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The mechanism of spin reorientation in Nd$_{2}$Fe$_{14}$B, which is a host crystal of a well-known neodymium permanent magnet, is studied by combining first-principles calculations and Monte Carlo simulations. The spin reorientation is…

Materials Science · Physics 2023-04-24 Hung Ba Tran , Yu-ichiro Matsushita

We have studied spin excitation spectra in the Shastry-Sutherland model compound SrCu$_2$(BO$_3$)$_2$ in magnetic fields using far-infrared Fourier spectroscopy. The transitions from the ground singlet state to the triplet state at 24…

Other Condensed Matter · Physics 2009-11-10 T. Rõõm , D. Hüvonen , U. Nagel , J. Hwang , T. Timusk

In magnetic multilayer systems, a large spin-orbit coupling at the interface between heavy metals and ferromagnets can lead to intriguing phenomena such as the perpendicular magnetic anisotropy, the spin Hall effect, the Rashba effect, and…

Frustrated triangular molecule magnets such as \{Cu$_3$\} are characterized by two degenerate S=1/2 ground-states with opposite chirality. Recently it has been proposed theoretically [PRL {\bf 101}, 217201 (2008)] and verified by {\it…

Mesoscale and Nanoscale Physics · Physics 2013-03-15 J. F. Nossa , M. F. Islam , C. M. Canali , M. R. Pederson

Dzyaloshinskii-Moriya interaction (DMI) is the primary mechanism for realizing real-space chiral spin textures, which are regarded as key components for the next-generation spintronics. However, DMI arises from a perturbation term of the…

Materials Science · Physics 2022-10-12 Fan Zhang , Xueao Li , Yabei Wu , Xiaolong Wang , Jijun Zhao , Weiwei Gao

We have investigated magnetoelectric coupling in the single-molecule magnet $\mathrm{Mn}_{4}\mathrm{Te}_{4}(\mathrm{P}\mathrm{Et}_{3})_{4}$ with tetrahedral spin frustration. Our density functional studies found that an electric dipole…

Materials Science · Physics 2022-08-31 Jie-Xiang Yu , Jia Chen , Neil Sullivan , Hai-Ping Cheng

The influence of the spin-orbit coupling on the magnetic structure of deposited transition metal nanostructure systems has been studied by fully relativistic electronic structure calculations. The interplay of exchange coupling and magnetic…

Materials Science · Physics 2009-02-20 S. Mankovsky , S. Bornemann , J. Minár , S. Polesya , H. Ebert , J. B. Staunton , A. I. Lichtenstein

Motivated by recent synthetic and theoretical progress we consider magnetism in crystals of multi-nuclear organometallic complexes. We calculate the Heisenberg symmetric exchange and the Dzyaloshinskii-Moriya antisymmetric exchange. We show…

Strongly Correlated Electrons · Physics 2017-08-04 B. J. Powell , J. Merino , A. L. Khosla , A. C. Jacko

We present an overview of the microscopic theory of the Dzyaloshinskii-Moriya (DM) coupling in strongly correlated 3d compounds. Most attention in the paper centers around the derivation of the Dzyaloshinskii vector, its value, orientation,…

Strongly Correlated Electrons · Physics 2019-10-24 A. S. Moskvin

We theoretically study the Dzyaloshinskii-Moriya interaction (DMI) mediated by band electrons with strong spin-orbit coupling (SOC). We first derive a general formula for the coefficient ${\bm D}_i$ of the DMI in free energy in terms of…

Mesoscale and Nanoscale Physics · Physics 2023-11-08 Yuto Hayakawa , Yusuke Imai , Hiroshi Kohno

We study how spin and orbital effects influence the capability of promoting Dzyaloshinskii-Moriya (DM) interaction by studying the two magnetic polar materials, Cu(IO3)2 (S = 1/2 with orbital contribution) and Mn(IO3)2 (S = 5/2 with…

Magnetic excitations in the isostructural spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8 are probed by means of high-field electron spin resonance at sub-terahertz frequencies. Three types of magnetic modes were observed. One mode is gapless and…

We perform a low temperature Raman scattering study of phononic and collective spin excitations in the orthogonal dimers compound SrCu_2(BO_3)_2, focussing on the symmetry and the effects of external fields on the magnetic modes. The zero…

Strongly Correlated Electrons · Physics 2009-11-11 A. Gozar , B. S. Dennis , H. Kageyama , G. Blumberg

Chirality-induced spin selectivity (CISS) was recently observed in photo-excited donor-chiral bridge-acceptor molecules, but a predictive theory able to explain available experiments is still lacking. Here we show that low-energy torsional…

The influence of the Dzyaloshinskii-Moriya interaction on the spin-wave dispersion in an Fe double layer grown on W(110) is measured for the first time. It is demonstrated that the Dzyaloshinskii-Moriya interaction breaks the degeneracy of…

Materials Science · Physics 2024-05-28 Kh. Zakeri , Y. Zhang , J. Prokop , T. -H. Chuang , N. Sakr , W. X. Tang , J. Kirschner

The Dzyaloshinskii-Moriya (DM) interaction is an antisymmetric exchange interaction that is responsible for the emergence of chiral magnetism. The origin of the DM interaction, however, remains to be identified albeit the large number of…

Mesoscale and Nanoscale Physics · Physics 2019-07-03 Naoaki Kato , Masashi Kawaguchi , Yong-Chang Lau , Toru Kikuchi , Yoshinobu Nakatani , Masamitsu Hayashi

We perform a symmetry analysis of the ABC-stacked kagome planes of Mn atoms common to the $L1_2$ Mn$_3$X and antiperovskite Mn$_3$AB alloys. In addition to the single-ion-anisotropy and Kitaev-type anisotropic exchange known to stabilize…

Strongly Correlated Electrons · Physics 2023-02-22 J. S. R. McCoombs , A. Zelenskiy , M. L. Plumer , B. W. Southern , T. L. Monchesky

Magnetoelectric properties are studied by a combined experimental and theoretical study of a quasi-two-dimensional material composed of square cupolas, Ba(TiO)Cu$_4$(PO$_4$)$_4$. The magnetization is measured up to above the saturation…

We present a physical picture for the emergence of the Dzyaloshinskii--Moriya (DM) interaction based on the idea of the Doppler shift by an intrinsic spin current induced by spin--orbit interaction under broken inversion symmetry. The…

Mesoscale and Nanoscale Physics · Physics 2016-06-15 Toru Kikuchi , Takashi Koretsune , Ryotaro Arita , Gen Tatara

We present a unified account of magnetic exchange and Raman scattering in the quasi-one-dimensional transition-metal oxide NaV$_2$O$_5$. Based on a cluster-model approach explicit expressions for the exchange integral and the Raman-operator…

Strongly Correlated Electrons · Physics 2009-10-31 Roser Valenti , Claudius Gros , Wolfram Brenig