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We argue on the basis of symmetry selection rules and Raman scattering spectra that NaV$_2$O$_5$ undergoes a charge ordering phase transition at T$_c$=34 K. Such a transition is characterized by the redistribution of the charges at the…

Strongly Correlated Electrons · Physics 2009-10-31 M. J. Konstantinovic , Z. V. Popovic , A. N. Vasil'ev , M. Isobe , Y. Ueda

A new X-ray diffraction study of the one-dimensional spin-Peierls compound \alpha-NaV_2O_5 reveals a centrosymmetric (Pmmn) crystal structure with one type of V site, contrary to the previously postulated non-centrosymmetric P2_1mn…

Condensed Matter · Physics 2009-10-31 H. Smolinski , C. Gros , W. Weber , U. Peuchert , G. Roth , M. Weiden , C. Geibel

We determine the electronic structure of the one-dimensional spin-1/2 Heisenberg compound $\gamma$-LiV$_2$O$_5$, which has two inequivalent vanadium ions, V(1) and V(2), via density-functional calculations. We find a relative V(1)-V(2)…

Condensed Matter · Physics 2009-11-07 R. Valenti , T. Saha-Dasgupta , J. V. Alvarez , K. Pozgajcic , C. Gros

Charge ordering of V4+ and V5+ in NaV2O5 has been studied by an X-ray diffraction technique using anomalous scattering near a vanadium K-absorption edge to critically enhance a contrast between the two ions. A dramatic energy dependence of…

Strongly Correlated Electrons · Physics 2009-10-31 H. Nakao , K. Ohwada , N. Takesue , Y. Fujii , M. Isobe , Y. Ueda , M. v. Zimmermann , J. P. Hill , D. Gibbs , J. C. Woicik , I. Koyama , Y. Murakami

The low-temperature (LT) superstructure of $\alpha'$-NaV$_2$O$_5$ was determined by synchrotron radiation x-ray diffraction. Below the phase transition temperature associated with atomic displacement and charge ordering at 34K, we observed…

An effective intra- and inter-ladder charge-spin hamiltonian for the quarter-filled ladder compound $\alpha'$-NaV$_2$O$_5$ has been derived by using the standard canonical transformation method. In the derivation, it is clear that a finite…

Condensed Matter · Physics 2009-10-31 Debanand Sa , C. Gros

We investigate the magnetic field dependence of the spin-Peierls transition in NaV$_2$O$_5$ in the field range 16T-30T. The transition temperature exhibits a very weak variation with the field, suggesting a novel mechanism for the formation…

Strongly Correlated Electrons · Physics 2009-10-31 S. G. Bompadre , Arthur F. Hebard , Valeri N. Kotov , D. Hall , G. Maris , J. Baas , T. T. M. Palstra

We study a novel S=1/2 cluster chain Hamiltonian which has recently been proposed in the context of the charge ordered low-temperature phase of alpha'-NaV2O5. We perform a detailed investigation of this model within a large range of…

Strongly Correlated Electrons · Physics 2009-10-31 Andreas Honecker , Wolfram Brenig

The present resonant x-ray scattering from each of monoclinically-split single domains of NaV2O5 has critically enhanced contrast between V4+ and V5+ ions strong enough to lead to unambiguous conclusion of the charge-order pattern of its…

We present our theoretical and numerical results on thermodynamic properties and the microscopic mechanism of two successive transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) obtained by Monte Carlo calculations of an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

High-resolution X-ray diffraction data show that the low-temperature superstructure of alpha-NaV2O5 has an F-centered orthorhombic 2a x 2b x 4c superlattice. A structure model is proposed, that is characterized by layers with zigzag charge…

Materials Science · Physics 2009-11-07 Sander van Smaalen , Peter Daniels , Lukas Palatinus , Reinhard K. Kremer

An investigation of the spin excitation spectrum of charge ordered (CO) NaV2O5 is presented. We discuss several different exchange models which may be relevant for this compound, namely in- line and zig-zag chain models with weak as well as…

Strongly Correlated Electrons · Physics 2015-06-25 P. Thalmeier , A. N. Yaresko

We propose a mechanism for the observed stacking charge order in the quarter-filled ladder compound NaV2O5. Via a standard mapping of the charge degrees of freedom onto Ising spins we explain the stacking order as a result of competition…

Strongly Correlated Electrons · Physics 2009-11-10 G. Y. Chitov , C. Gros

23Na NMR spectrum measurements in alpha'-NaV2O5 with a single- crystalline sample are reported. In the charge-ordered phase, the number of inequivalent Na sites observed is more than that expected from the low-temperature structures of…

Strongly Correlated Electrons · Physics 2009-10-31 Tetsuo Ohama , Atsushi Goto , Tadashi Shimizu , Emi Ninomiya , Hiroshi Sawa , Masahiko Isobe , Yutaka Ueda

We present results of high-resolution thermal-expansion and specific-heat measurements on single crystalline alpha'-NaV2O5. We find clear evidence for two almost degenerate phase transitions associated with the formation of the dimerized…

Condensed Matter · Physics 2009-10-30 M. Koeppen , D. Pankert , R. Hauptmann , M. Lang , M. Weiden , C. Geibel , F. Steglich

The one-dimensional transverse Ising model is a paradigmatic example of quantum criticality. In spin-orbit coupled systems, however, effective Ising interactions arise alongside bond-dependent couplings such as Kitaev ($K$) and $\Gamma$…

Strongly Correlated Electrons · Physics 2026-03-17 Mandev Bhullar , Philip Richard , Hae-Young Kee

We study a model of two weakly coupled isotropic spin-1/2 Heisenberg chains with an antiferromagnetic coupling along the chains. It is shown that the system always has a spectral gap. For the case of identical chains the model in the…

Condensed Matter · Physics 2009-10-28 D. G. Shelton , A. A. Nersesyan , A. M. Tsvelik

We discuss magnetic excitations of a spin-cluster model which has been suggested to describe the low temperature phase of alpha'-NaV_2O_5. This model fulfills all symmetry criteria proposed by recent x-ray investigations. We find that this…

Strongly Correlated Electrons · Physics 2008-03-26 Simon Trebst , Anirvan Sengupta

The semiconductor-semiconductor transition of La2RuO5 is studied by means of augmented spherical wave (ASW) electronic structure calculations as based on density functional theory and the local density approximation. This transition has…

Strongly Correlated Electrons · Physics 2007-05-23 Volker Eyert , Stefan Ebbinghaus , Thilo Kopp

We present our theoretical results on the mechanism of two transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) in which magnetic V cations constitute a geometrically-frustrated pyrochlore structure. We have derived an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu