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The linear conductance of a molecular conductor oscillating between two metallic leads is investigated numerically both for Hubbard interacting and noninteracting electrons. The molecule-leads tunneling barriers depend on the molecule…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 K. A. Al-Hassanieh , C. A. Büsser , G. B. Martins , E. Dagotto

Time-resolved Faraday rotation has recently demonstrated coherent transfer of electron spin between quantum dots coupled by conjugated molecules. Using a transfer Hamiltonian ansatz for the coupled quantum dots, we calculate the Faraday…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Florian Meier , Veronica Cerletti , Oliver Gywat , Daniel Loss , D. D. Awschalom

The dependence of the transport properties on the specific location of the Fermi level in molecular electronics devices is studied by using electrodes of different materials. The zero-bias transport properties are shown to depend…

Mesoscale and Nanoscale Physics · Physics 2008-12-06 V. M. García-Suárez , C. J. Lambert

Biological systems are known to communicate by diffusing chemical signals in the surrounding medium. However, most of the recent literature has neglected the electron transfer mechanism occurring amongst living cells, and its role in…

Emerging Technologies · Computer Science 2015-02-23 Nicolo Michelusi , Sahand Pirbadian , Mohamed Y. El-Naggar , Urbashi Mitra

The electronic conduction of a novel, three-terminal molecular architecture, analogous to a heterojunction bipolar transistor is studied. In this architecture, two diode arms consisting of donor-acceptor molecular wires fuse through a ring,…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Haiying He , Ravindra Pandey , Shashi P. Karna

Tunneling of electrons through the barriers in heterostructures has been studied, within unified transfer matrix approach. The effect of barrier width on the transmission coefficient of the electrons has been investigated for different…

Mesoscale and Nanoscale Physics · Physics 2010-02-10 Jatindranath Gain , Madhumita Das Sarkar , Sudakshina Kundu

We obtain the conductance of a system of electrons connected to leads, within time-dependent density-functional theory, using a direct relation between the conductance and the density response function. Corrections to the non-interacting…

Materials Science · Physics 2007-10-04 P. Bokes , J. Jung , R. W. Godby

Electron transport is theoretically investigated in a molecular device made of anthracene molecule attached to the electrodes by thiol end groups in two different configurations (para and meta, respectively). Molecular system is described…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Kamil Walczak

We discuss a new mechanism for the electron capture in fast ion-atom collisions. Similarly like in the radiative capture, where the electron transfer occurs due to photon emission, within the mechanism under consideration the electron…

Atomic Physics · Physics 2008-08-06 A. B. Voitkiv , B. Najjari , J. Ullrich

Electronic transport through a quantum wire sandwiched between two metallic electrodes and coupled to a quantum ring, threaded by a magnetic flux $\phi$, is studied. An analytic approach for the electron transport through the bridge system…

Mesoscale and Nanoscale Physics · Physics 2009-11-06 Santanu K. Maiti

We study a simple quantum mechanical symmetric donor-acceptor model for electron transfer (ET) with coupling to internal deformations. The model contains several basic properties found in biological ET in enzymes and photosynthetic centers;…

Quantum Physics · Physics 2015-06-26 P. G. Etchegoin

Molecules of bisthiolterthiophene have been adsorbed on the two facing gold electrodes of a mechanically controllable break junction in order to form metal-molecule(s)-metal junctions. Current-voltage (I-V) characteristics have been…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 C. Kergueris , J. -P. Bourgoin , S. Palacin , D. Esteve , C. Urbina , M. Magoga , C. Joachim

Electron transfer at electrode interfaces to molecules in solution or at the electrode surface plays a vital role in numerous technological processes. However, treating these processes requires a unified and accurate treatment of the…

Chemical Physics · Physics 2023-07-19 Kenneth A. Jung , Joseph Kelly , Thomas E. Markland

We consider a prototype polyene chain: donor-$\pi$(bridge)-acceptor. The distance between the donor and the acceptor is varied by increasing the number of bridged atoms and rate of electron transfer, k$_{et}$ is studied for a series of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. Lakshmi , Ayan Datta , Swapan K. Pati

We have investigated the transport characteristics of an electron pump consisting of an asymmetric double quantum dot at zero bias voltage which is subject to electromagnetic radiation. Depending on the energies of the intermediate states…

Mesoscale and Nanoscale Physics · Physics 2008-02-03 T. H. Stoof , Yu. V. Nazarov

We develop an Over Barrier Model for computing charge exchange between ions and one-active-electron atoms at low impact energies. The main feature of the model is the treatment of the barrier crossing process by the electron within a…

Atomic Physics · Physics 2007-05-23 F. Sattin

The interaction of metal-molecule-metal junctions with light is considered within a simple generic model. We show, for the first time, that light induced current in unbiased junctions can take place when the bridging molecule is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan

We develop a mathematically rigorous theory for the quantum transfer processes in degenerate donor-acceptor dimers in contact with a thermal environment. We calculate explicitly the transfer rates and the acceptor population efficiency. The…

Quantum Physics · Physics 2020-07-15 Marco Merkli , Gennady P. Berman , Avadh Saxena

Conduction of electrons in matter is ultimately described by quantum mechanics. Yet at low frequency or long time scales, low temperature quantum transport is perfectly described by this very simple idea: electrons are emitted by the…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Karl Thibault , Julien Gabelli , Christian Lupien , Bertrand Reulet

We study electron transfer between two separated nuclei using local control theory. By conditioning the algorithm in a symmetric system formed by two protons, one can favored slow transfer processes, where tunneling is the main mechanism,…

Quantum Physics · Physics 2018-04-18 Patricia Vindel-Zandbergen , Christoph Meier , Ignacio R. Sola