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The mechanisms and efficiency of charge transport in lithium peroxide (Li2O2) are key factors in understanding the performance of non-aqueous Li-air batteries. Towards revealing these mechanisms, here we use first-principles calculations to…

Materials Science · Physics 2013-06-25 Maxwell D. Radin , Donald J. Siegel

We suggest universal expressions for the rates of charge transition between molecules in organic disordered semiconductors, which differ between electrons and holes. The donor and acceptor molecules (monomers) are represented in terms of…

Disordered Systems and Neural Networks · Physics 2015-08-17 E. D. Gutliansky , Nir Tesler , Uri Peskin

In this manuscript, recent theoretical investigations by the authors in the area of oxide multilayers are briefly reviewed. The calculations were carried out using model Hamiltonians and a variety of non-perturbative techniques. Moreover,…

Strongly Correlated Electrons · Physics 2009-11-13 I. Gonzalez , S. Okamoto , S. Yunoki , A. Moreo , E. Dagotto

We develop a theory of the low-temperature charge transfer between a superconductor and a hopping insulator. We show that the charge transfer is governed by the coherent two-electron -- Cooper pair conversion process, time reversal…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 V. I. Kozub , A. A. Zyuzin , Y. M. Galperin , V. Vinokur

Three driving forces control the energy level alignment between transition-metal oxides and organic materials: the chemical interaction between the two materials, the organic electronegativity and the possible space charge layer formed in…

Charge separation properties, that is the ability of a chromophore, or a chromophore/semiconductor interface, to separate charges upon light absorption, are crucial characteristics for an efficient photovoltaic device. Starting from this…

Chemical Physics · Physics 2019-12-05 Thibaud Etienne , Mariachiara Pastore

We explore electron transport properties in molecular wires made of heterocyclic molecules (pyrrole, furan and thiophene) by using the Green's function technique. Parametric calculations are given based on the tight-binding model to…

Mesoscale and Nanoscale Physics · Physics 2009-09-13 Santanu K. Maiti , S. N. Karmakar

The quasi-one-dimensional organic conductors (TMTTF)$_2X$ with non-centrosymmetric anions commonly undergo charge- and anion-order transitions upon cooling. While for compounds with tetrahedral anions ($X$ = BF$_4^-$, ReO$_4^-$, and…

Strongly Correlated Electrons · Physics 2021-04-23 Olga Iakutkina , Lena Nadine Majer , Guilherme Gorgen Lesseux , Gabriele Untereiner , Martin Dressel

The transfer of charge between different regions of a phase-coherent mesoscopic sample is investigated. Charge transfer from a side branch quantum dot into a ring changes the persistent current through a sequence of plateaus of diamagnetic…

Condensed Matter · Physics 2007-05-23 M. Büttiker , C. A. Stafford

Transport in electronic devices based on high-Tc superconductors depends critically on the charge redistribution at interfaces, since the band structure is modified on a local scale. Using the density functional theory approach for relaxed…

Superconductivity · Physics 2009-11-13 Cosima Schuster , Udo Schwingenschloegl

Charge transfer between molecules and catalysts plays a critical role in determining the efficiency and yield of photo-chemical catalytic processes. In this paper, we study light-induced electron transfer between transition metal doped…

Materials Science · Physics 2021-09-15 Alexandra Göbel , Angel Rubio , Johannes Lischner

Spin-transfer torques occur in magnetic heterostructures because the transverse component of a spin current that flows from a non-magnet into a ferromagnet is absorbed at the interface. We demonstrate this fact explicitly using free…

Materials Science · Physics 2009-11-07 M. D. Stiles , A. Zangwill

Interfacial charge transfer plays an essential role in establishing the relative alignment of the metal Fermi level and the energy bands of organic semiconductors. While the details remain elusive in many systems, this charge transfer has…

Materials Science · Physics 2009-05-21 J. H. Worne , R. Giridharagopal , K. F. Kelly , D. Natelson

The electron transport properties of ZnO nano-wires coupled by two aluminium electrodes were studied by {\it ab initio} method based on non-equilibrium Green's function approach and density functional theory. A clearly rectifying…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Zijiang Yang , Langhui Wan , Yunjin Yu , Yadong Wei , Jian Wang

Charge-carrier transport in a paradigmatic semicrystalline polymer semiconductor (P3HT) is important for both fundamental understanding and applications. In samples with enhanced structural disorder due to ad-hoc point defects, the mobility…

Soft Condensed Matter · Physics 2016-07-20 Breanndan O. Conchuir , Carlo Tarantini , Chris R. McNeill , Sven Hüttner , Alessio Zaccone

We introduce a theoretical approach based on scattering theory and total energy methods that treats transport non-linearities, conformational changes and charging effects in molecular wires in a unified way. We apply this approach to…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Eldon Emberly , George Kirczenow

We discuss the origin of an additional dip other than the charge neutrality point observed in transfer characteristics of graphene-based field-effect transistors. The double-dip is proved to arise from charge transfer between graphene and…

Whether at phenomenological or microscopic levels, most theoretical approaches to charge transport through molecular junctions postulate or attempt to justify microscopically the existence of a dominant molecular orbital (MO). Within such…

Mesoscale and Nanoscale Physics · Physics 2015-11-26 Ioan Baldea

The organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ provides the prime example of a charge-order-driven metal-insulator transition. Restricted chemical substitution of S atoms by Se in the constituent molecules allows us to modify the…

The quasi-two-dimensional nature of the charge carriers energy spectrum in layered conductors leads to specific effects in an external magnetic field. The magnetoresistance of layered conductors in a wide range of strong magnetic fields…

Statistical Mechanics · Physics 2010-06-09 O. V. Kirichenko , Yu. A. Kolesnichenko , V. G. Peschansky