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Superconductivity, magnetic order, and quadrupolar order have been investigated in the filled skutterudite system Pr$_{1-x}$Nd$_{x}$Os$_4$Sb$_{12}$ as a function of composition $x$ in magnetic fields up to 9 tesla and at temperatures…

Strongly Correlated Electrons · Physics 2015-05-19 P. -C. Ho , T. Yanagisawa , W. M. Yuhasz , A. A. Dooraghi , C. C. Robinson , N. P. Butch , R. E. Baumbach , M. B. Maple

Only few selected examples among the great diversity of anomalous rare earth skutterudite are reviewed. Focus is first given on PrFe4P12 in comparison with URu2Si2. For PrFe4P12, great progress has been made on determining the nature of the…

Strongly Correlated Electrons · Physics 2015-05-13 E. Hassinger , J. Derr , J. Levallois , D. Aoki , K. Behnia , F. Bourdarot , G. Knebel , C. Proust , J. Flouquet

Magnetization, specific heat, and electrical resistivity measurements were made on single crystals of the filled skutterudite compound PrOs$_{4}$As$_{12}$. Specific heat measurements indicate an electronic specific heat coefficient $\gamma$…

We report measurements of low-temperature specific heat on the 4f^2-based heavy-fermion superconductor PrOs4Sb12. In magnetic fields above 4.5 T in the normal state, distinct anomalies are found which demonstrate the existence of a…

Strongly Correlated Electrons · Physics 2009-11-07 Y. Aoki , T. Namiki , S. Ohsaki , S. R. Saha , H. Sugawara , H. Sato

Specific heat and transport measurements have revealed an unconventional heavy-fermion (HF) state in SmOs4Sb12 single crystals. The electronic specific-heat coefficient (gamma=0.82 J/K^2mol) and the coefficient (A) of the quadratic…

Strongly Correlated Electrons · Physics 2009-11-10 Shotaro Sanada , Yuji Aoki , Hidekazu Aoki , Akihisa Tsuchiya , Daisuke Kikuchi , Hitoshi Sugawara , Hideyuki Sato

Rare 4f^2-based heavy-fermion behaviors have been revealed recently in Pr-based filled skutterudites PrFe4P12 and PrOs4Sb12. Recent studies on the thermal properties on both compounds are reported, putting emphasis on the field-induced…

Strongly Correlated Electrons · Physics 2007-05-23 Y. Aoki , T. Namiki , T. Kanayama , S. Ohsaki , S. R. Saha , H. Sugawara , H. Sato

The filled skutterudite compound PrOs4Sb12, the first example of a Pr-based heavy fermion superconductor, displays superconductivity with $T_c\sim 1.85$ K and has an effective mass $m^* \sim$ {50 $m_e$}, where $m_e$ is the free electron…

Strongly Correlated Electrons · Physics 2007-05-23 P. -C. Ho , N. A. Frederick , V. S. Zapf , E. D. Bauer , T. D. Do , M. B. Maple , A. D. Christianson , A. H. Lacerda

The filled skutterudite compound \PrOsSb{} exhibits superconductivity below a critical temperature $T_\mathrm{c} = 1.85$ K that develops out of a nonmagnetic heavy Fermi liquid with an effective mass $m^{*} \approx 50 m_\mathrm{e}$, where…

Superconductivity · Physics 2007-05-23 M. B. Maple , P. -C. Ho , N. A. Frederick , V. S. Zapf , W. M. Yuhasz , E. D. Bauer

In the unconventional f-electron-associated charge order phase of filled skutterudite PrRu4P12, the low-temperature behaviors of the triplet crystalline-electric-field ground state of Pr ions have been studied by specific heat and…

The filled skutterudite compound \PrOsSb{} has been found to exhibit superconductivity with a critical temperature $T_\mathrm{c} = 1.85$ K that develops out of a heavy Fermi liquid with an effective mass $m^{*} \approx 50 m_\mathrm{e}$. The…

Superconductivity · Physics 2016-08-31 M. B. Maple , P. -C. Ho , V. S. Zapf , W. M. Yuhasz , N. A. Frederick , E. D. Bauer

Superconductivity is observed in the filled skutterudite compound \PrOsSb{} below a critical temperature temperature $T_\mathrm{c} = 1.85$ K and appears to develop out of a nonmagnetic heavy Fermi liquid with an effective mass $m^{*}…

Comprehensive magnetic-field-orientation dependent studies of the susceptibility and de Haas-van Alphen effect have been carried out on single crystals of the filled skutterudites PrOs$_4$As$_{12}$ and LaOs$_4$As$_{12}$ using magnetic…

Strongly Correlated Electrons · Physics 2009-11-13 Pei-Chun Ho , J. Singleton , M. B. Maple , Hisatomo Harima , P. A. Goddard , Z. Henkie , A. Pietraszko

We report $^{123}$Sb nuclear quadrupole resonance (NQR) measurements of the filled skutterudite heavy-fermion superconductor PrOs$_4$Sb$_{12}$ under high pressure. The temperature dependence of NQR frequency and the spin-lattice relaxation…

Superconductivity · Physics 2009-11-13 S. Kawasaki , K. Katayama , H. Sugawara , D. Kikuchi , H. Sato , G. -q. Zheng

Single crystals of the filled-skutterudite compound NdOs$_4$Sb$_{12}$ have been investigated by means of electrical resistivity, magnetization, and specific heat measurements. The NdOs$_4$Sb$_{12}$ crystals have the LaFe$_4$P$_{12}$-type…

Strongly Correlated Electrons · Physics 2009-11-10 P. -C. Ho , W. M. Yuhasz , N. P. Butch , N. A. Frederick , T. A. Sayles , J. R. Jeffries , M. B. Maple , J. B. Betts , A. H. Lacerda , P. Rogl , G. Giester

We report the de Haas-van Alphen (dHvA) experiment on the filled skutterudite PrFe$_4$P$_{12}$ exhibiting apparent Kondo-like behaviors in the transport and thermal properties. We have found enormously enhanced cyclotron effective mass…

Strongly Correlated Electrons · Physics 2009-10-31 H. Sugawara , T. D. Matsuda , K. Abe , Y. Aoki , H. Sato , S. Nojiri , Y. Inada , R. Settai , Y. Ōnuki

The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…

Strongly Correlated Electrons · Physics 2009-11-11 Annamaria Kiss , Yoshio Kuramoto

Current status is described toward identifying unconventional order parameters in filled skutterudites with unique ordering phenomena. The order parameters in PrFe$_4$P$_{12}$ and PrRu$_4$P$_{12}$ are discussed in relation to associated…

Strongly Correlated Electrons · Physics 2015-05-13 Yoshio Kuramoto , Annamaria Kiss

Thermal conductivity measurements were performed on single crystal samples of the superconducting filled skutterudite compounds PrOs$_4$Sb$_{12}$ and PrRu$_4$Sb$_{12}$ both as a function of temperature and magnetic field applied…

Superconductivity · Physics 2007-09-28 R. W. Hill , Shiyan Li , M. B. Maple , Louis Taillefer

We report on systematic study of superconducting characteristics and Pr crystalline-electric-field (CEF) levels of filled-skutterudite \pra ($T_{\rm c}$ = 2.33 K). The temperature dependences of the upper critical field $H_{\rm c2}$ and the…

Strongly Correlated Electrons · Physics 2007-10-03 T. Namiki , Y. Aoki , H. Sato , C. Sekine , I. Shirotani , T. D. Matsuda , Y. Haga , T. Yagi

Pr 4f electronic states in Pr-based filled skutterudites PrT4X12(T=Fe and Ru; X=P and Sb) have been studied by high-resolution bulk-sensitive Pr 3d-4f resonance photoemission. A very strong spectral intensity is observed just below the…

Strongly Correlated Electrons · Physics 2023-06-02 A. Yamasaki , S. Imada , T. Nanba , A. Sekiyama , H. Sugawara , H. Sato , C. Sekine , I. Shirotani , H. Harima , S. Suga
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