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Using a continuum description, we account for fluctuations in the ionic solvent surrounding a Gaussian, charged chain and derive an effective short-ranged potential between the charges on the chain. This potential is repulsive at short…

Soft Condensed Matter · Physics 2009-11-10 Shirish M. Chitanvis

We consider fluids where the attractive interaction at distances slightly larger than the particle size is dominated at larger distances by a repulsive contribution. A previous investigation of the effects of the competition between…

Soft Condensed Matter · Physics 2009-11-11 D. Pini , A. Parola , L. Reatto

Aggregation of stiff polyelectrolytes in solution and angle- and distance-dependent potential of mean force between two like-charged rods are studied in the presence of 3-valent salt using molecular dynamics simulations. In the bulk…

Soft Condensed Matter · Physics 2009-03-25 Sarah Mohammadinejad , Hossein Fazli , Ramin Golestanian

Using integral equation theory of liquids to a binary mixed fluid lipid membrane, we study the membrane-mediated interactions between the macroions and the redistribution of neutral and charged lipids due to binding macroions. We find that…

Soft Condensed Matter · Physics 2015-06-25 Xia-qing Shi , Yu-qiang Ma

We investigate end-effects in the ion distribution around strongly charged, flexible polyelectrolytes with a quenched charge distribution by molecular dynamics simulations of dilute polyelectrolyte solutions. We take the counterions…

Soft Condensed Matter · Physics 2015-06-24 Hans Jörg Limbach , Christian Holm

Effect of ionic solute on a near-critical binary aqueous mixture confined between charged walls with different adsorption preferences is considered within a simple density functional theory. For the near-critical system containing small…

Soft Condensed Matter · Physics 2015-05-28 F. Pousaneh , A. Ciach

Properties of polyelectrolytes in tetravalent salt solutions are intensively investigated by a coarse-grained model. The concentration of salt and the size of tetravalent counterions are found playing a decisive role on chain properties. If…

Soft Condensed Matter · Physics 2009-09-29 Pai-Yi Hsiao

There is growing evidence that slow dynamics and dynamic heterogeneity possess structural signatures in glass-forming liquids. However, even in the weakly frustrated glass-forming liquids, whether or not the dynamic heterogeneity has a…

Soft Condensed Matter · Physics 2015-06-11 Wen-Sheng Xu , Zhao-Yan Sun , Li-Jia An

The effective interaction between two probe particles in a one-dimensional driven system is studied. The analysis is carried out using an asymmetric simple exclusion process with nearest-neighbor interactions. It is found that the driven…

Statistical Mechanics · Physics 2009-11-10 E. Levine , D. Mukamel , G. M. Schutz

Effective attraction between like-charged walls mediated by counterions is studied using local molecular field (LMF) theory. Monte Carlo simulations of the "mimic system'' given by LMF theory, with short-ranged "Coulomb core" interactions…

Statistical Mechanics · Physics 2009-11-11 Jocelyn M. Rodgers , Charanbir Kaur , Yng-Gwei Chen , John D. Weeks

Complexation in symmetric solutions of oppositely charged polyelectrolytes is studied theoretically. We include polyion crosslinking due to formation of thermoreversible ionic pairs. The electrostatic free energy is calculated within the…

Soft Condensed Matter · Physics 2009-11-10 Alexander Kudlay , Alexander V. Ermoshkin , Monica Olvera de la Cruz

We report a mechanism which can lead to long range attractions between like-charged spherical macroions, stemming from the existence of metastable ionized states. We show that the ground state of a single highly charged colloid plus a few…

Soft Condensed Matter · Physics 2009-10-31 Rene Messina , Christian Holm , Kurt Kremer

We report new attractive force between ions that are shielded by degenerate electrons in quantum plasmas. Specifically, we show that the electric potential around an isolated ion has a hard core negative part that resembles the…

Plasma Physics · Physics 2012-08-13 Padma Kant Shukla , Bengt Eliasson

The persistence length of a single, strongly charged, stiff polyelectrolyte chain is investigated theoretically. Path integral formulation is used to obtain the effective electrostatic interaction between the monomers. We find significant…

Soft Condensed Matter · Physics 2009-11-07 Gil Ariel , David Andelman

We present theoretical and numerical studies on stiff, linear polyelectrolytes within the framework of the cell model. We first review analytical results obtained on a mean-field Poisson-Boltzmann level, and then use molecular dynamics…

Soft Condensed Matter · Physics 2009-11-07 Markus Deserno , Christian Holm

Charge correlations in dense ionic fluids give rise to novel effects such as long-range screening and colloidal stabilization which are not predicted by the classic Debye-Huckel theory. We show that a Coulomb or charge-frustrated Ising…

Soft Condensed Matter · Physics 2018-11-01 Nicholas B. Ludwig , Kinjal Dasbiswas , Dmitri V. Talapin , Suriyanarayanan Vaikuntanathan

The long range attractive force between two hydrophobic surfaces immersed in water is observed to decrease exponentially with their separation -- this distance-dependence of effective force is known as the hydrophobic force law (HFL). We…

Soft Condensed Matter · Physics 2015-06-24 Saikat Banerjee , Rakesh S. Singh , Biman Bagchi

Conditions at which a quasi-one-dimensional (1D) electron system can be considered as a quantum liquid of impenetrable charged particles are theoretically analyzed. In the presence of an inert, neutralizing background, a motion of…

Superconductivity · Physics 2024-06-21 Yu. P. Monarkha

The electrostatic screening length predicted by Debye-H\"uckel theory decreases with increasing ionic strength, but recent experiments have found that the screening length can instead increase in concentrated electrolytes. This phenomenon,…

Soft Condensed Matter · Physics 2021-10-13 Emily Krucker-Velasquez , James W. Swan

Molecular dynamics simulations have been used extensively to determine equilibrium properties of the electrode-electrolyte interface in supercapacitors held at various potentials. While such studies are essential to understand and optimize…

Soft Condensed Matter · Physics 2024-02-26 Nicolas Gaudy , Mathieu Salanne , Céline Merlet