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In forced wetting, a rapidly moving surface drags with it a thin layer of trailing fluid as it is plunged into a second fluid bath. Using high-speed interferometry, we find characteristic structure in the thickness of this layer with…

Soft Condensed Matter · Physics 2019-01-16 Mengfei He , Sidney R. Nagel

We present a generalized theory for studying phase separation in blends of polymers containing dipoles on their backbone. The theory is used to construct co-existence curves and to study the effects of dipolar interactions on interfacial…

Soft Condensed Matter · Physics 2014-11-04 Rajeev Kumar , Bobby G. Sumpter , M. Muthukumar

The paper is devoted to the thermodynamics of normal surface electromagnetic fields within a nonuniform dispersive and absorptive system. This system is formed by vacuum and lossy medium separated by a plane interface. As a medium, we used…

Other Condensed Matter · Physics 2012-12-04 Illarion Dorofeyev

Motivated by renewed interest in the physics of branched polymers, we present here a complete characterization of the connectivity and spatial properties of $2$ and $3$-dimensional single-chain conformations of randomly branching polymers…

Soft Condensed Matter · Physics 2020-03-23 Irene Adroher-Benítez , Angelo Rosa

We present new method for studying the equilibrium properties of interacting fluids in an arbitrary external filed. The method is valid in any dimension and it yields an exact results in one dimension. Using this approach, we derive a…

Soft Condensed Matter · Physics 2017-02-17 Benaoumeur Bakhti

We present an application of Flory-type self-consistent field theory of the flexible polymer chain dissolved in the binary mixture of solvents to theoretical description of co-nonsolvency. We show that our theoretical predictions are in…

Soft Condensed Matter · Physics 2017-11-10 Yu. A. Budkov , A. L. Kolesnikov

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer

Constitutive equations are derived for the viscoelastic response of rubbery polymers at finite strains. A polymer is thought of as a network of long chains connected to temporary junctions. At a random time, a chain detaches from a…

Soft Condensed Matter · Physics 2007-05-23 Aleksey D. Drozdov , Al Dorfmann

A fluid constituted of hard spherocylinders is studied using a density functional theory for non-spherical hard particles, which can be written as a function of weighted densities. This is based on an extended deconvolution of the Mayer…

Soft Condensed Matter · Physics 2015-06-18 René Wittmann , Klaus Mecke

The results obtained from molecular dynamics simulations of the friction at an interface between polymer melts and weakly attractive crystalline surfaces are reported. We consider a coarse-grained bead-spring model of linear chains with…

Soft Condensed Matter · Physics 2012-06-12 Nikolai V. Priezjev

We introduce a density functional formalism to study the ground-state properties of strongly-correlated dipolar and ionic ultracold bosonic and fermionic gases, based on the self-consistent combination of the weak and the strong coupling…

In this work, we consider a semi-dilute solution of identical star-polymers, made of attached flexible long polymer chains of the same polymerization degree N. We first compute the effective pair-potential between star-polymers. Such a…

Soft Condensed Matter · Physics 2007-05-23 F. Benzouine , M. Yassine , A. Derouiche , A. Bettachy , M. Benhamou

Using small-angle neutron scattering and liquid integral equation theory, we relate the structure factor of flexible dendrimers of 4th generation to their average shape. The shape is measured as a radial density profile of monomers…

Soft Condensed Matter · Physics 2009-10-31 C. N. Likos , M. Schmidt , H. Loewen , M. Ballauff , D. Poetschke , P. Lindner

The Flory Huggins equation of state for monodisperse polymers can be turned into a density functional by adding a square gradient term, with a coefficient fixed by appeal to RPA (random phase approximation). We present instead a model…

Soft Condensed Matter · Physics 2009-11-07 I. Pagonabarraga , M. E. Cates

Density-functional theory is utilized to investigate the zero-temperature transition from a Fermi liquid to an inhomogeneous stripe, or Wigner crystal phase, predicted to occur in a one-component, spin-polarized, two-dimensional dipolar…

Quantum Gases · Physics 2015-08-14 B. P. van Zyl , W. Kirkby , W. Ferguson

A fundamental theory is presented for the mechanical response of polymer networks undergoing large deformation which seamlessly integrates statistical mechanical principles with macroscopic thermodynamic constitutive theory. Our formulation…

Soft Condensed Matter · Physics 2020-07-06 Michael R. Buche , Meredith N. Silberstein

We consider the three-dimensional Ising model slightly below its critical temperature, with boundary conditions leading to the presence of an interface. We show how the interfacial properties can be deduced starting from the particle modes…

Statistical Mechanics · Physics 2020-08-17 Gesualdo Delfino , Walter Selke , Alessio Squarcini

We extend classical Flory-Rehner theory for the expansion and compression of porous materials such as cross-linked polymer networks. The theory includes volume exclusion, affinity with the solvent, and finite stretching of the polymer…

Chemical Physics · Physics 2023-09-28 P. M. Biesheuvel , H. Fan , M. Elimelech

This work introduces a methodology for the statistical mechanical analysis of polymeric chains under tension controlled by optical or magnetic tweezers at thermal equilibrium with an embedding fluid medium. The response of single bonds…

Soft Condensed Matter · Physics 2020-02-26 Aaron C. Meyer , Yahya Öz , Norman Gundlach , Michael Karbach , Ping Lu , Gerhard Müller

Dynamical properties of homogeneous Fermi-Fermi mixtures of dipolar and non-dipolar atoms are studied at zero temperature, where dipoles are polarized by an external field. We calculate the density-density correlation functions in a…

Quantum Gases · Physics 2024-04-24 Takahiko Miyakawa , Eiji Nakano , Hiroyuki Yabu