An effective spin-orbital Hamiltonian is derived in the strong coupling limit of Hubbard model for d-electrons on Fe and W ions. The…

Strongly Correlated Electrons · Physics 2009-11-10 S. Di Matteo , G. Jackeli , N. B. Perkins

We have implemented a systematic LSDA and LSDA+U study of the double perovskites $A_{2}$FeReO$_{6}$ (A=Ba,Sr,Ca) and Sr$_{2}$$M$MoO$_{6}$ (M=Cr,Mn,Fe,Co) for understanding of their intriguing electronic and magnetic properties. The results…

Materials Science · Physics 2009-11-07 Hua Wu

Using the first-principles density functional approach, we investigate a material Pr$_2$MgIrO$_6$ (PMIO) of double perovskite structure synthesized recently. According to the calculations, PMIO is a magnetic Mott-Hubbard insulator…

Materials Science · Physics 2016-04-29 Madhav P. Ghimire , Long-Hua Wu , Xiao Hu

Using density functional calculations, we find that the newly synthesized Ca$_2$FeOsO$_6$ has the high-spin Fe$^{3+}$ ($3d^5$)-Os$^{5+}$ ($5d^3$) state. The octahedral Os$^{5+}$ ion has a large intrinsic exchange splitting, and its…

Strongly Correlated Electrons · Physics 2014-08-13 Hongbo Wang , Shasha Zhu , Xuedong Ou , Hua Wu

We present an interacting model for the electronic and magnetic behavior of a strained $(001)$ atomic layer of Sr$_2$FeMoO$_6,$ which shows room-temperature ferrimagnetism and magnetoresistance with potential spintronics application in the…

Strongly Correlated Electrons · Physics 2020-07-22 Masahiko G. Yamada , George Jackeli

We put forward double perovskites of the R$_2$NiMnO$_6$ family (with $R$ a rare-earth atom) as a new class of multiferroics on the basis of {\it ab initio} density functional calculations. We show that changing $R$ from La to Y drives the…

Strongly Correlated Electrons · Physics 2015-05-14 Sanjeev Kumar , Gianluca Giovannetti , Jeroen van den Brink , Silvia Picozzi

The magnetic properties of the double perovskite oxide $Sr_{2}$FeMo$O_{6}$ are analyzed using a mixed-spin Ising model with spins $\left( \frac{1}{2},\frac{5}{2}\right) $ in the presence of a random crystal field $\Delta$ and exchange…

Statistical Mechanics · Physics 2025-03-10 Said Khaireddine , Redouane Assad , Mohammed El Falaki , Rachid Ahl Lamara , Lalla Btissam Drissi

A comprehensive theory for electronic transport in itinerant ferromagnets is developed. We first show that the Q-field theory used previously to describe a disordered Fermi liquid also has a saddle-point solution that describes a…

Statistical Mechanics · Physics 2009-10-31 T. R. Kirkpatrick , D. Belitz

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Strongly Correlated Electrons · Physics 2016-09-01 W. K. Zhu , J. -C. Tung , W. Tong , L. Ling , M. Starr , J. M. Wang , W. C. Yang , Y. Losovyj , H. D. Zhou , Y. Q. Wang , P. -H. Lee , Y. -K. Wang , Chi-Ken Lu , S. X. Zhang

The puzzling observation of room temperature ferromagnetism in double perovskites (A$_2$BB$'$O$_6$), despite having the magnetic lattice of B-ions diluted by non-magnetic B$'$-ions, have been examined for Sr$_2$FeReO$_6$. {\it Ab-initio}…

Strongly Correlated Electrons · Physics 2022-02-03 Shishir K. Pandey , Ashis K. Nandy , Poonam Kumari , Priya Mahadevan

The electronic structure and magnetism of Sr$_2$CeIrO$_6$, an Ir-based double perovskite system has been investigated using first-principles calculations. We found that a strong spin-orbit coupling dictate the electronic and magnetic…

Strongly Correlated Electrons · Physics 2013-01-29 S. K. Panda , I. Dasgupta

The double perovskite material \SFMO has the rare and desirable combination of a half-metallic ground state with 100% spin polarization and ferrimagnetic \Tc$\simeq 420$K, well above room temperature. In this two-part paper, we present a…

Strongly Correlated Electrons · Physics 2013-04-08 O. Nganba Meetei , Onur Erten , Anamitra Mukherjee , Mohit Randeria , Nandini Trivedi , Patrick Woodward

Motivated by the recent observation of evidences of ferromagnetism in correlated insulating states in systems with Moir\'{e} superlattices, we study a two-orbital quantum antiferromagnetic model on the triangular lattice, where the two…

Strongly Correlated Electrons · Physics 2019-07-31 Xiao-Chuan Wu , Anna Keselman , Chao-Ming Jian , Kelly Ann Pawlak , Cenke Xu

The possible heavy fermion superconductivity is carefully reexamined in the two-dimensional Kondo lattice model with an antiferromagnetic Heisenberg superexchange between local magnetic moments. In order to establish an effective mean field…

Strongly Correlated Electrons · Physics 2012-08-02 Yu Liu , Huan Li , Guang-Ming Zhang , L. Yu

Exploring new magnetic materials is essential for finding advantageous functional properties such as magnetoresistance, magnetocaloric effect, spintronic functionality, and multiferroicity. Versatile classes of double perovskite compounds…

Strongly Correlated Electrons · Physics 2019-05-03 M. K. Kim , J. Y. Moon , S. H. Oh , D. G. Oh , Y. J. Choi , N. Lee

The functional characteristics of double perovskites with unique ferromagnetic-insulator ground state have been controversial due to the unavoidable presence of anti-site disorders (ASDs). Here, we aim to investigate the origin of magnetic…

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