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We investigate theoretically polyelectrolyte bridging interactions on the two-body level. The model system is composed of two macroions with two oppositely charged flexible chains. The electrostatic interactions are treated on the Debye -…

Soft Condensed Matter · Physics 2009-11-10 Rudi Podgornik

Magnetohydrodynamically induced interface instability in liquid metal batteries is analyzed. The batteries are represented by a simplified system in the form of a rectangular cell, in which strong vertical electric current flows through…

Fluid Dynamics · Physics 2018-04-12 Oleg Zikanov

Magnetic beads attract each other forming chains. We pushed such chains into an inclined Hele-Shaw cell and discovered that they spontaneously form self-similar patterns. Depending on the angle of inclination of the cell, two completely…

Statistical Mechanics · Physics 2021-04-21 Danilo S. Borges , Hans J. Herrmann , Humberto A. Carmona , José S. Andrade , Ascânio D. Araújo

We investigate the properties of a system of semi-diluted polymers in the presence of charged groups and counter-ions, by means of self-consistent field theory. We study a system of polyelectrolyte chains grafted to a similarly, as well as…

Soft Condensed Matter · Physics 2015-05-19 Gabriele Migliorini

We discuss the effect of slow phase relaxation and the spin off-diagonal $S$-matrix correlations on the cross section energy oscillations and the time evolution of the highly excited intermediate systems formed in complex collisions. Such…

Quantum Physics · Physics 2008-11-26 Luis Benet , Lewis T. Chadderton , Sergey Yu. Kun , Oleg K. Vorov , Wang Qi

The article presents a comprehensive study of counterion dynamics around a generic linear polyelectrolyte (PE) chain with the help of coarse-grained computer simulations. The ion-chain coupling is discussed in the form of binding time,…

Soft Condensed Matter · Physics 2022-04-13 Keerthi Radhakrishnan , Sunil P. Singh

Nanoporous supercapacitors play an important role in modern energy storage systems, and their modeling is essential to predict and optimize the charging behaviour. Two classes of models have been developed that consist of finite and…

Soft Condensed Matter · Physics 2019-02-12 Konrad Breitsprecher , Manuel Abele , Svyatoslav Kondrat , Christian Holm

We present the results from an extensive atomistic molecular dynamics simulation study of poly(ethylene oxide) (PEO) doped with various amounts of lithium-bis(trifluoromethane)sulfonimide (LiTFSI) salt under the influence of external…

Soft Condensed Matter · Physics 2021-03-10 Alina Wettstein , Diddo Diddens , Andreas Heuer

Similarly-charged polymers in solution, known as polyelectrolytes, are known to form aggregated structures in the presence of oppositely charged counterions. Understanding the dependence of the equilibrium phases and the dynamics of the…

Soft Condensed Matter · Physics 2017-07-03 Anvy Moly Tom , Ravindran Rajesh , Satyavani Vemparala

The development of novel electrolytes and electrodes for supercapacitors is hindered by a gap of several orders of magnitude between experimentally measured and theoretically predicted charging timescales. Here, we propose an electrode…

Chemical Physics · Physics 2020-02-26 Cheng Lian , Mathijs Janssen , Honglai Liu , René van Roij

We have investigated the electronic structure of iridates in the double perovskite crystal structure containing either Ir$^{4+}$ or Ir$^{5+}$ using hard x-ray photoelectron spectroscopy. The experimental valence band spectra can be well…

Several statistical mechanical theories predict that colloidal suspensions of highly charged macroions and monovalent microions can exhibit unusual thermodynamic phase behavior when strongly deionized. Density-functional, extended…

Soft Condensed Matter · Physics 2009-11-11 A. R. Denton

In the presence of attraction, the jamming transition of packings of frictionless particles corresponds to the rigidity percolation. When the range of attraction is long, the distribution of the size of rigid clusters, $P(s)$, is continuous…

Soft Condensed Matter · Physics 2021-01-26 Yuchuan Wang , Sheng Fang , Ning Xu , Youjin Deng

We consider the rupture dynamics of a homopolymer chain pulled at one end at a constant loading rate. Our model of the breakable polymer is related to the Rouse chain, with the only difference that the interaction between the monomers is…

Soft Condensed Matter · Physics 2009-10-29 S. Fugmann , I. M. Sokolov

Understanding the behavior of charged complex fluids is crucial for a plethora of important industrial, technological, and medical applications. Using coarse-grained molecular dynamics simulations, here we investigate the properties of a…

Soft Condensed Matter · Physics 2022-08-04 Debarshee Bagchi

A simple lattice model of a solid electrolyte presented as a xy-slab geometry system of mobile cations on a background of energetic landscape of the host system and a compensating field of uniformly distributed anions is studied. The system…

Statistical Mechanics · Physics 2019-03-14 T. Patsahan , G. Bokun , D. di Caprio , M. Holovko , V. Vikhrenko

In this paper, we present a continuation of our research on modeling electrolyte solutions within charged slit pores. We make use of the model developed by Blossey et al., which takes into account the structural interactions between ions…

Soft Condensed Matter · Physics 2023-07-26 Victoria A. Vasileva , Daria A. Mazur , Yury A. Budkov

Charged systems with partially annealed charge disorder are investigated using field-theoretic and replica methods. Charge disorder is assumed to be confined to macroion surfaces surrounded by a cloud of mobile neutralizing counterions in…

Soft Condensed Matter · Physics 2009-05-24 Yevgeni Sh. Mamasakhlisov , Ali Naji , Rudolf Podgornik

It is known that a large, charged body immersed in a solution of multivalent counterions may undergo charge inversion as the counterions adsorb to its surface. We use the theory of charge inversion to examine the case of a deformable,…

Soft Condensed Matter · Physics 2009-09-29 Brian Skinner , B. I. Shklovskii

Experiments with polymer latex solutions show the coexistence of order-disorder structures of macroions. Because of the large macroions' sizes, this order-disorder phase coexistence imply the existence of very long-range attractive and…

Soft Condensed Matter · Physics 2019-02-20 Alfredo González-Calderón , Enrique González-Tovar , Marcelo Lozada-Cassou
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