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We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…

Condensed Matter · Physics 2007-05-23 Igor Tupitsyn , Bernard Barbara

We investigate the spin- and energy dependent tunneling through a single organic molecule (CoPc) adsorbed on a ferromagnetic Fe thin film, spatially resolved by low-temperature spin-polarized scanning tunneling microscopy. Interestingly,…

Process of quantum tunneling of particles in various physical systems can be effectively controlled even by a weak and slow varying in time electromagnetic signal if to adapt specially its shape to a particular system. During an…

Quantum Physics · Physics 2009-02-05 B. I. Ivlev

Molecular nanomagnets are quantum spin systems potentially serving as qudits for future quantum technologies thanks to their many accessible low-energy states. At low temperatures, the primary source of error in these systems is pure…

A spin (qubit) is in contact with a bosonic reservoir. The state of the reservoir contains a parameter {\varepsilon} interpolating between quantum and classical reservoir features. We derive the explicit expression for the time-dependent…

Quantum Physics · Physics 2024-12-11 Michele Correggi , Marco Falconi , Michele Fantechi , Marco Merkli

We study the macroscopic quantum tunneling of magnetization of the F=1 spinor condensate interacting through dipole-dipole interaction with an external magnetic field applied along the longitudinal or transverse direction. We show that the…

Other Condensed Matter · Physics 2007-05-23 Limin Yang , Yunbo Zhang

Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. Such applications require protection of the spin states against quantum decoherence due to interactions with…

Mesoscale and Nanoscale Physics · Physics 2018-11-13 Yujeong Bae , Kai Yang , Philip Willke , Taeyoung Choi , Andreas J. Heinrich , Christopher P. Lutz

Spectroscopic measurements with low-temperature scanning tunneling microscopes have been used very successfully for studying not only individual atomic or molecular spins on surfaces but also complexly designed coupled systems. The symmetry…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 Markus Ternes

The works on decoherence due to spin baths usually agree in studying a one-spin system in interaction with a large spin bath. In this paper we generalize those models by analyzing a many-spin system and by studying decoherence or its…

Quantum Physics · Physics 2010-01-21 Mario Castagnino , Sebastian Fortin , Olimpia Lombardi

We revisit the problem of decoherence of a qubit centrally coupled to an interacting spin environment, here modeled by a quantum compass chain or an extended XY model in a staggered magnetic field. These two models both support distinct…

Statistical Mechanics · Physics 2017-12-22 R. Jafari , Henrik Johannesson

Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…

Quantum Physics · Physics 2026-05-06 Timothy J. Krogmeier , James Bradley , Anthony W. Schlimgen , Kade Head-Marsden

The problem of tunneling control in systems "quantum dot - quantum well" (as well as "quantum dot - quantum dot" or quantum molecule) and "quantum dot - bulk contact" is studied as a quantum tunneling with dissipation process in the…

We consider electrical transport through molecules with Heisenberg-coupled spins arranged in a ring structure in the presence of an easy-axis anisotropy. The molecules are coupled to two metallic leads and a gate. In the charged state of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Daniel Loss

Molecular spin clusters are mesoscopic systems whose structural and physical features can be tailored at the synthetic level. Besides, their quantum behavior is directly accessible in laboratory and their magnetic properties can be…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 F. Troiani , V. Bellini , A. Candini , G. Lorusso , M. Affronte

In semiconductors, the T2* coherence time of a single confined spin is limited either by the fluctuating magnetic environment (via the hyperfine interaction), or by charge fluctuations (via the spin-orbit interaction). We demonstrate that…

Mesoscale and Nanoscale Physics · Physics 2012-04-13 K. M. Weiss , J. M. Elzerman , Y. L. Delley , J. Miguel-Sanchez , A. Imamoglu

An ensemble of multilevel atoms is a good candidate for a quantum information storage device. The information is encrypted in the collective ground state atomic coherence, which, in the absence of external excitation, is decoupled from the…

Quantum Physics · Physics 2009-11-13 C. Genes , P. R. Berman

The inelastic portion of the tunnel current through an individual magnetic atom grants unique access to read out and change the atom's spin state, but it also provides a path for spontaneous relaxation and decoherence. Controlled closure of…

Mesoscale and Nanoscale Physics · Physics 2016-01-05 B. Bryant , R. Toskovic , A. Ferrón , J. L. Lado , A. Spinelli , J. Fernández-Rossier , A. F. Otte

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Florian Elste , Carsten Timm

We consider theoretically transport in a spinfull one-channel interacting quantum wire placed in an external magnetic field. For the case of two point-like impurities embedded in the wire, under a small voltage bias the spin-polarized…

Strongly Correlated Electrons · Physics 2010-02-17 Zoran Ristivojevic , George I. Japaridze , Thomas Nattermann

Spin coherent state path integrals with discontinuous semiclassical paths are investigated with special reference to a realistic model for the magnetic degrees of freedom in the Fe8 molecular solid. It is shown that such paths are essential…

Condensed Matter · Physics 2009-11-07 Ersin Kececioglu , Anupam Garg