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We investigate the structure of 13-particle clusters in binary alloys for various size ratios and different concentrations via MD simulation. Our goal is to predict which systems are likely to form local icosahedral structures when rapidly…

Condensed Matter · Physics 2007-05-23 Stefano Cozzini , Marco Ronchetti

The global minima of clusters bound by a Dzugutov potential form non-compact polytetrahedral clusters mainly composed of interpenetrating and face-sharing 13-atom icosahedra. As the size increases, these icosahedral units first form linear…

Condensed Matter · Physics 2007-05-23 Jonathan Doye , David Wales , Sergei Simdyankin

We present an operational method to determine the 'locally preferred structure'' of model liquids, a notion often put forward to explain supercooling of a liquid and glass formation. The method relies on finding the global minimum in the…

Disordered Systems and Neural Networks · Physics 2011-05-05 S. Mossa , G. Tarjus

The atomic structure of the supercooled liquid has often been discussed as a key source of glass formation in metals. The presence of icosahedrally-coordinated clusters and their tendency to form networks have been identified as one…

Materials Science · Physics 2013-10-30 Logan Ward , Dan Miracle , Wolfgang Windl , Oleg Senkov , Katharine Flores

We use the ``isoconfigurational ensemble'' [Phys. Rev. Lett. {\bf 93}, 135701 (2004)] to analyze both dynamical and structural properties in simulations of a glass forming molecular liquid. We show that spatially correlated clusters of low…

Materials Science · Physics 2009-11-11 Gurpreet S. Matharoo , M. S. Gulam Razul , Peter H. Poole

Putative global minima have been located for clusters interacting with an aluminium glue potential for N<190. Virtually all the clusters have polytetrahedral structures, which for larger sizes involve an ordered array of disclinations that…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye

We have attempted to find the global minima of clusters containing between 20 and 80 atoms bound by the Morse potential as a function of the range of the interatomic force. The effect of decreasing the range is to destabilize strained…

Condensed Matter · Physics 2008-02-03 Jonathan Doye , David Wales

Zinc and cadmium clusters interacting with a Gupta potential have previously been identified as prototypical metallic systems that exhibiting disordered cluster structures. Here, putative global minima of the potential energy have been…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye

We have located the global minimum for all lead clusters with up to 160 atoms using a glue potential to model the interatomic interactions. The lowest-energy structures are not face-centred cubic as suggested previously. Rather, for N<40…

Condensed Matter · Physics 2007-05-23 Jonathan P. K. Doye , Shaun C. Hendy

The liquid structure of a glass-forming binary alloy is studied using molecular dynamics simulations. The analysis combines common neighbour analysis with the geometrical approach of Frank and Kasper to establish that the supercooled liquid…

Soft Condensed Matter · Physics 2010-03-11 Ulf R. Pedersen , Thomas B. Schrøder , Jeppe C. Dyre , Peter Harrowell

We investigate the formation of cluster crystals with multiply occupied lattice sites on a spherical surface in systems of ultra-soft particles interacting via repulsive, bounded pair potentials. Not all interactions of this kind lead to…

Soft Condensed Matter · Physics 2018-07-31 Stefano Franzini , Luciano Reatto , Davide Pini

Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…

Soft Condensed Matter · Physics 2016-10-18 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

We numerically investigate slow dynamics of a binary mixture of ultrasoft particles interacting with the generalized Hertzian potential. If the softness parameter, $\alpha$, is small, the particles at high densities start penetrating each…

Soft Condensed Matter · Physics 2019-03-27 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

During the solidification of Al-Sm metallic glasses the evolution of the supercooled liquid atomic structure has been identified with an increasing population of icosahedral-like clusters with increasing Sm concentration. These clusters…

Computational Physics · Physics 2016-08-04 G. B. Bokas , L. Zhao , J. H. Perepezko , I. Szlufarska

Colloidal particles, amphiphiles, and functionalized nanoparticles are examples of systems that frequently exhibit short-range attractions coupled with long-range repulsions. In this work, we observe striking differences in the dynamics of…

Soft Condensed Matter · Physics 2017-06-01 Jakub Pȩkalski , Andrew P. Santos , Athanassios Z. Panagiotopoulos

We present computer simulations of concentrated solutions of unknotted nonconcatenated semiflexible ring polymers. Unlike in their flexible counterparts, shrinking involves a strong energetic penalty, favoring interpenetration and…

We investigate the ordering properties of vertically-vibrated monolayers of granular cylinders in a circular container at high packing fraction. In line with previous works by other groups, we identify liquid-crystalline ordering behaviour…

Soft Condensed Matter · Physics 2017-05-16 Miguel Gonzalez-Pinto , Florentino Borondo , Yuri Martinez-Raton , Enrique Velasco

Although the existence of 13-atom icosahedral clusters in one-component close-packed undercooled liquids was predicted more than half a century ago by Frank, the existence of such icosahedral clusters is less clear in liquid alloys. We…

Materials Science · Physics 2009-11-13 M. Iwamatsu , S. K. Lai

The mechanical, optical, and chemical properties of a wide variety of soft materials are enabled and constrained by their bulk structure. How this structure emerges at small system sizes during self-assembly has been the subject of decades…

Soft Condensed Matter · Physics 2024-12-09 Jennifer E. Doyle , Maya M. Martirossyan , Julia Dshemuchadse , Erin G. Teich

Putative global minima of sodium clusters with up to 380 atoms have been located for two model interatomic potentials. Structures based upon the Mackay icosahedra predominate for both potentials, and the magic numbers for the…

Other Condensed Matter · Physics 2007-06-13 Eva G. Noya , Jonathan P. K. Doye , David J. Wales
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