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Related papers: Spin-1/2 Kagome Like Lattice in Volborthite Cu3V2O…

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Volborthite compound is one of the very few realizations of S=1/2 quantum spins on a highly frustrated kagome-like lattice. Low-T SQUID measurements reveal a broad magnetic transition below 2K which is further confirmed by a peak in the 51V…

Strongly Correlated Electrons · Physics 2009-11-11 F. Bert , D. Bono , P. Mendels , F. Ladieu , F. Duc , J. -C Trombe , P. Millet

We determined the spin exchanges between the Cu2+ ions in the kagome layers of volborthite, Cu3V2O7(OH)2x2H2O, by performing the energy-mapping analysis based on DFT+U calculations, to find that the kagom\'e layers of Cu2+ ions are hardly…

Strongly Correlated Electrons · Physics 2022-03-02 Myung-Hwan Whangboa , Hyun-Joo Koo , Eva Brücher , Pascal Puphal , Reinhard K. Kremer

We report 51V-NMR study on a high-quality powder sample of volborthite Cu3V2O7(OH)2/2H2O, a spin-1/2 Heisenberg antiferromagnet on a distorted kagome lattice formed by isosceles triangles. In the magnetic fields below 4.5 T, a sharp peak in…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , M. Takigawa , H. Yoshida , Y. Okamoto , Z. Hiroi

Magnetic properties of the spin-1/2 kagome-like compound volborthite are studied using a high-quality polycrystalline sample. It is evidenced from magnetization and specific heat measurements that the spins on the kagome lattice still…

The Kagome-lattice-based material, Volborthite, $\mathrm{Cu_3 V_2 O_7 (OH)_2 \cdot 2 H_2 O}$, has been considered as a promising platform for discovery of unusual quantum ground states due to the frustrated nature of spin interactions. Here…

Strongly Correlated Electrons · Physics 2017-07-19 Li Ern Chern , Kyusung Hwang , Tomonari Mizoguchi , Yejin Huh , Yong Baek Kim

In Volborthite, spin-1/2 moments form a distorted Kagom\'e lattice, of corner sharing isosceles triangles with exchange constants $J$ on two bonds and $J'$ on the third bond. We study the properties of such spin systems, and show that…

Strongly Correlated Electrons · Physics 2007-09-29 Fa Wang , Ashvin Vishwanath , Yong Baek Kim

Thermodynamic investigations on volborthite (Cu3V2O7(OH)2 2H2O), which possesses a two-dimensional kagome structure of S-1/2 spins, are presented. The low-temperature heat capacities of volborthite and its Zn analogue compound were measured…

Strongly Correlated Electrons · Physics 2010-08-12 Satoshi Yamashita , Tomoya Moriura , Yasuhiro Nakazawa , Hiroyuki Yoshida , Yoshihiko Okamoto , Zenji Hiroi

A polycrystalline sample of vesignieite BaCu3V2O8(OH)2 comprising a nearly ideal kagome lattice composed of Cu2+ ions carrying spin 1/2 has been synthesized and studied by magnetization and heat capacity measurements. Magnetic…

Strongly Correlated Electrons · Physics 2009-11-13 Yoshihiko Okamoto , Hiroyuki Yoshida , Zenji Hiroi

We report the study of high quality samples of the frustrated S = 1/2 kagome antiferromagnet vesignieite, Cu3Ba(VO5H)2. Neutron powder diffraction measurements evidence the high quality of the kagome lattice and show no sign of a transition…

We report results of 51V NMR in the field-induced phase of volborthite Cu3V2O7(OH)dot2H2O, a spin-1/2 antiferromagnet on a distorted kagome lattice. In magnetic fields above 4.5 T, two types of V sites with different spin-echo decay rates…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , M. Takigawa , H. Yoshida , Y. Okamoto , Z. Hiroi

We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices---barlowite Cu$_{4}$(OH)$_{6}$FBr. Magnetic susceptibility gives $\theta_{CW}$ = $-$136 K, while long-range order does not happen…

Strongly Correlated Electrons · Physics 2014-12-05 Tian-Heng Han , John Singleton , John A. Schlueter

Two kagome compounds, volborthite Cu3V2O7(OH)2-2H2O and herbertsmithite ZnCu3(OH)6Cl2, are compared in order to derive information about the intrinsic properties of the spin-1/2 kagome antiferromagnet. Volborthite shows a broad maximum at T…

Strongly Correlated Electrons · Physics 2009-11-13 Z Hiroi , H Yoshida , Y Okamoto , M Takigawa

We study polycrystalline samples of KCu3As2O7(OH)3, a new candidate spin-1/2 kagome antiferromagnet, by magnetic susceptibility and heat capacity measurements above 2 K. The unique arrangement of the 3z2 - r2 and x2 - y2 orbitals on the…

Materials Science · Physics 2015-06-04 Yoshihiko Okamoto , Hajime Ishikawa , Gøran J. Nilsen , Zenji Hiroi

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

We report results of 51V NMR experiments on a high-quality powder sample of volborthite Cu3V2O7(OH)2/2H2O, a spin-1/2 Heisenberg antiferromagnet on a distorted kagome lattice. Following the previous experiments in magnetic fields $B$ below…

Kagome lattice decorated with S=1/2 spins is one of the most discussed ways to realize a quantum spin liquid. However, all previous material realizations of this model have suffered from additional complications, ranging from additional…

In the search for spin-1/2 kagome antiferromagnets, the mineral volborthite has recently been the subject of experimental studies [Hiroi et al.,2001]. It has been suggested that the magnetic properties of this material are described by a…

Strongly Correlated Electrons · Physics 2009-11-11 W. Apel , T. Yavors'kii , H. -U. Everts

We have synthesized high-quality single crystals of volborthite, a seemingly distorted kagome antiferromagnet, and carried out high-field magnetization measurements up to 74 T and 51V NMR measurements up to 30 T. An extremely wide 1/3…

Strongly Correlated Electrons · Physics 2015-06-03 H. Ishikawa , M. Yoshida , K. Nawa , M. Jeong , S. Krämer , M. Horvatić , C. Berthier , M. Takigawa , M. Akaki , A. Miyake , M. Tokunaga , K. Kindo , J. Yamaura , Y. Okamoto , Z. Hiroi

We report results of magnetic susceptibility and 51V- and 63,65Cu-NMR measurements on a high-quality powder sample of vesignieite BaCu3V2O8(OH)2, a candidate for the spin-1/2 kagome antiferromagnet. We observed a twostep magnetic…

Strongly Correlated Electrons · Physics 2017-12-01 Makoto Yoshida , Yoshihiko Okamoto , Masashi Takigawa , Zenji Hiroi

The recently discovered natural minerals Cu3Zn(OH)6Cl2 and Cu3Mg(OH)6Cl2 are spin 1/2 systems with an ideal kagome geometry. Based on electronic structure calculations, we develop a realistic model which includes couplings across the kagome…

Strongly Correlated Electrons · Physics 2008-09-05 O. Janson , J. Richter , H. Rosner
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