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We present the phase diagram of a system of mesogenic top-shaped molecules based on the Parsons- Lee density functional theory and Monte Carlo simulation. The molecules are modeled as a hard spherocylinder with a hard sphere embedded in its…

Soft Condensed Matter · Physics 2011-06-13 D. de las Heras , S. Varga , F. J. Vesely

We numerically investigate two-dimensional systems of hard rectangles at constant pressure through extensive hard-particle Monte Carlo simulations. We determine the complete phase diagram as a function of packing fraction and aspect ratio,…

Soft Condensed Matter · Physics 2025-05-15 Denis Dertli , Thomas Speck

We have carried out Monte Carlo simulations of zig-zag shaped molecules where the the molecules is composed of three rigidly linked hard spherocylinder arranged in a zigzag fashion. By varying zigzag angle we have mapped out the whole phase…

Statistical Mechanics · Physics 2013-05-29 Prabal K. Maiti , Yves Lansac , Matthew A. Glaser , Noel A. Clark

Using the classical density functional theory of freezing and Monte Carlo computer simulations, we explore the liquid-crystalline phase behavior of hard rectangles on flat and cylindrical manifolds. Moreover, we study the effect of a static…

Soft Condensed Matter · Physics 2018-02-19 Christoph E. Sitta , Frank Smallenburg , Raphael Wittkowski , Hartmut Löwen

Using particle-resolved molecular-dynamics simulations, we compute the phase diagram for soft repulsive spherocylinders confined on the surface of a sphere. While crystal (K), smectic (Sm), and isotropic (I) phases exhibit a stability…

Soft Condensed Matter · Physics 2025-11-03 Jaydeep Mandal , Hartmut Löwen , Prabal K. Maiti

Recently, a new class of smectic liquid crystal phases (SmCP phases) characterized by the spontaneous formation of macroscopic chiral domains from achiral bent-core molecules has been discovered. We have carried out Monte Carlo simulations…

Statistical Mechanics · Physics 2009-11-07 Yves Lansac , Prabal K. Maiti , Noel A. Clark , Matthew A. Glaser

Using Monte Carlo simulation methods, we explore the role of molecular shape in the phase behavior of liquid crystals and the electroclinic effect. We study a "bent-rod" mesogen shaped like the letter Z, composed of seven soft spheres…

Soft Condensed Matter · Physics 2009-10-31 J. Xu , R. L. B. Selinger , J. V. Selinger , B. R. Ratna , R. Shashidhar

Monte Carlo simulation based on Metropolis algorithm has been used with a great success to analyze the dynamic phase transition properties of a single spherical core-shell nanoparticle system with a spin-3/2 core surrounded by a spin-1…

Statistical Mechanics · Physics 2015-06-15 Erol Vatansever , Hamza Polat

We investigated the nematic to smectic transition undergone by parallel hard spherocylinders in the framework provided by the residual multi-particle entropy (RMPE) formalism. The RMPE is defined as the sum of all contributions to the…

Soft Condensed Matter · Physics 2011-10-26 D. Costa , F. Saija , P. V. Giaquinta

Semiflexible polymers in concentrated lyotropic solution are studied within a bead-spring model by molecular dynamics simulations, focusing on the emergence of a smectic A phase and its properties. We systematically vary the density of the…

Soft Condensed Matter · Physics 2019-01-28 Andrey Milchev , Arash Nikoubashman , Kurt Binder

A coupled phase-field and hydrodynamic model is introduced to describe a two-phase, weakly compressible smectic (layered phase) in contact with an isotropic fluid of different density. A non-conserved smectic order parameter is coupled to a…

Soft Condensed Matter · Physics 2022-02-02 Eduardo Vitral , Perry H. Leo , Jorge Viñals

The scaled particle theory is developed for the description of thermodynamical properties of a mixture of hard spheres and hard spherocylinders. Analytical expressions for free energy, pressure and chemical potentials are derived. From the…

Soft Condensed Matter · Physics 2017-12-15 M. F. Holovko , M. V. Hvozd

This research focuses on the unique phase behavior of non-spherical patchy colloids in porous environments. Based on the theory of scaled particle (SPT), methods have been refined and applied to analyze the thermodynamic properties of…

Soft Condensed Matter · Physics 2024-04-02 V. I. Shmotolokha , M. F. Holovko

We report a molecular dynamics simulation demonstrating that the Smectic B crystalline phase (Cr-B), commonly observed in mesogenic systems of anisotropic molecules, can be formed by a system of identical particles interacting via a…

Soft Condensed Matter · Physics 2013-12-16 A. Metere , T. Oppelstrup , S. Sarman , A. Laaksonen , M. Dzugutov

By employing Molecular Dynamics computer simulations, the phase behavior of systems of rodlike particles with varying degree of internal flexibility has been traced from the perfectly rigid rod limit till very flexible particles, and from…

Soft Condensed Matter · Physics 2009-11-13 Giorgio Cinacchi , Luca De Gaetani

We investigate the phase behaviour of a two-dimensional colloidal model system of ultra-soft particles on a substrate which varies periodically along one spatial direction. Our calculations are based on mean-field density functional theory…

Soft Condensed Matter · Physics 2021-03-17 Alexander Kraft , Sabine H. L. Klapp

We report the smectic $A_F$, a new liquid crystal phase of the ferroelectric nematic realm. The smectic $A_F$ is a phase of small polar, rod-shaped molecules which form two-dimensional fluid layers spaced by approximately the mean molecular…

We use numerical simulations to understand how random deviations from the ideal spherical shape affect the ability of hard particles to form fcc crystalline structures. Using a system of hard spheres as a reference, we determine the…

Soft Condensed Matter · Physics 2010-12-23 William L. Miller , Angelo Cacciuto

Following the groundbreaking discovery of the ferroelectric nematic liquid crystal phase (NF), a series of closely-related new polar phases have also been found. An especially interesting one is the ferroelectric smectic A phase (SmAF) with…

Soft Condensed Matter · Physics 2024-11-14 Aitor Erkoreka , Minjung Huang , Satoshi Aya , Josu Martinez-Perdiguero

We investigate the isotropic-to-nematic phase transition in systems of hard helical particles, using Onsager theory and Monte Carlo computer simulations. Motivation of this work resides in the ubiquity of the helical shape motif in many…

Soft Condensed Matter · Physics 2013-05-01 Elisa Frezza , Alberta Ferrarini , Hima Bindu Kolli , Achille Giacometti , Giorgio Cinacchi
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