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This paper reviews recent Monte Carlo simulation studies of the glassy behavior in thin polymer films. The simulations employ a version of the bond-fluctuation lattice model, in which the glass transition is driven by the competition…

Soft Condensed Matter · Physics 2007-05-23 C. Mischler , J. Baschnagel , K. Binder

We calculate the ideal-glass-transition line for adhesive hard spheres in the temperature-volume-fraction plane within the framework of the mode-coupling theory. We find two intersecting lines, controlled by the hard-core and the adhesive…

Soft Condensed Matter · Physics 2019-08-17 L. Fabbian , W. Goetze , F. Sciortino , P. Tartaglia , F. Thiery

We investigate how structural relaxation in mixtures with strong dynamical asymmetry is affected by the microscopic dynamics. Brownian and Newtonian dynamics simulations of dense mixtures of fast and slow hard spheres reveal a striking…

Soft Condensed Matter · Physics 2017-10-02 Suvendu Mandal , Thomas Franosch , Thomas Voigtmann

We calculate for a binary mixture of Lennard-Jones particles the time dependence of the solution of the mode-coupling equations in which the full wave vector dependence is taken into account. In addition we also take into account the short…

Statistical Mechanics · Physics 2009-11-07 Walter Kob , Markus Nauroth , Francesco Sciortino

We discuss a schematic model of mode-coupling theory for force-driven active nonlinear microrheology, where a single probe particle is pulled by a constant external force through a dense host medium. The model exhibits both a glass…

Soft Condensed Matter · Physics 2018-07-11 Manuel Victor Gnann , Thomas Voigtmann

We study swelling and structural properties of ionic microgel suspensions within a comprehensive coarse-grained model that combines the polymeric and colloidal natures of microgels as permeable, compressible, charged spheres governed by…

Soft Condensed Matter · Physics 2018-06-07 Tyler J. Weyer , Alan R. Denton

We present a theory for the single-particle dynamics in binary mixtures with particle size swaps. The general structure of the theory follows that of the theory for the collective dynamics in binary mixtures with particle size swaps, which…

Soft Condensed Matter · Physics 2019-11-18 Grzegorz Szamel

We study -- using molecular dynamics simulations -- the temperature dependence of the dynamics in a dense short-ranged attractive colloidal glass to find evidence of the kinetic glass-glass transition predicted by the ideal Mode Coupling…

Disordered Systems and Neural Networks · Physics 2009-11-10 Emanuela Zaccarelli , Giuseppe Foffi , Francesco Sciortino , Piero Tartaglia

Analysis of the thermo-mechanical behaviour of polymers has been and still is the subject of many rheological studies both experimentally and theoretically. For small deformations, the modelling framework retained by rheologists is often of…

Soft Condensed Matter · Physics 2019-04-05 Pankaj Yadav , Andre Chrysochoos , Olivier Arnould , Sandrine Bardet

We study structural properties of a ring polymeric melt confined in a film in comparison to a linear counterpart using molecular dynamics simulations. Local structure orderings of ring and linear polymers in the vicinity of the surface are…

Soft Condensed Matter · Physics 2015-10-21 Eunsang Lee , YounJoon Jung

We study the nonlinear rheology of a glass-forming binary mixture under the reversal of shear flow using molecular dynamics simulations and a schematic model of the mode-coupling theory of the glass transition (MCT). Memory effects lead to…

Soft Condensed Matter · Physics 2015-06-12 Fabian Frahsa , Amit Kumar Bhattacharjee , Jürgen Horbach , Matthias Fuchs , Thomas Voigtmann

Hybrid molecular dynamics/Monte Carlo simulations used to study melts of unentangled, thermoreversibly associating supramolecular polymers. In this first of a series of papers, we describe and validate a model that is effective in…

Soft Condensed Matter · Physics 2015-05-13 Robert S. Hoy , Glenn H. Fredrickson

We present a mode-coupling theory (MCT) for the high-density dynamics of two-dimensional spherical active Brownian particles (ABP). The theory is based on the integration-through-transients (ITT) formalism and hence provides a starting…

Soft Condensed Matter · Physics 2017-12-20 Alexander Liluashvili , Jonathan Onody , Thomas Voigtmann

We use thermodynamic perturbation theory to calculate the free energies and resulting phase diagrams of binary systems of spherical colloidal particles and interacting polymer coils in good solvent within an effective one-component…

Soft Condensed Matter · Physics 2009-11-10 B. Rotenberg , J. Dzubiella , J. -P. Hansen , A. A. Louis

Coupled mode theory (CMT) is a powerful framework for decomposing interactions between electromagnetic waves and scattering bodies into resonances and their couplings with power-carrying channels. It has widespread use in few-resonance,…

Optics · Physics 2020-10-22 Hanwen Zhang , Owen D. Miller

Conformation-dependent design of polymer sequences can be considered as a tool to control macromolecular self-assembly. We consider the monomer unit sequences created via the modification of polymers in a homogeneous melt in accordance with…

Soft Condensed Matter · Physics 2021-07-07 Elena N. Govorun , Ruslan M. Shupanov , Sophia A. Pavlenko , Alexei R. Khokhlov

We introduce a new model of random layered media, extending the Matheron-de Marsily model: Here we allow for the flows to change in time. For such layered structures, we solve exactly the equations of motion for single particles, and also…

Statistical Mechanics · Physics 2009-10-31 S. Jespersen , G. Oshanin , A. Blumen

We suggest a new focus for turbulence studies -- multi-mode correlations -- which reveal the hitherto hidden nature of turbulent state. We apply this approach to shell models describing basic properties of turbulence. The family of such…

Chaotic Dynamics · Physics 2023-08-08 Gregory Falkovich , Yotam Kadish , Natalia Vladimirova

Using extensive computer simulations, the behavior of the structural modes --- more precisely, the eigenmodes of a phantom Rouse polymer --- are characterized for a polymer in the three-dimensional repton model, and are used to study the…

Soft Condensed Matter · Physics 2015-03-18 Gerard T. Barkema , Debabrata Panja , J. M. J. van Leeuwen

Critical slowing down dynamics of supercooled glass-forming liquids is usually understood at the mean-field level in the framework of Mode Coupling Theory, providing a two-time relaxation scenario and power-law behaviors of the time…

Disordered Systems and Neural Networks · Physics 2013-01-30 Ulisse Ferrari , Luca Leuzzi , Giorgio Parisi , Tommaso Rizzo
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