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Analytical expressions for the binding energy of electrons and positrons in dielectric clusters, analysed in this work, neglect the elastic effects. Therefore, we present the density-functional theory for neutral liquid clusters that…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Valentin V. Pogosov , Walter V. Pogosov , Denis P. Kotlyarov

Both spontaneous emission and resonant energy transfer can be enhanced significantly when the emitter is placed in the vicinity of metallic or crystal structures. This enhancement can be described using the electromagnetic Green tensor and…

Optics · Physics 2022-07-27 Asaf Farhi , Aristide Dogariu

We present theoretical description of conduction electrons interacting with a domain wall in ferromagnetic metals. The description takes into account interaction between electrons. Within the semiclassical approximation we calculate the…

Materials Science · Physics 2009-11-07 V. K. Dugaev , J. Barnas , A. Lusakowski , L. A. Turski

We present a novel method to extract the various contributions to the photonic local density of states from near-field fluorescence maps. The approach is based on the simultaneous mapping of the fluorescence intensity and decay rate, and on…

In this thesis we present a new formalism to study linear and non-linear response in extended systems. Our approach is based on real-time solution of an effective Schr\"odinger equation. The coupling between electrons and external field is…

Materials Science · Physics 2017-04-24 Claudio Attaccalite

We apply the time-dependent local density approximation (TDLDA) to calculate dipole excitations in small carbon clusters. A strong low-frequency mode is found which agrees well with observation for clusters C_n with n in the range 7-15. The…

Chemical Physics · Physics 2009-10-30 K. Yabana , G. F. Bertsch

Quantitative predictions from synthetic radiation diagnostics often have to consider all accelerated particles. For particle-in-cell (PIC) codes, this not only means including all macro-particles but also taking into account the discrete…

Computational Physics · Physics 2018-02-13 Richard Pausch , Alexander Debus , Axel Huebl , Ulrich Schramm , Klaus Steiniger , René Widera , Michael Bussmann

We calculate from first principles the electronic structure, relaxation and magnetic moments in small Fe particles, applying the numerical local orbitals method in combination with norm-conserving pseudopotentials. The accuracy of the…

Materials Science · Physics 2009-11-07 A. V. Postnikov , P. Entel , Jose M. Soler

We show here that the Hamiltonian for an electronic system may be written exactly in terms of fluctuation operators that transition constituent fragments between internally correlated states, accounting rigorously for inter-fragment…

Chemical Physics · Physics 2019-05-24 Anthony D. Dutoi , Yuhong Liu

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

Atomic and Molecular Clusters · Physics 2007-05-23 Prachi Pradhan , Asok K. Ray

We study the electromagnetic field scattered by a metallic nanoparticle with dispersive material parameters in a resonant regime. We consider the particle placed in a homogeneous medium in a low-frequency regime. We define modes for the…

Mathematical Physics · Physics 2021-02-11 Lorenzo Baldassari , Pierre Millien , Alice L. Vanel

Machine learning techniques can reveal hidden structure in large data amounts and can potentially extent or even replace analytical scientific methods. In nanophotonics, modes can increase the light yield from emitters located inside the…

Optics · Physics 2018-10-02 Carlo Barth , Christiane Becker

Electronic and optical properties of silver clusters were calculated using two different \textit{ab initio} approaches: 1) based on all-electron full-potential linearized-augmented plane-wave method and 2) local basis function…

Mesoscale and Nanoscale Physics · Physics 2016-11-28 John T. Titantah , Mikko Karttunen

In this paper we show that 1-electron properties such as Compton profiles and structure factors of crystals can be asymptotically retrieved through cluster-based calculations, followed by an appropriate partition of the 1-electron reduced…

Chemical Physics · Physics 2015-06-26 Sebastien Ragot , Jean-Michel Gillet , Pierre J Becker

Large scale Density Functional Theory (DFT) based electronic structure calculations are highly time consuming and scale poorly with system size. While semi-empirical approximations to DFT result in a reduction in computational time versus…

Materials Science · Physics 2016-12-21 Ganesh Hegde , R. Chris Bowen

Resonant modes determine the response of electromagnetic devices, including dielectric and plasmonic resonators. Relying on the degrees of freedom that metamaterials provide, this contribution shows how to design, at will, the resonant…

Another way to evaluate the spectral-correlation properties of thermal fields of solids is suggested. Such a method takes into account detailed structure of the interface transition layer separating one bulk region from those of the vacuum…

Quantum Physics · Physics 2015-06-15 Illarion Dorofeyev

The cumulant expansion is a powerful approach for including correlation effects in electronic structure calculations beyond the GW approximation. However, current implementations are incomplete since they ignore terms that lead to partial…

Strongly Correlated Electrons · Physics 2014-02-04 J. J. Kas , J. J. Rehr , L. Reining

Theoretically, the presence of a metallic nanoparticle enhances the intermolecular energy transfer. We calculate this enhancement factor with a modal approach pertaining analytical results in the case of a nanosphere. We calculate the…

Mesoscale and Nanoscale Physics · Physics 2019-07-02 Titus Sandu , Catalin Tibeica , Oana Nedelcu , Mihai Gologanu

Plasmonic resonance of a metallic nanostructure results from coherent motion of its conduction electrons driven by incident light. At the resonance, the induced dipole in the nanostructure is proportional to the number of the conduction…

Materials Science · Physics 2016-04-20 Mingliang Zhang , Hongping Xiang , Xu Zhang , Gang Lu