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The effect of laser fields on the electron transport through a molecular wire being weakly coupled to two leads is investigated. The molecular wire acts as a coherent quantum ratchet if the molecule is composed of periodically arranged,…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Jörg Lehmann , Sigmund Kohler , Peter Hänggi , Abraham Nitzan

The treatment of the previous paper is extended to molecular wires. Specifically, the effect of electron-vibrational interactions on the electronic transport induced by femtosecond $\omega+2\omega$ laser fields along unbiased molecular…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Sigmund Kohler , Volkhard May , Peter Hänggi

We investigate the possibility of optical current control through single molecules which are weakly coupled to leads. A master equation approach for the transport through a molecule is combined with a Floquet theory for the time-dependent…

Chemical Physics · Physics 2016-09-08 Jörg Lehmann , Sébastien Camalet , Sigmund Kohler , Peter Hänggi

A minimal model for coherent transport through a donor/acceptor molecular junction is presented. The two donor and acceptor sites are described by single levels energetically separated by an intramolecular tunnel barrier. In the limit of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Florian Pump , Gianaurelio Cuniberti

New features of molecular wires can be observed when they are irradiated by laser fields. These effects can be achieved by periodically oscillating fields but also by short laser pulses. The theoretical foundation used for these…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Sven Welack , Michael Schreiber , Ulrich Kleinekathoefer

The electron tunneling through a molecular junction modeled by a single site weakly coupled to two leads is studied in the presence of a time-dependent external field using a master equation approach. In the case of small bias voltages and…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Guangqi Li , Michael Schreiber , Ulrich Kleinekathoefer

We investigate the influence of external laser excitations on the average current through bridged molecules. For the computation of the current, we use a numerically very efficient formalism that is based on the Floquet solutions of the…

Chemical Physics · Physics 2007-05-23 Sigmund Kohler , Jörg Lehmann , Sébastien Camalet , Peter Hänggi

A molecular wire coupled to two electron reservoirs is investigated within a tight-binding approach including spin and Coulomb interaction. Under the assumption of weak coupling to the electron reservoirs a quantum master equation can be…

Mesoscale and Nanoscale Physics · Physics 2007-08-28 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

The influence of Gaussian laser pulses on the transport through molecular wires is investigated within a tight-binding model for spinless electrons including correlation. Motivated by the phenomenon of coherent destruction of tunneling for…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

We investigate transport through molecular wires whose energy levels are affected by environmental fluctuations. We assume that the relevant fluctuations are so slow that they, within a tight-binding description, can be described by…

Mesoscale and Nanoscale Physics · Physics 2008-07-09 Franz J. Kaiser , Peter Hänggi , Sigmund Kohler

We introduce a theoretical approach based on scattering theory and total energy methods that treats transport non-linearities, conformational changes and charging effects in molecular wires in a unified way. We apply this approach to…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Eldon Emberly , George Kirczenow

We consider several fundamental optical phenomena involving single molecules in biased metal-molecule-metal junctions. The molecule is represented by its highest occupied and lowest unoccupied molecular orbitals, and the analysis involves…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan

Electrophoresis is a motion of charged dispersed particles relative to a fluid in a uniform electric field. The effect is widely used to separate macromolecules, to assemble colloidal structures, to transport particles in nano- and…

Soft Condensed Matter · Physics 2011-01-21 Oleg D. Lavrentovich , Israel Lazo , Oleg P. Pishnyak

We present a simple model of electrical transport through a metal-molecule-metal nanojunction that includes charging effects as well as aspects of the electronic structure of the molecule. The interplay of a large charging energy and an…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Matthias H. Hettler , Herbert Schoeller , Wolfgang Wenzel

We explore heat transfer in molecular junctions between two leads in the absence of a finite net thermal bias. The application of an unbiased, time-periodic temperature modulation of the leads entails a dynamical breaking of reflection…

Mesoscale and Nanoscale Physics · Physics 2009-12-18 Fei Zhan , Nianbei Li , Sigmund Kohler , Peter Hänggi

We develop a new general formulation to explore light-driven electron transport through a single-molecule device with multiple pathways. Three individual systems are proposed including (i) a two-terminal molecular junction based on…

Mesoscale and Nanoscale Physics · Physics 2014-01-20 Liang-Yan Hsu , Herschel Rabitz

We give a detailed derivation of the master equation description of the coherent backscattering of laser light by cold atoms. In particular, our formalism accounts for the nonperturbative nonlinear response of the atoms when the injected…

Quantum Physics · Physics 2009-11-13 Vyacheslav Shatokhin , Cord A. Müller , Andreas Buchleitner

The alternative to dynamic alignment explanation of experimental results on spatial-asymmetric dissociation of molecules in a laser field is proposed. The concept of geometrical alignment is sufficient for explanation of these results. In…

Optics · Physics 2007-05-23 V. A. Kuz'menko

Charge transport through a rectangular vector potential barrier modulated by a continuum laser in monolayer phosphorene is studied theoretically in the ballistic regime along the line of Floquet formalism. Laser free transmission profile…

Mesoscale and Nanoscale Physics · Physics 2019-06-12 R. Biswas , R. Dey , C. Sinha
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