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Using density functional theory we calculate the density profiles of a binary solvent adsorbed around a pair of big solute particles. All species interact via repulsive Gaussian potentials. The solvent exhibits fluid-fluid phase separation…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , R. Evans , R. Roth , M. Oettel

The effective interaction between two planar walls immersed in a fluid is investigated by use of Density Functional Theory in the super-critical region of the phase diagram. A hard core Yukawa model of fluid is studied with special…

Statistical Mechanics · Physics 2017-04-05 Pietro Anzini , Alberto Parola

We determine the solvent mediated contribution to the effective potentials for model colloidal or nano- particles dispersed in a binary solvent that exhibits fluid-fluid phase separation. Using a simple density functional theory we…

Soft Condensed Matter · Physics 2011-06-24 Paul Hopkins , Andrew J. Archer , Robert Evans

As a first step towards a microscopic understanding of the effective interaction between colloidal particles suspended in a solvent we study the wetting behavior of one-component fluids at spheres and fibers. We describe these phenomena…

Condensed Matter · Physics 2015-06-25 T. Bieker , S. Dietrich

Particle segregation in dense flowing size-disperse granular mixtures is driven by gravity and shear, but predicting the associated segregation force due to both effects has remained an unresolved challenge. Here, a model of the combined…

Soft Condensed Matter · Physics 2024-11-20 Yifei Duan , Lu Jing , Paul B. Umbanhowar , Julio M. Ottino , Richard M. Lueptow

We use microscopic density functional theory to study filling transitions in systems with long-ranged wall-fluid and short-ranged fluid-fluid forces occurring in a right-angle wedge. By changing the strength of the wall-fluid interaction we…

Statistical Mechanics · Physics 2016-05-04 Alexandr Malijevský , Andrew O. Parry

The influence of poor solvent quality on fluid demixing of a model mixture of colloids and nonadsorbing polymers is investigated using density functional theory. The colloidal particles are modelled as hard spheres and the polymer coils as…

Soft Condensed Matter · Physics 2009-11-07 Matthias Schmidt , Alan R. Denton

Nanoscopic pores are used in various systems to attract nanoparticles. In general the behaviour is a result of two types of interactions: the material specific affinity and the solvent-mediated influence also called the depletion force. The…

Soft Condensed Matter · Physics 2018-03-02 Julien Lam , James F. Lutsko

We show that the Gaussian core model of particles interacting via a penetrable repulsive Gaussian potential, first considered by Stillinger (J. Chem. Phys. 65, 3968 (1976)), behaves like a weakly correlated ``mean field fluid'' over a…

Soft Condensed Matter · Physics 2009-10-31 A. A. Louis , P. G. Bolhuis , J. P. Hansen

We discuss the simple microscopic derivation of a hydrophobic effect. Our approach is based on the standard functional representation of the partition function of interacting classical particles and subsequent passage to collective…

Statistical Mechanics · Physics 2016-08-31 G. Sitnikov , S. Nechaev

The equation of the density field of an assembly of macroscopic particles advected by a hydrodynamic flow is derived from the microscopic description of the system. This equation allows to recognize the role and the relative importance of…

Chaotic Dynamics · Physics 2016-09-08 Cristobal Lopez , Andrea Puglisi

A micro-hydrodynamics model based on elastic collisions of light point solvent particles with a heavy solute particle is investigated in the setting where the light particles have velocity distribution corresponding to a background flow.…

Fluid Dynamics · Physics 2023-11-21 Radek Erban , Robert A. Van Gorder

The connection between fundamental interactions acting in molecules in a fluid and macroscopically measured properties, such as the viscosity between colloidal particles coated with polymers, is studied here. The role that hydrodynamic and…

Soft Condensed Matter · Physics 2015-09-02 A. Gama Goicochea , M. A. Balderas Altamirano , R. Lopez-Esparza , M. A. Waldo , E. Perez

The Morse-Witten theory (D. Morse and T. Witten, EPL 22 (1993) 549-555) provides a formulation for the inter-bubble forces and corresponding deformations in a liquid foam, accurate in the limit of high liquid fraction. Here we show how the…

Soft Condensed Matter · Physics 2019-08-13 Friedrich F. Dunne , Jens Winkelmann , Denis Weaire , Stefan Hutzler

This work is concerned with a simple model for a polar fluid, a Gaussian field model based on the excess density and on the polarization. It is a convenient framework to implement the dielectric properties of correlated liquids that stem…

Chemical Physics · Physics 2018-04-04 Hélène Berthoumieux

Solvation of small and large clusters are studied by simulation, considering a range of solvent-solute attractive energy strengths. Over a wide range of conditions, both for solvation in the Lennard-Jones liquid and in the SPC model of…

Statistical Mechanics · Physics 2007-07-29 Lutz Maibaum , David Chandler

We present a simple density functional theory for the solid phases of systems of particles interacting via soft-core potentials. In particular, we apply the theory to particles interacting via repulsive point Yukawa and Gaussian pair…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer

The method to calculate the grand partition function of a particle system, in which constituents interact with each other via potential, that include repulsive and attractive components, is proposed. The cell model, which was introduced to…

Statistical Mechanics · Physics 2016-04-14 Mikhailo Kozlovskii , Oksana Dobush

We present a density-functional study of a binary phase-separating mixture of soft core particles immersed in a random matrix of quenched soft core particles of larger size. This is a model for a binary polymer mixture immersed in a…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , M. Schmidt , R. Evans

We analyze the depletion interaction between two hard colloids in a hard--sphere solvent and pay special attention to the limit of large size ratio between colloids and solvent particles which is governed by the well--known Derjaguin…

Soft Condensed Matter · Physics 2007-05-23 M. Oettel
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