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We study morphologies of thin-film diblock copolymers between two flat and parallel walls. The study is restricted to the weak segregation regime below the order-disorder transition temperature. The deviation from perfect lamellar shape is…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , David Andelman

We study thin films of A/B diblock copolymer in a lamellar phase confined between two parallel plates (electrodes) that impose a constant voltage across the film. The weak-segregation limit is explored via a Ginzburg-Landau-like free-energy…

Soft Condensed Matter · Physics 2019-02-21 B. Zheng , X. -K. Man , Z. C. Ou-Yang , M. Schick , D. Andelman

We present several ordering mechanisms in diblock copolymers. For temperatures above the order-disorder temperature and in the weak segregation regime, a linear response theory is presented which gives the polymer density in the vicinity of…

Soft Condensed Matter · Physics 2007-05-23 Yoav Tsori , David Andelman

We investigate the phase behavior of symmetric AB diblock copolymers confined into a thin film. The film boundaries are parallel, impenetrable and attract the A component of the diblock copolymer. Using a self-consistent field technique…

Statistical Mechanics · Physics 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

The dynamics of microphase separation and the orientation of lamellae in diblock copolymers is investigated in terms of a mean-field model. The formation of lamellar structures and their stable states are explored and it is shown that…

Soft Condensed Matter · Physics 2015-06-15 Vanessa Weith , Alexei Krekhov , Walter Zimmermann

We investigate the effect of chemically patterned surfaces on the morphology of diblock copolymers below the order-disorder transition. Profiles for lamellar phases in contact with one surface, or confined between two surfaces are obtained…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , David Andelman

Mixtures of near-symmetric oppositely charged components with strong attractive short range interactions exhibit ordered lamellar phases at low temperatures. In the strong segregation limit the state of these systems can be described by the…

Soft Condensed Matter · Physics 2007-05-23 Francisco J. Solis , Galen T. Pickett

We consider the relative stability of parallel and perpendicular lamellar layers on corrugated surfaces. The model can be applied to smectic phases of liquid crystals, to lamellar phases of short-chain amphiphiles and to lamellar phases of…

Soft Condensed Matter · Physics 2009-11-10 Yoav Tsori , David Andelman

We present numerical calculations of lamellar phases of di-block copolymers (BCP) confined between two surfaces, where the top surface is flat and the bottom one is corrugated. The corrugated substrate is assumed to have a single $q$-mode…

Soft Condensed Matter · Physics 2016-02-17 Xingkun Man , Jiuzhou Tang , Pan Zhou , Dadong Yan , David Andelman

The structure of lamellar phases of symmetric $AB$ diblock copolymers in a thin film is investigated. We quantitatively compare the composition profiles and profiles of individual segments in self-consistent field calculations with Monte…

Statistical Mechanics · Physics 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

Thin films of diblock copolymer subject to gravitational field are simulated by means of a cell dynamical system model. The difference in density of the two sides of the molecule and the presence of the field causes the formation of…

Materials Science · Physics 2009-10-31 S. Martins , W. A. M. Morgado , M. S. O. Massunaga , M. Bahiana

The orientation of the lamellae formed by the phase separation of symmetric diblock copolymer thin films is strongly affected by the wetting properties of the polymer blocks with respect to the substrate. On bare silicon wafers the lamellae…

In the present work, we study morphologies arising due to competing substrate interaction, electric field and confinement effects on a symmetric diblock copolymer. We employ a coarse grained non-local Cahn-Hilliard phenomenological model…

Materials Science · Physics 2016-04-06 Arnab Mukherjee , Rajdip Mukherjee , Kumar Ankit , Avisor Bhattacharya , Britta Nestler

We consider orientational transitions of lamellar phases under the influence of a spatially nonuniform electric field. The transition between parallel and perpendicular lamellar stackings with respect to the substrate is investigated as a…

Materials Science · Physics 2009-11-11 Yoav Tsori

We present numerical calculations of lamellar phases of block copolymers at patterned surfaces. We model symmetric di-block copolymer films forming lamellar phases and the effect of geometrical and chemical surface patterning on the…

Soft Condensed Matter · Physics 2016-02-18 Xingkun Man , David Andelman , Henri Orland

Self-Consistent Field Theory is applied to a film of cylindrical-forming block copolymer subject to a surface field which tends to align the cylinders parallel to electrical plates, and to an external electric field tending to align them…

Soft Condensed Matter · Physics 2009-11-11 Chin-Yet Lin , M. Schick

We study the effect of monomer immobilization (quenching) on the orientation of the lamellae in symmetric diblock copolymer thin films with neutrally wetting surfaces. A small fraction of the monomers immediately next to the solid substrate…

Condensed Matter · Physics 2009-10-30 Wilfred H. Tang , Thomas A. Witten

In this paper we consider thin films of AB block copolymer melts confined between two parallel plates. The plates are identical and may have a preference for one of the monomer types over the other. The system is characterized by four…

Soft Condensed Matter · Physics 2009-11-11 Hindrik Jan Angerman , Albert Johner , Alexander N. Semenov

We present few ordering mechanisms in block copolymer melts in the coarse-graining approach. For chemically homogeneous or modulated confining surfaces, the surface ordering is investigated above and below the order-disorder temperature. In…

Soft Condensed Matter · Physics 2012-01-31 Yoav Tsori , David Andelman

A mesoscopic model of a diblock copolymer is used to study the stability of a uniform lamellar phase under a reciprocating shear flow. Approximate viscosity contrast between the microphases is allowed through a linear dependence of the…

Soft Condensed Matter · Physics 2009-11-07 Peilong Chen , Jorge Vinals
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