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Using a first principles approach, we study the electron transport properties of a new class of molecular wires containing fluorenone units, whose features open up new possibilities for controlling transport through a single molecule. We…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. J. Lambert , I. M. Grace , T. Papadopoulos

We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

The possibility of using single molecule junctions as electron pumps for energy conversion and storage is considered. It is argued that the small dimensions of these systems enable to make use of unique intra-molecular quantum coherences in…

Quantum Physics · Physics 2015-05-20 Roie Volkovich , Uri Peskin

The transport properties of a octane-dithiol (ODT) molecule coupled to Au(001) leads are analyzed using density functional theory and non-equilibrium Green functions. It is shown that a symmetric molecule can turn into a diode under…

Mesoscale and Nanoscale Physics · Physics 2010-02-09 Tomasz Kostyrko , Víctor M. García-Suárez , Colin J. Lambert , Bogdan R. Bułka

Electron charging play key roles in physiochemical processes, whose intrinsic stabilization in single molecules is desirable for tailoring molecular functionality and developing molecular devices, but remains elusive on surfaces. Here, we…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Xin Liao , Rui-Jing Sun , Emi Minamitani , Lian-Zhi Yang , Tao Xie , Wen-Hao Zhang , Chaofei Liu , Svetlana Klyatskaya , Mario Ruben , Ying-Shuang Fu

An overview of results of models of coupled quantum rotors is presented. We focus on rotors with dipolar and quadrupolar potentials in two and three dimensions, potentials which correspond to approximate descriptions of real molecules…

Statistical Mechanics · Physics 2015-05-13 Yuri A. Freiman , B. Hetenyi , S. M. Tretyak

We study bistability in the electron transport through a ring of N coupled quantum dots with two orbitals in each dot. One orbital is localized (called b orbital) and coupling of the b orbitals in any two dots is negligible; the other is…

Mesoscale and Nanoscale Physics · Physics 2012-05-29 Shiue-Yuan Shiau , Yia-Chung Chang , David M. -T. Kuo

We have calculated components of the torque and the interaction energy of rotating dipole particle in the case where the rotation axis is perpendicular to the surface and the dipole axis is inclined to it. An important property of this…

Mesoscale and Nanoscale Physics · Physics 2012-10-05 A. A. Kyasov , G. V. Dedkov

It is established within the Thomas -- Fermi model that a bound state of a proton with a heavy atom should exist. On the one hand, the electrons of the atom screen the proton's field. This decreases the repulsion force between the proton…

Atomic Physics · Physics 2007-05-23 V. P. Chaly , V. L. Gurevich , M. Yu. Pogorelsky , Yu. V. Pogorelsky

We examine the rotational states of a pair of polar $^2\Sigma$ molecules subject to a uniform magnetic field. The electric dipole-dipole interaction between the molecules creates entangled pair-eigenstates of two types. In one type, the…

Chemical Physics · Physics 2016-05-25 Ketan Sharma , Bretislav Friedrich

We investigate the transient nonequilibrium dynamics of a molecular junction biased by a finite voltage and strongly coupled to internal vibrational degrees of freedom. Using two different, numerical exact techniques, diagrammatic Monte…

Mesoscale and Nanoscale Physics · Physics 2012-10-05 Klaus Ferdinand Albrecht , Haobin Wang , Lothar Muehlbacher , Michael Thoss , Andreas Komnik

We explore electron transport properties for the model of benzene-1, 4-dithiolate (BDT) molecule and for some other geometric models of benzene molecule attached to two semi-infinite one-dimensional metallic electrodes using the Green's…

Mesoscale and Nanoscale Physics · Physics 2010-04-13 Santanu K. Maiti

Test particles interact with a medium by means of a bimolecular reversible chemical reaction. Two species are assumed to be much more numerous so that they are distributed according fixed distributions: Maxwellians and Dirac's deltas.…

Statistical Mechanics · Physics 2009-11-11 A. Rossani , A. M. Scarfone

It is shown that the dipole moment of polar (water, methanol, formamide, acetone and acetonitrile) molecules in the neighborhood of a cation is increased primarily by polarization from the bare electrostatic charge of the cation, although…

Chemical Physics · Physics 2021-03-31 Imre Bakó , Dániel Csókás , István Mayer , Szilvia Pothoczki , László Pusztai

We analyze the collective behavior of hydrodynamically coupled molecular motors. We show that the local fluxes induced by motors displacement can induce the experimentally observed bidirectional motion of cargoes and vesicles. By means of a…

Soft Condensed Matter · Physics 2017-11-22 P. Malgaretti , I. Pagonabarraga , J. F. Joanny

We analyze the interplay between vibrational and electronic degrees of freedom in charge transport across a molecular single-electron transistor. We focus on the wide class of molecules which possess quasi-degenerate vibrational…

Soft Condensed Matter · Physics 2007-05-23 Andrea Donarini , Milena Grifoni , Klaus Richter

Bistability in nanomechanical resonators can be exploited for sensing, signal processing, and memory applications due to its potential for switching and high sensitivity to external stimuli. External vibration can be used to drive a…

Applied Physics · Physics 2025-09-26 Toji Thomas , Kevin F. MacDonald , Eric Plum

Coulomb and spin blockade spectroscopy investigations have been performed on an electrostatically defined ``artificial molecule'' connected to spin polarized leads. The molecule is first effectively reduced to a two-level system by placing…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Pioro-Ladriere , M. Ciorga , J. Lapointe , P. Zawadzki , M. Korkusinski , P. Hawrylak , A. S. Sachrajda

Polar molecules in selected quantum states can be guided, decelerated, and trapped using electric fields created by microstructured electrodes on a chip. Here we explore how transitions between two of these quantum states can be induced…

Atomic Physics · Physics 2015-03-17 Gabriele Santambrogio , Samuel A. Meek , Mark J. Abel , Liam M. Duffy , Gerard Meijer

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Florian Elste , Carsten Timm