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Using the density-functional-theory based electronic structure calculations, we study the electronic state of recently discovered mixed-valent manganese oxides $A$Mg$_4$Mn$_6$O$_{15}$ ($A=$ K, Rb, Cs), which are fully spin-polarized…

Strongly Correlated Electrons · Physics 2018-04-18 T. Yamaguchi , K. Sugimoto , Y. Ohta , Y. Tanaka , H. Sato

Electron spin resonance and magnetization data in magnetic fields up to 55 T of a novel multicenter paramagnetic molecular complex [L_2Ni_4(N_3)(O_2C Ada)_4](Cl O_4) are reported. In this compound, four Ni centers each having a spin S = 1…

The ternary semiconductor AgInTe$_2$ is a thermoelectric material with chalcopyrite-type structure that transforms reversibly into a rocksalt-type structure under high pressure. Nuclear magnetic resonance (NMR) is considered to provide…

Materials Science · Physics 2024-10-01 Robin Guehne , Carsten Kattinger , Marko Bertmer , Simon Welzmiller , Oliver Oeckler , Jürgen Haase

We study Mn12O12(C6H5COO)16(H2O)4 (Mn12-Ph) single-molecule magnets on highly ordered pyrolytic graphite (HOPG) using low temperature scanning tunneling microscopy (LT-STM) experiments. We report Mn12-Ph in isolation, resembling single…

Mesoscale and Nanoscale Physics · Physics 2012-11-09 Kelley Reaves , Kyongwan Kim , Katsuya Iwaya , Taro Hitosugi , Hanhua Zhao , Kim R. Dunbar , Helmut G. Katzgraber , Winfried Teizer

Manganese nitrides should be with amazing properties and promised application, because manganese atom is particular for its magnetism, valence states, high electron density, etc., and N atoms in compounds form different substructures. It is…

Materials Science · Physics 2021-11-04 Li Li , Kuo Bao , Xingbin Zhao , Tian Cui

In this work, we examine low-energy adsorption configurations of four dodecanuclear manganese single-molecule magnets [Mn$_{12}$O$_{12}$(O$_2$CR)$_{16}$(H$_2$O)$_4$] (Mn$_{12}$), where the ligand R being H, CH$_3$, CHCl$_2$ or C$_6$H$_5$,…

Materials Science · Physics 2025-09-16 Shuanglong Liu , Adam V. Bruce , Dmitry Skachkov , James N. Fry , Hai-Ping Cheng

Magnet-superconductor hybrid (MSH) systems have recently emerged as one of the most significant developments in condensed matter physics. This has generated, in the last decade, a steadily rising interest in the understanding of their…

Superconductivity · Physics 2024-10-29 Roberto Lo Conte , Jens Wiebe , Stephan Rachel , Dirk K. Morr , Roland Wiesendanger

The magnetic susceptibility, and low-temperature magnetization curve, of the [3 x 3] grid [Mn(III)4Mn(II)5(2poap-2H)6](ClO4)10.10H2O is analyzed within a spin Hamiltonian approach. The Hilbert space is huge (4,860,000 states), but the…

Strongly Correlated Electrons · Physics 2007-05-23 O. Waldmann , H. U. Güdel , T. L. Kelly , L. K. Thompson

The M-1222 compounds are synthesized in near single phase form. These compounds crystallise in I4/mmm Tetragonal structure. None of the studied compound is superconducting but they asre weakly magnetic. This is first report on synthesis of…

Superconductivity · Physics 2007-05-23 V. P. S. Awana , S. Balamurugan , H. Kishan , E. Takayama-Muromachi

We report a systematic study of Sm valence in the prototypical intermediate valence compound SmB$_6$. Sm mean valence, $v_{\rm Sm}$, was measured by X-ray absorption spectroscopy as functions of pressure ($1<P<13$ GPa) and temperature…

Strongly Correlated Electrons · Physics 2018-05-09 N. Emi , N. Kawamura , M. Mizumaki , T. Koyama , N. Ishimatsu , G. Pristáš , T. Kagayama , K. Shimizu , Y. Osanai , F. Iga , T. Mito

Manganese-rich Heusler compounds are attracting much interest in the context of spin transfer torque and rare-earth free hard magnets. Here we give a comprehensive overview of the magnetic properties of non-centrosymmetric cubic…

Materials Science · Physics 2014-12-10 Lukas Wollmann , Stanislav Chadov , Jürgen Kübler , Claudia Felser

Magnetic switching of a single molecular magnet (SMM) due to spin-polarized current flowing between ferromagnetic metallic electrodes is investigated theoretically. Magnetic moments of the electrodes are assumed to be collinear and parallel…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 Maciej Misiorny , Józef Barnas

The interplay between covalency and magnetism is non-trivial and can be harnessed for designing new functional magnetic materials. Based on a survey using density functional calculations, we show that $TM\unicode{x2013}O$ bond covalency can…

Materials Science · Physics 2020-04-24 M. H. N. Assadi , H. Katayama-Yoshida

The chemical composition, crystal structure, and magnetic properties of a manganese zinc alloy with an ideal composition of YMn2Zn20, which comprises a pyrochlore lattice made of Mn atoms, are reported. The compound is stable only when In…

Materials Science · Physics 2015-06-04 Yoshihiko Okamoto , Takeshi Shimizu , Jun-ichi Yamaura , Zenji Hiroi

The preparation and physical characterization are reported for several single-molecule magnet salts to investigate the effects of paramagnetic cations on the magnetization relaxation behavior of [Mn12]- anionic single-molecule magnets.

Mixed-valence perovskite manganites (Re$_{1-x}$A$_{x}$MnO$_{3}$ where Re=rare earth, A=alkaline earth) provide a unique opportunity to study the relationships between the structure and the magnetotransport properties due to an interplay…

Materials Science · Physics 2009-11-07 W. Prellier , Ph. Lecoeur , B. Mercey

Homogeneous mixed-valence (MV) behaviour is one of the most intriguing phenomena of $f$-electron systems. Despite extensive efforts, a fundamental aspect which remains unsettled is the determination of the limiting cases for which MV…

A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. Tiron , W. Wernsdorfer , D. Foguet-Albiol , N. Aliaga-Alcalde , G. Christou

We examine theoretically electron paramagnetic resonance (EPR) lineshapes as functions of resonance frequency, energy level, and temperature for single crystals of three different kinds of single-molecule nanomagnets (SMMs): Mn$_{12}$…

Composite metamaterials(CMMs) combining a subwavelength metallic hole array (i.e. one-layer fishnet structure) and an array of split-ring resonators(SRRs) on the same board are fabricated with gold films on silicon wafer. Transmission…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Ming Li , Zhenchao Wen , Jinxin Fu , Xu Fang , Yaomin Dai , Rongjuan Liu , Xiufeng Han , Xianggang Qiu