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Accurate atomic structure calculations of complicated atoms with 4 or more valence electrons begin to push the memory and time limits of supercomputers. This paper presents a robust method of decreasing the size of \textit{ab initio}…

Atomic Physics · Physics 2018-10-24 A. J. Geddes , D. A. Czapski , E. V. Kahl , J. C. Berengut

Semi-empirical interatomic potentials have been developed for Al, alpha-Ti, and gamma-TiAl within the embedded atomic method (EAM) by fitting to a large database of experimental as well as ab-initio data. The ab-initio calculations were…

Materials Science · Physics 2009-11-10 Rajendra R. Zope , Y. Mishin

Establishing the phase diagram of hydrogen is a major challenge for experimental and theoretical physics. Experiment alone cannot establish the atomic structure of solid hydrogen at high pressure, because hydrogen scatters X-rays only…

Single cluster covering approach provides a plausible mechanism for the formation and stability of octagonal and decagonal quasiperiodic structures. For dodecagonal quasiperiodic pattern such a single cluster covering scheme is still…

Other Condensed Matter · Physics 2015-06-11 Longguang Liao , Zexian Cao

While density functional theory (DFT) serves as a prevalent computational approach in electronic structure calculations, its computational demands and scalability limitations persist. Recently, leveraging neural networks to parameterize the…

Computational Physics · Physics 2024-06-18 Yang Zhong , Hongyu Yu , Jihui Yang , Xingyu Guo , Hongjun Xiang , Xingao Gong

Jellium model achieved great success in predicting stable clusters with closed electronic shells and zero spin. In order to explain the stability of open shell clusters, it is necessary to consider the case of non-degenerate energy levels.…

Materials Science · Physics 2022-09-30 Jin Liu , Zhi-Jie Yan , YI-Chao Jin , Meng Zhang

In pursuit of a colloidal analogue to quantum density functional theory (DFT) predictions of atomic crystal structures, we report a new, classical DFT that predicts the relative thermodynamic stability of colloidal crystals of hard, convex…

Soft Condensed Matter · Physics 2026-01-15 Kristi Pepa , Isaac R. Spivack , Trevor F. G. Teague , Ryn Y. Oliphant , Domagoj Fijan , Sharon C. Glotzer

We have investigated structure and properties of small metal clusters using all-electron ab initio theoretical methods based on the Hartree-Fock approximation and density functional theory, perturbation theory and compared results of our…

Atomic and Molecular Clusters · Physics 2009-11-07 Ilia A. Solov'yov , Andrey V. Solov'yov , Walter Greiner

The full design of relevant systems for quantum applications, ranging from quantum simulation to sensing, is presented using a combination of atomistic methods. A prototypical system features a two-dimensional ordered distribution of spins…

Quasicrystals are fascinating structures, characterized by strong positional order but lacking the periodicity of a crystal. In colloidal systems, quasicrystals are typically predicted for particles with complex or highly specific…

Soft Condensed Matter · Physics 2022-02-28 Etienne Fayen , Marianne Impéror-Clerc , Laura Filion , Giuseppe Foffi , Frank Smallenburg

The intermetallic $\tau_{11}$ Al$_4$Fe$_{1.7}$Si phase is of interest for high-temperature structural application due to its combination of low density and high strength. We determine the crystal structure of the $\tau_{11}$ phase through a…

Quantum Monte Carlo (QMC) is an advanced simulation methodology for studies of manybody quantum systems. In this review, we focus on the electronic structure QMC, i.e., methods relevant for systems described by the electron-ion…

Other Condensed Matter · Physics 2010-08-16 Michal Bajdich , Lubos Mitas

We discuss a computationally efficient classical many-body potential designed to model the Al-Al interaction in a wide range of bonding geometries. We show that the potential yields results in properties in excellent agreement with…

Materials Science · Physics 2009-10-31 U. Hansen , P. Vogl , V. Fiorentini

Accuracy of molecular dynamics simulations depends crucially on the interatomic potential used to generate forces. The gold standard would be first-principles quantum mechanics (QM) calculations, but these become prohibitively expensive at…

We describe a way to obtain a two-dimensional quasiperiodic tiling with eight-fold symmetry using cold atoms. A series of such optical tilings, related by scale transformations, is obtained for a series of specific values of the chemical…

Quantum Gases · Physics 2016-09-29 Nicolas Macé , Anuradha Jagannathan , Michel Duneau

The atomic and electronic structures of Pd3N, PdN and PdN2 were investigated using ab initio density-functional theory (DFT). We studied cohesive energy vs. volume equation of states (EOS) for a set of reported and hypothetical structures.…

Materials Science · Physics 2013-10-11 Mohammed S. H. Suleiman , Daniel P. Joubert

Multi-principle element alloys have enormous potential, but their exploration suffers from the tremendously large range of configurations. In the last decade such alloys have been designed with a focus on random solid solutions. Here we…

Materials Science · Physics 2017-02-15 Lukasz Rogal , Piotr Bobrowski , Fritz Koermann , Sergiy Divinski , Frank Stein , Blazej Grabowski

In antecedent experiments the electron screening energies of the d+d reactions in metallic environments have been determined to be enhanced by an order of magnitude in comparison to the case of gaseous deuterium targets. The analytical…

Nuclear Theory · Physics 2008-11-26 A. Huke , K. Czerski , S. M. Chun , A. Biller , P. Heide

Chemical interaction and changes in local electronic structure of Cr, Fe, Co, Ni and Cu transition metals (TMs) upon formation of an $Al_{8}Co_{17}Cr_{17}Cu_{8}Fe_{17}Ni_{33}$ compositionally complex alloy (CCA) have been studied by X-ray…

In the present paper, we have studied atomic structure of nitrogenous austenite. High precision ab-initio calculation was utilized for the calculation of the pair potentials of interatomic interactions N-N in FCC Fe lattice. These…

Atomic and Molecular Clusters · Physics 2011-12-01 A. N. Timoshevskii , S. O. Yablonovskii
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