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The interaction between electronic and nuclear spins in the presence of external magnetic fields can be described by a spin Hamiltonian, with parameters obtained from first principles, electronic structure calculations. We describe an…

Materials Science · Physics 2019-04-10 Krishnendu Ghosh , He Ma , Vikram Gavini , Giulia Galli

First principles constrained density functional theory scheme in Wannier functions formalism has been used to calculate Coulomb repulsion U and Hund's exchange J parameters for iron 3d electrons in LaFeAsO. Results strongly depend on the…

Strongly Correlated Electrons · Physics 2009-01-31 V. I. Anisimov , Dm. M. Korotin , S. V. Streltsov , A. V. Kozhevnikov , J. Kuneš , A. O. Shorikov , M. A. Korotin

The Electron Localization Function (ELF) -- as proposed originally by Becke and Edgecombe -- has been widely adopted as a descriptor of atomic shells and covalent bonds. The ELF takes into account the antisymmetry of Fermions but it…

Materials Science · Physics 2015-09-15 Stefano Pittalis , Alain Delgado , Carlo Andrea Rozzi

We present electric dipole polarizabilities ($\alpha_d$) of the alkali-metal negative ions, from H$^-$ to Fr$^-$, by employing four-component relativistic many-body methods. Differences in the results are shown by considering Dirac-Coulomb…

Atomic Physics · Physics 2021-01-07 B. K. Sahoo

New insights into the microscopic origin of itinerant ferromagnetism were recently gained from investigations of electronic lattice models within dynamical mean-field theory (DMFT). In particular, it is now established that even in the…

Strongly Correlated Electrons · Physics 2007-05-23 D. Vollhardt , N. Blümer , K. Held , M. Kollar

We calculate magnetic anisotropy energy of Fe and Ni by taking into account the effects of strong electronic correlations, spin-orbit coupling, and non-collinearity of intra--atomic magnetization. The LDA+U method is used and its…

Strongly Correlated Electrons · Physics 2007-05-23 Imseok Yang , Sergej Y. Savrasov , Gabriel Kotliar

Magnetic properties of Fe, Co, and Ni at finite temperatures have been investigated on the basis of the first-principles dynamical CPA (Coherent Potential Approximation) combined with the LDA (Local Density Approximation) + $U$ Hamiltonian…

Strongly Correlated Electrons · Physics 2015-05-27 Yoshiro Kakehashi , M. Atiqur R. Patoary

The heavy fermion (HF) state of $d$-electron systems is of great current interest since it exhibits various exotic phases and phenomena that are reminiscent of the Kondo effect in $f$-electron HF systems. Here, we present a combined…

Strongly Correlated Electrons · Physics 2025-03-03 Bing Xu , Rui Liu , Hongliang Wo , Zhiyu Liao , Shaohui Yi , Chunhong Li , Jun Zhao , Xianggang Qiu , Zhiping Yin , Christian Bernhard

Effects of electron correlation in FeSi are studied in terms of the two-band Hubbard model with the density of states obtained from the band calculation. Using the self-consistent second-order perturbation theory combined with the local…

Strongly Correlated Electrons · Physics 2009-10-31 Kentaro Urasaki , Tetsuro Saso

Atomic properties such as field shift constants, magnetic dipole and electric quadrupole hyperfine structure constants, Land\'e $g_J$ factors, and electric quadrupole moments that are described by electronic operators with different ranks…

Atomic Physics · Physics 2018-03-14 Pradeep Kumar , Cheng-Bin Li , B. K. Sahoo

Effects of Coulomb correlation on LaOFeAs electronic structure have been investigated by LDA+DMFT(QMC) method. The calculation results show that LaOFeAs is in the regime of intermediate correlation strength with significant part of the…

Strongly Correlated Electrons · Physics 2009-11-13 A. O. Shorikov , M. A. Korotin , S. V. Streltsov , S. L. Skornyakov , D. M. Korotin , V. I. Anisimov

We study the low-temperature behavior of a magnetic impurity which is weakly coupled to correlated conduction electrons. To account for conduction electron interactions a diagrammatic approach in the frame of the 1/N expansion is developed.…

Strongly Correlated Electrons · Physics 2009-11-07 M. Neef , S. Tornow , V. Zevin , G. Zwicknagl

The electronic structure and magnetic properties of a single Fe adatom on a CuN surface have been studied using density functional theory in the local spin density approximation (LSDA), the LSDA+U approach and the local density…

Strongly Correlated Electrons · Physics 2016-04-20 S. K. Panda , I. Di Marco , O. Grånäs , O. Eriksson , J. Fransson

Electronic correlations were long suggested not only to be responsible for the complexity of many novel materials, but also to form essential prerequisites for their intriguing properties. Electronic behavior of iron-based superconductors…

The correlated electronic structure of iron, cobalt and nickel is investigated within the dynamical mean-field theory formalism, using the newly developed full-potential LMTO-based LDA+DMFT code. Detailed analysis of the calculated electron…

Strongly Correlated Electrons · Physics 2009-03-16 Alexei Grechnev , Igor Di Marco , M. I. Katsnelson , A. I. Lichtenstein , John Wills , Olle Eriksson

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

We study the influence of short range antiferromagnetic correlations between local $f$-electrons on the transport and thermodynamic properties of Kondo insulators, as first proposed by Coqblin et al. for metallic heavy fermions. The…

Strongly Correlated Electrons · Physics 2009-10-31 Tatiana G. Rappoport , M. S. Figueira , M. A. Continentino

The influence of dynamical correlation effects on the magneto-optical properties of ferromagnetic Fe and Ni has been investigated. In addition the temperature dependence of the self-energy and its influence on the DOS and optical…

Strongly Correlated Electrons · Physics 2009-11-10 A. Perlov , S. Chadov , H. Ebert , L. Chioncel , A. I. Lichtenstein , M. I. Katsnelson

Understanding the effects of electron-electron interactions in half metallic magnets (HMs), which have band structures with one gapped spin channel and one metallic channel, poses fundamental theoretical issues as well as having importance…

Strongly Correlated Electrons · Physics 2013-04-10 M. Jiang , W. E. Pickett , R. T. Scalettar

The mechanism of f-electron delocalization is investigated within the multi-orbital Anderson lattice model by means of diagrammatic perturbation theory from the atomic limit. The derived equations couple the intra-atomic transition…

Strongly Correlated Electrons · Physics 2009-11-07 U. Lundin , I. Sandalov , O. Eriksson , B. Johansson