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We simulate the compression of a two-component Lennard-Jones liquid at a variety of constant temperatures using a molecular dynamics algorithm in an isobaric-isothermal ensemble. The viscosity of the liquid increases with pressure,…

chem-ph · Physics 2009-10-22 Shelly L. Shumway , Andrew S. Clarke , Hannes Jónsson

Molecular dynamics simulations of a Lennard-Jones binary mixture confined in a disordered array of soft spheres are presented. The single particle dynamical behavior of the glass former is examined upon supercooling. Predictions of mode…

Statistical Mechanics · Physics 2009-11-07 P. Gallo , R. Pellarin , M. Rovere

We explain the findings by Di Leonardo et al. [Phys. Rev. Lett. 84, 6054 (2000)] that the effective temperature of a Lennard-Jones glass depends only on the final value of the density in the volume and/or temperature jump that produces the…

Statistical Mechanics · Physics 2013-05-14 Nicoletta Gnan , Claudio Maggi , Thomas B. Schroeder , Jeppe C. Dyre

We investigate a binary Lennard-Jones mixture with molecular dynamics simulations. We consider first a system cooled linearly in time with the cooling rate gamma. By varying gamma over almost four decades we study the influence of the…

Statistical Mechanics · Physics 2015-06-25 K. Vollmayr-Lee , W. Kob , K. Binder , A. Zippelius

We report results of molecular dynamics simulations of a binary Lennard-Jones system at zero pressure in the undercooled liquid and glassy states. We first follow the evolution of diffusivity and dynamic heterogeneity with temperature and…

Disordered Systems and Neural Networks · Physics 2007-05-23 H. R. Schober

The dynamics of Lennard-Jones fluid is studied through extended mode coupling theory (MCT) with the inclusion of the slow mode of defect density. Inclusion of defect density facilitates the liquid like state for temperatures much lower than…

Statistical Mechanics · Physics 2009-11-07 Sudha Srivastava , Shankar P. Das

We investigate the calorimetric liquid-glass transition by performing simulations of a binary Lennard-Jones mixture in one through four dimensions. Starting at a high temperature, the systems are cooled to T=0 and heated back to the ergodic…

Disordered Systems and Neural Networks · Physics 2009-01-01 Ralf Brüning , Denis A. St-Onge , Steve Patterson , Walter Kob

We study the pressure dependence of the melting mechanism of a surface free Lennard-Jones crystal by constant pressure Monte Carlo simulation. The difference between the overheating temperature($T_{OH}$) and the thermodynamical melting…

Materials Science · Physics 2009-11-11 L. Gómez , C. Gazza , H. Dacharry , L. Peñaranda , A. Dobry

We study shear yielding and steady state flow of glassy materials with molecular dynamics simulations of two standard models: amorphous polymers and bidisperse Lennard-Jones glasses. For a fixed strain rate, the maximum shear yield stress…

Soft Condensed Matter · Physics 2009-11-10 Joerg Rottler , Mark O. Robbins

Properties of local minima as a function of density are studied in a binary Lennard-Jones system for kinetic equipartition temperatures $T=1.0$ (normal liquid), 0.5 (supercooled liquid), and 0.4 (glass), in reduced units. The number of…

Disordered Systems and Neural Networks · Physics 2009-11-07 Javier Hernandez-Rojas , David J. Wales

We investigate the jump motion among potential energy minima of a Lennard-Jones model glass former by extensive computer simulation. From the time series of minima energies, it becomes clear that the energy landscape is organized in…

Soft Condensed Matter · Physics 2009-11-07 B. Doliwa , A. Heuer

The stress-strain relations and the yield behavior of model glass (a 80:20 binary Lennard-Jones mixture) is studied by means of MD simulations. First, a thorough analysis of the static yield stress is presented via simulations under imposed…

Soft Condensed Matter · Physics 2009-11-10 F. Varnik , L. Bocquet , J. -L. Barrat

We theoretically investigate structural relaxation and activated diffusion of glass-forming liquids at different pressures using both the Elastically Collective Nonlinear Langevin Equation (ECNLE) theory and molecular dynamics (MD)…

Soft Condensed Matter · Physics 2020-09-23 Anh D. Phan , Kajetan Koperwas , Marian Paluch , Katsunori Wakabayashi

Using molecular dynamics computer simulations we investigate the dependence of bulk properties of a Lennard-Jones glass on the cooling rate with which the glass was produced. By studying the clusters formed by the nearest neighbor shells of…

Condensed Matter · Physics 2009-10-28 K. Vollmayr , W. Kob , K. Binder

Using a molecular dynamics computer simulation we determine the temperature dependence of the partial structure factors for a binary Lennard-Jones system. These structure factors are used as input data to solve numerically the wave-vector…

Condensed Matter · Physics 2016-08-31 Markus Nauroth , Walter Kob

Using molecular dynamics computer simulations we investigate how the glass transition and the properties of the resulting glass depend on the cooling rate with which the sample has been quenched. This is done by studying a two component…

Condensed Matter · Physics 2009-10-28 Katharina Vollmayr , Walter Kob , Kurt Binder

We use molecular dynamics computer simulations to investigate the relaxation dynamics of a binary Lennard-Jones liquid confined in a narrow pore. We find that the average dynamics is strongly influenced by the confinement in that time…

Statistical Mechanics · Physics 2009-10-31 Peter Scheidler , Walter Kob , Kurt Binder

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

Statistical Mechanics · Physics 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

We present a calculation of a fourth-order, time-dependent density correlation function that measures higher-order spatiotemporall correlations of the density of a liquid. From molecular dynamics simulations of a glass-forming Lennard-Jones…

Statistical Mechanics · Physics 2009-11-07 N. Lacevic , F. W. Starr , T. B. Schroder , V. N. Novikov , S. C. Glotzer

We present results of theoretical description and numerical calculation of the dynamics of molecular liquids based on the Reference Interaction Site Model / Mode-Coupling Theory. They include the temperature-pressure(density) dependence of…

Chemical Physics · Physics 2007-05-23 A. E. Kobryn , T. Yamaguchi , F. Hirata
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