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Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Wernsdorfer , N. E. Chakov , G. Christou

The Landau Zener model has recently been used to measure very small tunnel splittings in molecular clusters of Fe8, which at low temperature behaves like a nanomagnet with a spin ground state of S = 10. The observed oscillations of the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , I. Chiorescu , R. Sessoli , D. Gatteschi , D. Mailly

The tunnel splitting in biaxial antiferromagnetic particles is studied with a magnetic field applied along the hard anisotropy axis. We observe the oscillation of tunnel splitting as a function of the magnetic field due to the quantum phase…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q. Liang , H. J. W. Müller-Kirsten , D. K. Park , F. -C. Pu

The detailed theoretical understanding of quantum spin dynamics in various molecular magnets is an important step on the roadway to technological applications of these systems. Quantum effects in both ferromagnetic and antiferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael N. Leuenberger , Florian Meier , Daniel Loss

Magnetization measurements of a Mn12mda wheel single-molecule magnet with a spin ground state of S = 7 show resonant tunneling and quantum phase interference, which are established by studying the tunnel rates as a function of a transverse…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 W. Wernsdorfer , T. C. Stamatatos , G. Christou

Macroscopic quantum coherence and spin-phase interference are studied between excited levels in single-domain ferromagnetic particles in a magnetic field along the hard anisotropy axis. The system has the general structure of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Pan Hui , Rong Lu , Jia-Lin Zhu , Yi Zhou

We present details about an experimental method based on the Landau Zener model which allows to measure very small tunnel splittings $\Delta$ in molecular clusters Fe8. The measurements are performed with an array of micro-SQUIDs. The…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , R. Sessoli , A. Caneschi , D. Gatteschi , A. Cornia , D. Mailly

We present a detailed study of the influence of various interactions on the spin quantum tunneling in a Mn12 wheel molecule. The effects of single-ion and exchange (spin-orbit) anisotropy are first considered, followed by an analysis of the…

Materials Science · Physics 2010-09-23 E. del Barco , S. Hill , C. C. Beedle , D. N. Hendrickson , I. S. Tupitsyn , P. C. E. Stamp

The quantum interference effects induced by the topological phase are studied analytically in biaxial antiferromagnets with an external magnetic field at an arbitrarily angle. This study provides a nontrivial generalization of the Kramers…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Rong Lu , Hui Pan , Jia-Lin Zhu , Bing-Lin Gu

We make a theoretical study of the quantum oscillations of the tunneling magnetoresistance (TMR) as a function of the spacer layer thickness. Such oscillations were recently observed in tunneling junctions with a nonmagnetic metallic spacer…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 H. Itoh , J. Inoue A. Umerski , J. Mathon

We measure the low-temperature resistance of permalloy break junctions as a function of contact size and the magnetic field angle, in applied fields large enough to saturate the magnetization. For both nanometer-scale metallic contacts and…

Mesoscale and Nanoscale Physics · Physics 2013-02-07 Kirill I. Bolotin , Ferdinand Kuemmeth , D. C. Ralph

Magnetization measurements of a truly axial symmetry Mn12-tBuAc molecular nanomagnet with a spin ground state of S = 10 show resonance tunneling. This compound has the same magnetic anisotropy as Mn12-Ac but the molecules are better…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 W. Wernsdorfer , M. Murugesu , G. Christou

A Mn4 single-molecule magnet displays asymmetric Berry-phase interference patterns in the transverse-field (HT) dependence of the magnetization tunneling probability when a longitudinal field (HL) is present, contrary to symmetric patterns…

Mesoscale and Nanoscale Physics · Physics 2011-06-02 H. M. Quddusi , J. Liu , S. Singh , K. J. Heroux , E. del Barco , S. Hill , D. N. Hendrickson

The symmetry of magnetic quantum tunneling has been studied in the prototype single molecule magnet Mn$_{12}$-acetate using a micro-Hall effect magnetometer and superconducting high field vector magnet system. An average crystal fourfold…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 E. del Barco , A. D. Kent , E. M. Rumberger , D. N. Hendrickson , G. Christou

We present topological interference effects for the tunneling of a single large spin, which are caused by the symmetry of a general class of magnetic anisotropies. The interference originates from spin Berry phases associated with different…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Michael N. Leuenberger , Daniel Loss

Ramsey et al. [Nature Phys. 4, 277-281 (2008)] report the observation of quantum interference associated with tunnelling trajectories between states of different total spin length in a dimeric molecular nanomagnet. They argue that the…

Mesoscale and Nanoscale Physics · Physics 2008-07-07 W. Wernsdorfer

This article takes a broad view of the understanding of magnetic bistability and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on three families of relatively simple, low-nuclearity transition metal clusters: spin S…

A Mn4 single-molecule magnet (SMM) is used to show that quantum tunneling of magnetization (QTM) is not suppressed by moderate three dimensional exchange coupling between molecules. Instead, it leads to an exchange bias of the quantum…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. Tiron , W. Wernsdorfer , N. Aliaga-Alcalde , D. N. Hendrickson , G. Christou

We formulate the problem of electron transport through a single-molecule magnet (SMM) in the Coulomb blockade regime taking into account topological interference effects for the tunneling of the large spin of a SMM. The interference…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Gabriel Gonzalez , Michael N. Leuenberger

The tunneling splitting in biaxial ferrimagnetic particles at excited states with an explicit calculation of the prefactor of exponent is obtained in terms of periodic instantons which are responsible for tunneling at excited states and is…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q Liang , F. -C Pu
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