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We calculate the vibrational density-of-states in an insulating nanoparticle that is in weak mechanical contact with a semi-infinite substrate. The work is motivated by a recent experiment by Yang et al., where the low-energy phonon…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Kelly R. Patton , Michael R. Geller

We discuss the rich vibrational dynamics of nanometer-scale semiconducting and insulating crystals as probed by localized electronic impurity states, with an emphasis on nanoparticles that are only weakly coupled to their environment. Two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Michael R. Geller , W. M. Dennis , Vadim A. Markel , Kelly R. Patton , Daniel T. Simon , Ho-Soon Yang

The low-frequency vibrational spectrum of an isolated nanometer-scale solid differs dramatically from that of a bulk crystal, causing the decay of a localized electronic state by phonon emission to be inhibited. We show, however, that an…

Materials Science · Physics 2009-10-31 Ho-Soon Yang , Michael R. Geller , W. M. Dennis

The nanocrystallite have the finite number of the oscillation modes. Their number increases proportionally to a cube of the characteristic size. Thus the oscillation spectrum of nanocrystal becomes discrete, and the separate modes of…

Superconductivity · Physics 2010-12-21 V. G. Andreev , L. V. Kravchuk , S. G. Lebedev

Nanoparticles levitated in vacuum can be set to spin at ultimate frequencies, limited only by the tensile strength of the material. At such high frequencies, drastic changes to the dynamics of solid-state quantum excitations are to be…

Mesoscale and Nanoscale Physics · Physics 2020-05-14 Daniel Hümmer , René Lampert , Katja Kustura , Patrick Maurer , Carlos Gonzalez-Ballestero , Oriol Romero-Isart

The features of phonon spectra and their effect on the vibrational heat capacity of linear chains of inert gas atoms adsorbed onto a substrate, which is the surface of nanotubes bound to a nanobundle. The influence of the substrate results…

Mesoscale and Nanoscale Physics · Physics 2025-06-26 E. V. Manzhelii , S. B. Feodosyev , I. A. Gospodarev

Dynamics of dissipation of a local phonon distribution to the substrate is a key issue in friction between sliding surfaces as well as in boundary lubrication. We consider a model system consisting of an excited nano-particle which is…

Other Condensed Matter · Physics 2009-11-13 Haldun Sevinçli , Soma Mukhopadhyay , R. Tugrul Senger , Salim Ciraci

The spectrum of acoustic vibrational modes of an inhomogeneous elastic continuum are analyzed with application to a spherical nanoparticle embedded in an infinite glass block. The relationship of these modes to the discrete vibrational…

Materials Science · Physics 2007-05-23 Daniel B. Murray , Lucien Saviot

Nanostructured rare-earth-ion doped materials are increasingly being investigated for on-chip implementations of quantum information processing protocols as well as commercial applications such as fluorescent lighting. However, achieving…

Mesoscale and Nanoscale Physics · Physics 2018-09-12 Thomas Lutz , Lucile Veissier , Philip J. T. Woodburn , Rufus L. Cone , Paul E. Barclay , Wolfgang Tittel , Charles W. Thiel

This study presents a comprehensive computational investigation of magnetite nanoparticles, systematically evaluating a range of force fields against experimental results. We analyze the influence of particle size, temperature, and…

Materials Science · Physics 2025-10-13 Pablo Galaviz , Kyle A. Portwin , Dehong Yu , Kirrily C. Rule , David L. Cortie , Zhenxiang Cheng

In order to clarify the relationship between the phonon spectra of nanoparticles and their melting temperature, we studied in detail the size-dependent low energy vibration modes. A minimum model with atoms on a lattice and harmonic…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Kai Kang , Shaojing Qin , Chuilin Wang

We study the effect of the electromagnetic environment on the resonance frequency of plasmonic excitations in dimers of interacting metallic nanoparticles. The coupling between plasmons and vacuum electromagnetic fluctuations induces a…

Mesoscale and Nanoscale Physics · Physics 2017-10-11 Charles A. Downing , Eros Mariani , Guillaume Weick

We study theoretically spectrum of radial vibrational modes in composite metal nanostructures such as bimetallic core-shell particles and metal nanoshells with dielectric core in an environment. We calculate frequencies and damping rates of…

Materials Science · Physics 2008-08-27 Arman S. Kirakosyan , Tigran V. Shahbazyan

Nanoscale single-crystals possess modified phonon dispersions due to the truncation of the crystal. The introduction of surfaces alters the population of phonons relative to the bulk and introduces anisotropy arising from the breaking of…

Mesoscale and Nanoscale Physics · Physics 2020-02-27 Kyle M. McElhinny , Gokul Gopalakrishnan , Martin V. Holt , David A. Czaplewski , Paul G. Evans

The elastic response of suspended NbSe3 nanowires is studied across the charge density wave phase transition. The nanoscale dimensions of the resonator lead to a large resonant frequency (10-100 MHz), bringing the excited phonon frequency…

In the present paper, we utilize the coupled-oscillator model describing the hybridization of optical phonons in touching and/or overlapping particles in order to study the Raman spectra of nanoparticles organized into various types of…

Mesoscale and Nanoscale Physics · Physics 2023-12-01 S. V. Koniakhin , O. I. Utesov , A. G. Yashenkin

Phonons play a key role in the physical properties of materials, and have long been a topic of study in physics. While the effects of phonons had historically been considered to be a hindrance, modern research has shown that phonons can be…

The coupling effects affecting the vibrations of two close nanostructures (e.g., two metal nanoplates or nanospheres separated by a thin dielectric layer) may considerably alter their vibrational eigenfrequencies, as demonstrated by several…

Applied Physics · Physics 2021-05-06 Jean Lermé , Jérémie Margueritat , Aurélien Crut

Based on a description of an amorphous solid as a collection of coupled nanosize molecular clusters referred as basic blocks, we analyse the statistical properties of its Hamiltonian. The information is then used to derive the ensemble…

Statistical Mechanics · Physics 2021-08-24 Pragya Shukla

We investigate the electron population dynamics in an ensemble of nearly isolated insulating nanoparticles, each nanoparticle modeled as an electronic two-level system coupled to a single vibrational mode. We find that at short times the…

Materials Science · Physics 2009-10-31 Daniel T. Simon , Michael R. Geller
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