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We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

Strongly Correlated Electrons · Physics 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

Ferromagnetic compound PrRu2Si2 exhibits a giant magnetocrystalline anisotropy of about 400 T. Its ordered moment below Tc=14K reaches 2.7 mB and is parallel to [0 0 1] crystalline direction. We have attributed the magnetism of PrRu2S2 to…

Strongly Correlated Electrons · Physics 2009-10-31 R. Michalski , Z. Ropka , R. J. Radwanski

The cause for the preferred spin orientation in magnetic systems containing spin-1/2 transition-metal ions was explored by studying the origin of the easy-plane anisotropy of the spin-1/2 Cu2+ ions in CuCl2.2H2O, LiCuVO4, CuCl2 and CuBr2 on…

Strongly Correlated Electrons · Physics 2015-06-22 Jia Liu , Hyun-Joo Koo , Hongjun Xiang , Reinhard K. Kremer , Myung-Hwan Whangbo

We present a study of the magnetic susceptibility in carefully detwinned La_{2-x}Sr_{x}CuO_4 single crystals in the lightly-doped region (x=0-0.03), which demonstrates a remarkable in-plane anisotropy of the spin system. This anisotropy is…

Superconductivity · Physics 2009-11-07 A. N. Lavrov , Yoichi Ando , Seiki Komiya , I. Tsukada

Among the frustrated magnetic materials, spin-ice stands out as a particularly interesting system. Residual entropy, freezing and glassiness, Kasteleyn transitions and fractionalisation of excitations in three dimensions all stem from a…

Neutron diffraction has been used to investigate the magnetic correlations in single crystals of the spin ice materials Ho2Ti2O7 and Dy2Ti2O7 in an external magnetic field applied along either the [001] or [1-10] crystallographic…

Other Condensed Matter · Physics 2009-11-11 T. Fennell , O. A. Petrenko , B. Fak , J. S. Gardner , S. T. Bramwell , B. Ouladdiaf

Using magnetic neutron scattering we characterize an unusual low temperature phase in orthorhombic SrCuO2. The material contains zigzag spin ladders formed by pairs of S=1/2 chains (J=180 meV) coupled through a weak frustrated interaction…

Materials Science · Physics 2009-10-31 I. A. Zaliznyak , C. Broholm , M. Kibune , M. Nohara , H. Takagi

The spin ice compound Dy$_2$Ti$_2$O$_7$ is well-known to realise a three-dimensional Coulomb spin liquid with magnetically charged monopole excitations. Its fate at low temperatures, however, remains an intriguing open question. Based on a…

We report on the Fe17 high-spin molecular cluster and show that this system is an exemplification of nanostructured dipolar magnetism. Each Fe17 molecule, with spin S=35/2 and axial anisotropy as small as D=-0.02K, is the magnetic unit that…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Evangelisti , A. Candini , A. Ghirri , M. Affronte , G. W. Powell , I. A. Gass , P. A. Wood , S. Parsons , E. K. Brechin , D. Collison , S. L. Heath

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

Neutron scattering has been used to investigate the magnetic correlations in the the spin ice material dysprosium titanate, Dy2Ti2O7. An isotopically enriched sample was used to minimise neutron absorption. In zero field no magnetic order…

We present a detailed theoretical overview of the thermodynamic properties of the dipolar spin ice model, which has been shown to be an excellent quantitative descriptor of the Ising pyrochlore materials Dy_2Ti_2O_7 and Ho_2Ti_2O_7. We show…

Disordered Systems and Neural Networks · Physics 2015-06-24 Roger G. Melko , Matthew Enjalran , Byron C. den Hertog , Michel. J. P. Gingras

LiSr$_2$[CoN$_2$] single crystals were successfully grown out of Li-rich flux. Temperature- and field-dependent measurements of the magnetization in the range of $T = 2 - 300$ K and up to $\mu_{0}\textit{H} = 7$ T as well as measurements of…

Materials Science · Physics 2019-05-15 T. J. Ballé , Z. Zangeneh , L. Hozoi , A. Jesche , P. Höhn

The spin ice materials Ho$_{2}$Ti$_{2}$O$_{7}$ and Dy$_{2}$Ti$_{2}$O$_{7}$ are by now perhaps the best-studied classical frustrated magnets. A crucial step towards the understanding of their low temperature behaviour -- both regarding their…

Strongly Correlated Electrons · Physics 2019-08-14 Bruno Tomasello , Claudio Castelnovo , Roderich Moessner , Jorge Quintanilla

We present polarised-neutron diffraction measurements of the Ising-like spin-chain compound Ca3Co2O6 above and below the magnetic ordering temperature TN. Below TN, a clear evolution from a single-phase spin-density wave (SDW) structure to…

We used single-crystal x-ray and neutron diffraction to investigate the crystal and magnetic structures of trigonal lattice iridate Ca2Sr2IrO6. The crystal structure is determined to be $R\bar3$ with two distinct Ir sites. The system…

Strongly Correlated Electrons · Physics 2018-06-14 Jieming Sheng , Feng Ye , Christina Hoffmann , Valentino R. Cooper , Satoshi Okamoto , Jasminka Terzic , Hao Zheng , Hengdi Zhao , G. Cao

Spin ice systems represent a prime example of constrained spin systems and exhibit rich low-energy physics. In this study, we explore how introducing a tunable anisotropic spin coupling to the conventional Ising spin ice Hamiltonian on the…

Strongly Correlated Electrons · Physics 2025-10-28 Gloria Isbrandt , Frank Pollmann , Michael Knap

While sources of magnetic fields - magnetic monopoles - have so far proven elusive as elementary particles, several scenarios have been proposed recently in condensed matter physics of emergent quasiparticles resembling monopoles. A…

Magnetic properties of high-quality Al-free nonsuperconducting GdBa_2Cu_3O_{6+y} single crystals grown by flux method have been studied. The magnetic anisotropy below the N\'eel temperature T_N~2.3K corresponds to the direction of Gd^{3+}…

Materials Science · Physics 2016-08-31 V. N. Narozhnyi , D. Eckert , G. Fuchs , V. Nekvasil , K. -H. Müller

We report low temperature (1.8-15 K) ac magnetic susceptibility and isothermal remanent magnetization behavior for the single crystalline form of Dy2PdSi3, crystallizing in a AlB2-derived hexagonal structure, for two orientations. The…

Strongly Correlated Electrons · Physics 2007-05-23 K. K. Iyer , P. L. Paulose , E. V. Sampathkumaran , H. Bitterlich , G. Behr , Loeser
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