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A novel integral equations approach is applied for studying ion pairing in the restricted primitive model (RPM) electrolyte, i. e., the three point extension (TPE) to the Ornstein-Zernike integral equations. In the TPE approach, the…

Soft Condensed Matter · Physics 2007-05-23 Felipe Jimenez-Angeles , Rene Messina , Christian Holm , Marcelo Lozada-Cassou

We relate the phase separation observed in many crystals with pronounced electron correlations to the regions of negative electron compressibility. They were found in several models describing strong electron correlations. At low…

Strongly Correlated Electrons · Physics 2022-10-25 Alexei Sherman

For single-file translocations of a charged macromolecule through a narrow pore, the crucial step of arrival of an end at the pore suffers from free energy barriers, arising from changes in intrachain electrostatic interaction, distribution…

Soft Condensed Matter · Physics 2015-05-14 Rajeev Kumar , M. Muthukumar

The high efficiency of charge generation within organic photovoltaic blends apparently contrasts with the strong "classical" attraction between newly formed electron-hole pairs. Several factors have been identified as possible facilitators…

Mesoscale and Nanoscale Physics · Physics 2017-09-07 Mosè Casalegno , Raffaele Pastore , Julien Idé , Riccardo Po , Guido Raos

Photoelectrochemical (PEC) water splitting offers an elegant approach for solar energy conversion into hydrogen fuel. Large-scale hydrogen production requires stable and efficient photoelectrodes and scalable PEC cells that are fitted for…

We present for the first time a complex network approach to the study of the electrical properties of single protein devices. In particular, we consider an electronic nanobiosensor based on a G-protein coupled receptor. By adopting a coarse…

Molecular Networks · Quantitative Biology 2009-11-10 C. Pennetta , V. Akimov , E. Alfinito , L. Reggiani , G. Gomila

The issues of electronic polarizability in molecular dynamics simulations are discussed. We argue that the charges of ionized groups in proteins, and charges of ions in conventional non-polarizable force fields such as CHARMM, AMBER,…

Chemical Physics · Physics 2017-09-13 Igor Leontyev , Alexei Stuchebrukhov

Identification and characterization of large protein complexes is a mainstay of biochemical toolboxes. Utilization of cross-linking chemicals can facilitate the capture and identification of transient or weak interactions of a transient…

Molecular Networks · Quantitative Biology 2016-06-15 Timothy D. Cummins , Gopal P. Sapkota

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes onto a charged spherical surface is investigated by means of Monte Carlo simulations in a fashion which resembles the layer-by-layer deposition technique…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer

We present in this paper an original approach to compute the electrophoretic mobility of rigid nucleo-protein complexes like nucleosomes. This model allows to address theoretically the influence of complex position along DNA, as well as…

Biological Physics · Physics 2016-08-14 Martin Castelnovo , Sébastian Grauwin

We present a theoretical study of dielectrophoretic (DEP) crossover spectrum of two polarizable particles under the action of a nonuniform AC electric field. For two approaching particles, the mutual polarization interaction yields a change…

Chemical Physics · Physics 2007-05-23 J. P. Huang , Mikko Karttunen , K. W. Yu , L. Dong

We investigate the thermodynamic properties of a polyelectrolyte solution in a presence of {\it multivalent} salts. The polyions are modeled as rigid cylinders with the charge distributed uniformly along the major axis. The solution,…

Condensed Matter · Physics 2015-06-25 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

Essential protein plays a crucial role in the process of cell life. The identification of essential proteins can not only promote the development of drug target technology, but also contribute to the mechanism of biological evolution. There…

Molecular Networks · Quantitative Biology 2020-05-20 Pengli Lu , JingJuan Yu

The electrical double layer (EDL) is fundamental to the operation of devices for electrochemical energy storage and conversion. Existing models of EDL in solid electrolytes focus predominantly on the space charge layer and lack a complete…

Materials Science · Physics 2025-08-12 Zeeshan Ahmad

The complexation of a polyelectrolyte with an oppositely charged spherical macroion is studied for both salt free and salty solutions. When a polyelectrolyte winds around the macroion, its turns repel each other and form an almost…

Soft Condensed Matter · Physics 2009-10-31 T. T. Nguyen , B. I. Shklovskii

We have developed a multiple image method to compute the interparticle force for a polydisperse electrorheological (ER) fluid. We apply the formalism to a pair of dielectric spheres of different dielectric constants and calculate the force…

Soft Condensed Matter · Physics 2007-05-23 Y. L. Siu , Jones T. K. Wan , K. W. Yu

We report results from a molecular dynamics (MD) simulation on the conformations of a long flexible polyelectrolyte complexed to a charged sphere, \textit{both negatively charged}, in the presence of neutralizing counterions in the strong…

Soft Condensed Matter · Physics 2009-11-07 Rene Messina , Christian Holm , Kurt Kremer

This paper investigates the problem of electrophoretic motion of a polyelectrolyte capsule with a porous arbitrary charged conducting shell in an electrolyte under the action of an external electric field. The corresponding boundary value…

Fluid Dynamics · Physics 2021-08-11 Anatoly N. Filippov , Daria Yu. Khanukaeva , Petr A. Aleksandrov

We present a Ginzburg-Landau theory of inhomogeneous polyelectrolytes with a polar solvent. First, we take into account the molecular (solvation) interaction among the ions, the charged monomers, the uncharged monomers, and the solvent…

Soft Condensed Matter · Physics 2009-03-10 Akira Onuki , Ryuichi Okamoto

We study salt-induced charge overcompensation and charge inversion of flexible polyelectrolytes via computer simulations and demonstrate the importance of ion excluded volume. Reentrant condensation takes place when the ion size is…

Soft Condensed Matter · Physics 2008-06-26 Pai-Yi Hsiao
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