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Detailed Raman spectroscopy studies on polycrystalline Sr1-xPrxTiO3 (x=0.01, 0.025, 0.05, 0.075, 0.09, 0.13, 0.15, 0.17) samples are reported elucidating the microscopic mechanism of relaxor ferroelectrics. The polar mode was observed upto…

Materials Science · Physics 2019-06-26 Vivek Dwij , Binoy Krishna De , Shekhar Tyagi , Gaurav Sharma , V. G. Sathe

Perovskite structure materials based on the Ba1-xGdxTiO3 system, where x = 0.001, 0.002, 0.003, 0.004 and 0.005, were prepared via the Pechini chemical synthesis route. The dielectric properties have been analyzed over a wide temperature…

Materials Science · Physics 2024-09-25 T. H. T. Rosa , M. A. Oliveira , Y. Mendez-Gonzalez , F. Guerrero , R. Guo , A. S. Bhalla , J. D. S. Guerra

While defects are unavoidable in crystals and often detrimental to material performance, they can be a key ingredient for inducing functionalities when tailored. Here, we demonstrate that an A-site-deficient perovskite Y$_{1/3}$TaO$_3$…

Dielectric permittivity and infrared reflectivity spectra of Li doped KNbO3 single crystals have been studied for the first time for K1-xLixNbO3 (KLN) with x = 0.015, 0.02, 0.065. It was found that like in KTaO3, Li admixture results in…

Other Condensed Matter · Physics 2007-05-23 V. A. Trepakov , M. L. Savinov , V Zelezny , P. P. Syrnikov , A. G. Deyneka , L. Jastrabik

We report filling-fraction dependent dielectric spectroscopy measurements on the relaxation dynamics of the rod-like nematogen 7CB condensed in 13 nm silica nanochannels. In the film-condensed regime, a slow interface relaxation dominates…

Soft Condensed Matter · Physics 2015-04-21 Sylwia Calus , Andriy V. Kityk , Manfred Eich , Patrick Huber

We present a first-principles investigation of ferroelectricity in layered perovskite oxide La2Ti2O7 (LTO), one of the compounds with highest Curie temperature known (1770 K). Our calculations reveal that LTO's ferroelectric transition…

Materials Science · Physics 2015-05-27 Jorge Lopez-Perez , Jorge Iniguez

We review some of the current research on two of the ultra-high piezoelectric relaxors Pb(Mg1/3Nb2/3)O3 (PMN) and Pb(Zn1/3Nb2/3)O3 (PZN). The discovery of a monoclinic phase in Pb(Zr1-xTix)O3 (PZT) in 1999 by Noheda et al. forced a…

Materials Science · Physics 2007-05-23 G. Shirane , P. M. Gehring

We report measurements of the neutron diffuse scattering in a single crystal of the relaxor ferroelectric material 95.5%Pb(Zn1/3Nb2/3)O3-4.5%PbTiO3 (PZN-4.5%PT). We show that the diffuse scattering at high temperatures has a quasielastic…

Materials Science · Physics 2013-01-10 Zhijun Xu , Jinsheng Wen , E. Mamontov , C. Stock , P. M. Gehring , Guangyong Xu

Hybrid organic inorganic formate perovskites, AB(HCOO)$_3$, is a large family of compounds which exhibit variety of phase transitions and diverse properties. Some examples include (anti)ferroelectricity, ferroelasticity,…

We study the light-absorbing states of the mixed-halide perovskite CH$_{3}$NH$_{3}$PbI$_2$Cl and tri-iodide perovskite CH$_{3}$NH$_{3}$PbI$_3$ with density functional and many-body calculations to explain the desirable photovolatic features…

Materials Science · Physics 2014-11-06 Ravindra Nanguneri , John Parkhill

Under continuous light illumination, it is known that localized domains with segregated halide compositions form in semiconducting mixed-halide perovskites, thus severely limiting their optoelectronic applications due to the negative…

Materials Science · Physics 2023-03-21 Shengnan Feng , Rentong Duan , Yu Ju , Shuyi Li , Chunfeng Zhang , Shuxia Tao , Min Xiao , Xiaoyong Wang

Previously reported neutron scattering investigations of the canonical relaxor ferroelectric perovskite oxide with a chemical formula Pb(Mg(1/3)Nb(2/3))O3 (PMN) are revisited in order to appreciate the role of the intrinsic bulk…

Materials Science · Physics 2026-05-12 J. Hlinka

By using first-principles methods based on density functional theory we revisited the zero-temperature phase diagram of stoichiometric SrCoO3, a ferromagnetic metallic perovskite that undergoes significant structural, electronic, and…

Materials Science · Physics 2016-12-21 Pablo Rivero , Claudio Cazorla

Brillouin spectroscopic measurements have been carried out on relaxor ferroelectric Pb(Zn1/3Nb2/3)0.85Ti0.15O3 (PZN-PT) single crystal over the temperature range 300-585 K. The longitudinal acoustic phonon begins to soften below 650 K,…

Materials Science · Physics 2015-06-05 K. K. Mishra , V. Sivasubramanian , A. K. Arora , Dillip Pradhan

Relaxor ferroelectric perovskites are highly polarizable and can exhibit giant coupling between elastic strain and an applied electric field. Here, we report an in situ extended X-ray absorption fine structure (EXAFS) study of a…

The phase transition into the ferroelectric phase in barium titanate occurs in many stages with the appearance of nonlinear phenomena. The mixed nature of the transition: displacive and order-disorder type, causes the occurrence of a…

Materials Science · Physics 2024-10-18 Olga Mazur , Ken-ichi Tozaki , Leonid Stefanovich

We demonstrate that recent experimental data (E. Castel et al J.Phys. Cond. Mat. {\bf 21} (2009), 452201) on tungsten bronze compound (TBC) Ba$_2$Pr$_x$Nd$_{1-x}$FeNb$_4$O$_{15}$ can be well explained in our model predicting a crossover…

Materials Science · Physics 2015-05-18 V. A. Stephanovich

Chalcogenide perovskites are lead-free materials for potential photovoltaic or thermoelectric applications. BaZrS$_3$ is the most studied member of this family due to its superior thermal and chemical stability, desirable optoelectronic…

Materials Science · Physics 2025-02-10 Prakriti Kayastha , Erik Fransson , Paul Erhart , Lucy D. Whalley

Dielectric, anelastic and ^139La NMR relaxation measurements have been made on the relaxor ferroelectric Pb(1-3x/2)La(x)Zr(0.2)Ti(0.8)O(3) (PLZT) with x = 0.22. The dielectric susceptibility exihibits the frequency dispersive maximum due to…

Materials Science · Physics 2010-07-23 F. Cordero , M. Corti , F. Craciun , C. Galassi , D. Piazza , F. Tabak

Frequency-dependent and temperature-dependent dielectric measurements are performed on double perovskite Tb$_2$NiMnO$_6$. The real ($\epsilon_1$) and imaginary ($\epsilon_2$) parts of dielectric permittivity show three plateaus suggesting…

Materials Science · Physics 2015-06-18 Hariharan Nhalil , Harikrishnan. S. Nair , H. L. Bhat , Suja Elizabeth