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We use $^2$H NMR to study the rotational motion of supercooled water in silica pores of various diameters, specifically, in the MCM-41 materials C10, C12, and C14. Combination of spin-lattice relaxation, line-shape, and stimulated-echo…

Soft Condensed Matter · Physics 2015-06-22 Matthias Sattig , Stefan Reutter , Franz Fujara , Mayke Werner , Gerd Buntkowsky , Michael Vogel

We develop the multi-band BCS model of superconductivity in the ultrathin films using the orthogonal tight-binding approximation for constructing the electron wavefunctions. This allows for relatively simple determination of the band…

Superconductivity · Physics 2014-07-15 Karol Szałowski

The equilibrium properties of block copolymer micelles confined in polymer thin films are investigated using self-consistent field theory. The theory is based on a model system consisting of AB diblock copolymers and A homopolymers. Two…

Soft Condensed Matter · Physics 2014-01-16 Jiajia Zhou , An-Chang Shi

We study the finite-temperature dynamics of thin elastic sheets in a single-clamped cantilever configuration. This system is known to exhibit a tilt transition at which the preferred mean plane of the sheet shifts from horizontal to a plane…

Soft Condensed Matter · Physics 2023-12-27 Roberto Abril Valenzuela , Paul Z. Hanakata , Mark J. Bowick

Despite their technological relevance, a full microscopic understanding of glasses is still lacking. This applies even more to their surfaces whose properties largely differ from that of the bulk material. Here, we experimentally…

Soft Condensed Matter · Physics 2022-11-23 Li Tian , Clemens Bechinger

We use molecular dynamics simulations to study the static properties of a single linear multiblock copolymer chain under poor solvent conditions varying the block length $N$, the number of blocks $n$, and the solvent quality by variation of…

Soft Condensed Matter · Physics 2015-03-19 N. G. Fytas , P. E. Theodorakis

We introduce a machine-learning approach to predict the complex non-Markovian dynamics of supercooled liquids from static averaged quantities. Compared to techniques based on particle propensity, our method is built upon a theoretical…

Disordered Systems and Neural Networks · Physics 2023-03-17 Simone Ciarella , Massimiliano Chiappini , Emanuele Boattini , Marjolein Dijkstra , Liesbeth M. C. Janssen

The swelling dynamics of polymer gels are characterized by the (collective) diffusion coefficient $D$ of the polymer network. Here, we measure the temperature dependence of $D$ of polymer gels with controlled homogeneous network structures…

The morphological scaling properties of linear polymer films grown by vapor deposition polymerization (VDP) are studied by 1+1D Monte Carlo simulations. The model implements the basic processes of random angle ballistic deposition ($F$),…

Computational Physics · Physics 2010-10-25 Sairam Tangirala , David P. Landau , Y. -P. Zhao

Thin films of diblock copolymer subject to gravitational field are simulated by means of a cell dynamical system model. The difference in density of the two sides of the molecule and the presence of the field causes the formation of…

Materials Science · Physics 2009-10-31 S. Martins , W. A. M. Morgado , M. S. O. Massunaga , M. Bahiana

We compare predictions from two familiar models of the metastable supercooled liquid respectively constructed with thermodynamic and dynamic approach. In the so called density functional theory (DFT) the free energy $F[\rho]$ of the liquid…

Statistical Mechanics · Physics 2016-04-20 Leishangthem Premkumar , Neeta Bidhoodi , Shankar P. Das

Thin films, bubbles and membranes are central to numerous natural and engineering processes, i.e., in thin-film solar cells, coatings, biosensors, electrowetting displays, foams, and emulsions. Yet, the characterization and an adequate…

Fluid Dynamics · Physics 2024-07-18 Muhammad Rizwanur Rahman , Li Shen , James P. Ewen , D. M. Heyes , Daniele Dini , E. R. Smith

Nuclear liquid-gas phase transitions are investigated in the framework of static antisymmetrized molecular dynamics (static AMD) model under either a constant volume or a constant pressure. A deuteron quadrupole momentum fluctuation…

Nuclear Theory · Physics 2021-06-24 W. Lin , P. Ren , X. Liu , H. Zheng , M. Huang , G. Qu , R. Wada

Single particle dynamics of water confined in a nanopore is studied through Computer Molecular Dynamics. The pore is modeled to represent the average properties of a pore of Vycor glass. Dynamics is analyzed at different hydration levels…

Statistical Mechanics · Physics 2009-10-31 P. Gallo , M. Rovere , E. Spohr

Crystalline two-dimensional (2D) superconductors with low carrier density are an exciting new class of materials in which superconductivity coexists with strong interactions, the effects of complex topology are not obscured by disorder, and…

Systems under external confinement and constraints often show interesting properties. In this thesis, we study some systems under external confinement. We begin by finding out the probability distribution of end-to-end separation of a Worm…

Soft Condensed Matter · Physics 2007-05-23 Debasish Chaudhuri

Single partially confined collapsed polymers are studied in two dimensions. They are described by self-avoiding random walks with nearest-neighbour attractions below the $\Theta$-point, on the surface of an infinitely long cylinder. For the…

Statistical Mechanics · Physics 2009-11-07 Hsiao-Ping Hsu , Peter Grassberger

We generalize a recently investigated lattice model of semiflexible polymers formed under equilibrium polymerization in a solution and conduct a comprehensive investigation of its melting properties. The model is characterized by six…

Condensed Matter · Physics 2007-05-23 Sagar S. Rane , P. D. Gujrati

We present fully atomistic Molecular Dynamics simulation results on a main-chain polymer, 1,4-Polybutadiene, in the merging region of the $\alpha$- and $beta$-relaxations. A real space analysis reveals the occurrence of localized motions…

Soft Condensed Matter · Physics 2015-06-25 Juan Colmenero , Arturo Narros , Fernando Alvarez , Arantxa Arbe , Angel J. Moreno

All non-interacting two-dimensional electronic systems are expected to exhibit an insulating ground state. This conspicuous absence of the metallic phase has been challenged only in the case of low-disorder, low density, semiconducting…

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