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The methyl groups in hexamethylbenzene C$_6$(CH$_3$)$_6$ become magnetically ordered at the molecular level below 118 K. This is also near the temperature at which the system structurally transitions from triclinic to a unique near-cubic…

Strongly Correlated Electrons · Physics 2018-12-07 Fei Yen

As the simplest element in nature, unraveling the phase diagram of hydrogen is a primary task for condensed matter physics. As conjectured many decades ago, in the low-temperature and high-pressure part of the phase diagram, solid hydrogen…

Superconductivity · Physics 2023-11-14 Mehmet Dogan , Sehoon Oh , Marvin L. Cohen

We present an accurate study of the static-nucleus electronic energy band gap of solid molecular hydrogen at high pressure. The excitonic and quasiparticle gaps of the $C2/c$, $Pc$, $Pbcn$, and $P6_3/m$ structures at pressures of 250, 300,…

Materials Science · Physics 2017-01-25 Sam Azadi , N. D. Drummond , W. M. C. Foulkes

A calculation of the rotational S$_0$(0) frequencies in high pressure solid para-hydrogen is performed. Convergence of the perturbative series at high density is demonstrated by the calculation of second and third order terms. The results…

Statistical Mechanics · Physics 2009-11-10 Francesco Grazzi , Massimo Moraldi , Lorenzo Ulivi

We use the diffusion quantum Monte Carlo (DMC) method to calculate the ground state phase diagram of solid molecular hydrogen and examine the stability of the most important insulating phases relative to metallic crystalline molecular…

Materials Science · Physics 2015-06-16 S. Azadi , W. M. C. Foulkes , T. D. Kuehne

We study the electronic excitation spectra in solid molecular hydrogen (phase I) at ambient temperature and 5-90 GPa pressures using Quantum Monte Carlo methods and Many-Body Perturbation Theory. In this range, the system changes from a…

Materials Science · Physics 2024-05-21 Vitaly Gorelov , Markus Holzmann , David M. Ceperley , Carlo Pierleoni

Perturbed angular correlation spectroscopy combined with $ab-initio$ electronic structure calculations is used to unravel the structural phase transition path from the low-temperature polar structure to the high-temperature structural phase…

The high critical superconducting temperatures ($T_c$s) of metal hydride phases with clathrate-like hydrogen networks have generated great interest. Herein, we employ the Density Functional Theory-Chemical Pressure (DFT-CP) method to…

Superconductivity · Physics 2022-05-25 Katerina P. Hilleke , Eva Zurek

We compute the thermodynamic phase diagram of seventeen elemental metals with hexagonal close-packed (hcp), face-centered cubic (fcc), and body-centered cubic (bcc) crystal structures using finite-temperature density functional theory.…

Materials Science · Physics 2026-04-15 S. Azadi , S. M. Vinko , A. Principi , T. D. Kuehne , M. S. Bahramy

Extensive Path Integral Monte Carlo simulations of condensed para-Hydrogen in two dimensions at low temperature have been carried out. In the zero temperature limit, the system is a crystal at equilibrium, with a triangular lattice…

Statistical Mechanics · Physics 2009-11-10 Massimo Boninsegni

Firstly, I give a brief summary of the current understanding of QCD below and near $T_c$ (the critical temperature of the chiral transition). Some emphases are put on the qualitative difference between the Yukawa regime ($T \sim 0)$ and the…

High Energy Physics - Phenomenology · Physics 2016-09-01 Tetsuo Hatsuda

The transition of a warm dense fluid hydrogen from insulator to a conducting state at pressures of the order of 20-300 GPa and temperatures of 1000-5000 K has been the subject of active scientific research over the past few decades. The use…

Other Condensed Matter · Physics 2022-04-14 Ilya Fedorov , Vladimir Stegailov

We present results of a theoretical study of para-hydrogen and ortho-deuterium clusters at low temperature (0.5 K < T < 3.5 K), based on Path Integral Monte Carlo simulations. Clusters of size up to N=21 para-hydrogen molecules are nearly…

Statistical Mechanics · Physics 2007-05-23 Fabio Mezzacapo , Massimo Boninsegni

We present results predicting experimentally measurable structural quantities from molecular dynamics studies of hydrogen. In doing this, we propose a paradigm shift for experimentalists -- that the predictions from such calculations should…

Materials Science · Physics 2020-03-25 Graeme J. Ackland , John S. Loveday

We perform molecular dynamics simulations driven by accurate Quantum Monte Carlo forces on dense liquid hydrogen. Recently it has been reported a complete atomization transition between a mixed-atomic liquid and a completely dissociated…

Strongly Correlated Electrons · Physics 2015-06-23 Guglielmo Mazzola , Sandro Sorella

For a long time, there have been huge discrepancies between different models and experiments concerning the liquid-liquid phase transition (LLPT) in dense hydrogen. In this work, we present the results of extensive calculations of the LLPT…

Computational Physics · Physics 2019-12-10 Binbin Lu , Dongdong Kang , Dan Wang , Tianyu Gao , Jiayu Dai

Restricted path integral Monte Carlo simulations are used to calculate the equilibrium properties of hydrogen in the density and temperature range of $9.83 \times 10^{-4}\rm \leq \rho \leq 0.153 \rm gcm^{-3}$ and $5000 \leq T \leq 250 000…

Plasma Physics · Physics 2009-11-07 B. Militzer , D. M. Ceperley

The high-pressure II-III phase transition in solid hydrogen is investigated using the random phase approximation and diffusion Monte Carlo. Good agreement between the methods is found confirming that an accurate treatment of exchange and…

Materials Science · Physics 2024-10-08 Maria Hellgren , Damian Contant , Thomas Pitts , Michele Casula

Temperature dependent electrical resistivity, crystal structure and heat capacity measurements reveal a resistivity drop and metal to semiconductor transition corresponding to first order structural phase transition near 400 K in Ca3Co4O9.…

Materials Science · Physics 2012-04-17 Tao Wu , Trevor A. Tyson , Haiyan Chen , Jianming Bai , Hsin Wang , Cherno Jaye

Phase I of hydrogen has several peculiarities. Despite having a close-packed crystal structure, it is less dense than either the low temperature Phase II or the liquid phase. At high pressure, it transforms into either phase III or IV,…

Computational Physics · Physics 2016-05-17 Ioan B Magdau , Floris Balm , Graeme J Ackland