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We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb$_{2}$Mo$_{2}$O$_{7}$, $T$$_{g}$$\simeq$24 K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass…

Strongly Correlated Electrons · Physics 2013-09-17 D. K. Singh , Y. S. Lee

We report results of NMR experiments on the ruthenium oxide Hg2Ru2O7 with the pyrochlore structure, which exhibits a metal-insulator transition at TMI = 107 K. In the metallic phase above TMI, the nuclear spin-lattice relaxation rate 1/T1…

Strongly Correlated Electrons · Physics 2017-12-01 Makoto Yoshida , Masashi Takigawa , Ayako Yamamoto , Hidenori Takagi

We derive a simple system of equations to describe the magnetization relaxation of a molecular spin in weak interaction with a thermal bath for the whole temperature domain. Using this for the intermediate temperature domain where the…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

We propose a phenomenological spin fluctuation theory for antiferromagnetic quantum tricritical point (QTCP), where the first-order phase transition changes into the continuous one at zero temperature. Under magnetic fields, ferromagnetic…

Strongly Correlated Electrons · Physics 2010-10-20 Takahiro Misawa , Youhei Yamaji , Masatoshi Imada

We present the results of muon-spin relaxation (muSR) measurements on the hexagonal manganite HoMnO3. Features in the temperature-dependent relaxation rate, lambda, correlate with the magnetic transitions at 76 K, 38 K and 34 K. The highest…

Strongly Correlated Electrons · Physics 2015-05-14 H. J. Lewtas , T. Lancaster , P. J. Baker , S. J. Blundell , D. Prabhakaran , F. L. Pratt

We report on Ferromagnetic-Resonance experiments in a single crystal of La_0.8Sr_0.2MnO_3 in the temperature range from 4 to 300 K. The observed anisotropy of the resonance line changes on crossing the transition from the orthorhombic…

Strongly Correlated Electrons · Physics 2007-05-23 J. Deisenhofer , H. -A. Krug von Nidda , A. Loidl , M. V. Eremin , V. A. Ivanshin , T. Kimura , Y. Tokura

The Gd2Sn2O7 pyrochlore Heisenberg antiferromagnet displays a phase transition to a four sublattice Neel ordered state at a temperature near 1 K. Despite the seemingly conventional nature of the ordered state, the specific heat has been…

Materials Science · Physics 2007-08-16 Adrian Del Maestro , Michel J. P. Gingras

We present magnetization and Hall effect measurements on the pyrochlore iridate Nd2Ir2O7. Previous muon spin rotation measurements have shown that the system undergoes an unusual transition at T$_M$ = 110 K into a magnetic phase lacking…

Strongly Correlated Electrons · Physics 2015-06-12 S. M. Disseler , S. R. Giblin , Chetan Dhital , K. C. Lukas , Stephen D. Wilson , M. J. Graf

Owing to their high magnon frequencies, antiferromagnets are key materials for future high-speed spintronics. Picosecond switching of antiferromagnetic order has been viewed a milestone for decades and pursued only by using ultrafast…

We study the finite temperature properties of the candidate quantum spin ice material Yb$_2$Ti$_2$O$_7$ within the framework of an anisotropic nearest-neighbor spin $1/2$ model on the pyrochlore lattice. Using a combination of finite…

Strongly Correlated Electrons · Physics 2018-05-21 Hitesh J. Changlani

In the quest to realize a quantum spin liquid (QSL), magnetic long-range order is hardly welcome. Yet it can offer deep insights into a complex world of strong correlations and fluctuations. Much hope was placed in the cubic pyrochlore…

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

Strongly Correlated Electrons · Physics 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

We investigate the properties of the XY pyrochlore antiferromagnet with local <111> planar anisotropy. We find the ground states and show that the configurational ground state entropy is subextensive. By computing the free energy due to…

Statistical Mechanics · Physics 2014-04-11 Pawel Stasiak , Paul A. McClarty , Michel J. P. Gingras

We report $^{51}$V nuclear magnetic resonance (NMR) studies on single crystals of the multiferroic material FeVO$_4$. The high-temperature Knight shift shows Curie-Weiss behavior, $^{51}K = a/(T + \theta)$, with a large Weiss constant…

Strongly Correlated Electrons · Physics 2014-05-16 J. Zhang , L. Ma , J. Dai , Y. P. Zhang , Z. Z. He , B. Normand , Weiqiang Yu

By measurements of specific heat, we have investigated the magnetic field ($H$) induced spin-structural change in Nd$_2$Mo$_2$O$_7$ that shows spin-chirality-related magneto-transport phenomena. A broad peak around 2 K caused by the…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Onose , Y. Taguchi , T. Ito , Y. Tokura

We use numerical linked cluster (NLC) expansions to compute the specific heat, C(T), and entropy, S(T), of a quantum spin ice model of Yb2Ti2O7 using anisotropic exchange interactions recently determined from inelastic neutron scattering…

Strongly Correlated Electrons · Physics 2012-10-11 R. Applegate , N. R. Hayre , R. R. P. Singh , T. Lin , A. G. R. Day , M. J. P. Gingras

Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…

Statistical Mechanics · Physics 2016-01-19 P. Henelius , T. Lin , M. Enjalran , Z. Hao , J. G. Rau , J. Altosaar , F. Flicker , T. Yavors'kii , M. J. P. Gingras

Experimental investigation of the resistivity $\rho$, susceptibility $\chi$, specific heat C$_p$, and Hall coefficient R$_H$ of the pyrochlore Cd$_2$Re$_2$O$_7$ reveals the presence of a continuous phase transition of uncertain origin with…

Strongly Correlated Electrons · Physics 2016-08-31 R. Jin , J. He , J. R. Thompson , M. F. Chisholm , B. C. Sales , D. Mandrus

Iron (II) complexes with substituted tris(pyrazolyl) ligands, which exhibit a thermally driven transition from a low-spin state at low temperatures to a high-spin state at elevated temperatures, have been studied by M\"ossbauer spectroscopy…

We report $^{75}$As nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) studies on the superconductor Rb$_{2}$Cr$_{3}$As$_{3}$ with a quasi one-dimensional crystal structure. Below $T\sim$ 100 K, the spin-lattice…

Superconductivity · Physics 2015-10-07 J. Yang , Z. T. Tang , G. H. Cao , Guo-qing Zheng