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The competition between antiferromagnetic and spin-singlet ground states within quantum spin models and the 1/2-filled band Hubbard model has received intense scrutiny. Here we demonstrate a frustration-induced transition from N\'{e}el…

Strongly Correlated Electrons · Physics 2014-07-28 H. Li , R. T. Clay , S. Mazumdar

Quantum spin liquids (QSLs) represent highly entangled states of matter in which frustration-induced quantum fluctuations suppress any symmetry-breaking phase transition down to absolute zero, giving rise to fractionalized excitations and…

A field-induced quantum spin liquid (QSL) state is an extraordinary phenomenon, hitherto unobserved in metallic frustrated compounds. Recent bulk measurements have revealed intriguing field-induced magnetic states in metallic frustrated…

Strongly Correlated Electrons · Physics 2026-01-12 I. Ishant , Z. Guguchia , V. Fritsch , O. Stockert , M. Majumder

Inelastic neutron scattering measurements are reported that show a new longitudinal mode in the antiferromagnetically ordered phase of the spin-1/2 quasi-one-dimensional antiferromagnet KCuF3. This mode signals the cross-over from…

Strongly Correlated Electrons · Physics 2009-10-31 B. Lake , D. A. Tennant , S. E. Nagler

Motivated by the experimental realization of quantum spin models of polar molecule KRb in optical lattices, we analyze the spin 1/2 dipolar Heisenberg model with competing anisotropic, long-range exchange interactions. We show that, by…

Quantum Gases · Physics 2017-08-03 Haiyuan Zou , Erhai Zhao , W. Vincent Liu

Spinel-structured compounds serve as prototypical examples of highly frustrated systems, and are promising candidates for realizing the long-sought quantum spin liquid (QSL) state. However, structural disorder is inevitable in many real QSL…

Motivated by the recent synthesis of the spin-1 A-site spinel NiRh$_{\text 2}$O$_{\text 4}$, we investigate the classical to quantum crossover of a frustrated $J_1$-$J_2$ Heisenberg model on the diamond lattice upon varying the spin length…

Strongly Correlated Electrons · Physics 2018-02-01 Finn Lasse Buessen , Max Hering , Johannes Reuther , Simon Trebst

Inelastic neutron scattering is used to identify single-particle and continuum spin excitations in the quasi-one-dimensional $S=1/2$ antiferromagnet \ba. In the data analysis, close attention is given to resolution effects. A gap in the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Zheludev , M. Kenzelmann , S. Raymond , T. Masuda , K. Uchinokura , S. -H. Lee

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…

Strongly Correlated Electrons · Physics 2021-08-03 Samuel Mañas-Valero , Benjamin Huddart , Tom Lancaster , Eugenio Coronado , Francis Pratt

We present variational results for the ground state of the antiferromagnetic quantum Heisenberg model with frustrating next-nearest-neighbour interactions. The trial wave functions employed are of resonating-valence-bond type, elaborated to…

Strongly Correlated Electrons · Physics 2013-10-24 Xiaoming Zhang , Jin Xu , K. S. D. Beach

Quantum spin liquids are highly entangled magnetic states with exotic properties. The $S = 1/2$ square-lattice Heisenberg model is one of the foundational models in frustrated magnetism with a predicted, but never observed, quantum spin…

Spin waves in the type-III ordered antiferromagnetic state of the frustrated $t$-$t'$ Hubbard model on the fcc lattice are calculated to investigate finite-$U$-induced competing interaction and frustration effects on magnetic excitations…

Strongly Correlated Electrons · Physics 2017-04-04 Avinash Singh , Shubhajyoti Mohapatra , Timothy Ziman , Tapan Chatterji

Inelastic neutron scattering and bulk magnetic susceptibility studies of the quantum S=1/2 spin ladder system IPA-CuCl3 are performed under hydrostatic pressure. The pressure dependence of the spin gap $\Delta$ is determined. At $P=1.5$ GPa…

Strongly Correlated Electrons · Physics 2008-12-10 Tao Hong , V. O. Garlea , A. Zheludev , J. Fernandez-Baca , H. Manaka , S. Chang , J. B. Leao , S. J. Poulton

A comprehensive inelastic neutron scattering study of magnetic excitations in the near-optimally doped high-temperature superconductor ${\rm YBa_{2}Cu_{3}O_{6.85}}$ is presented. The spin correlations in the normal state are commensurate…

Superconductivity · Physics 2009-10-31 P. Bourges , Y. Sidis , H. F. Fong , L. P. Regnault , J. Bossy , A. Ivanov , B. Keimer

We study the magnetism of a quantum spin-1/2 antiferromagnet on a maple-leaf lattice which is obtained by regularly depleting 1/7 of the sites of a triangular lattice. Although the interactions are set to be spatially uniform, the ground…

Strongly Correlated Electrons · Physics 2021-12-14 Ryo Makuta , Chisa Hotta

The magnetic susceptibility of the gapped quantum spin liquid compound (C$_4$H$_{12}$N$_2$)Cu$_2$Cl$_6$ and its chemically disordered derivatives (C$_4$H$_{12}$N$_2$)Cu$_2$(Cl$_{1-x}$Br$_{x}$)$_6$ are systematically studied in magnetic…

Strongly Correlated Electrons · Physics 2015-06-16 D. Hüvonen , G. Ballon , A. Zheludev

We present powder inelastic neutron scattering measurements of the S=1 dimerized antiferromagnet Ba$_3$Mn$_2$O$_8$. The $T=1.4$ K magnetic spectrum exhibits a spin-gap of $\Delta \approx 1.0$ meV and a dispersive spectrum with a bandwidth…

Strongly Correlated Electrons · Physics 2009-11-13 M. B. Stone , M. D. Lumsden , Y. Qiu , E. C. Samulon , C. D. Batista , I. R. Fisher

Neutron elastic and inelastic scattering measurements have been performed in order to investigate the spin structure and the magnetic excitations in the impurity-induced antiferromagnetic ordered phase of the doped spin gap system…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , M. Fujisawa , K. Kakurai , H. Tanaka

Inelastic neutron scattering study on the spin-chain compound Sr$_3$NiIrO$_6$ reveals gapped quasi-1D magnetic excitations. The observed one-magnon band between 29.5 and 39 meV consists of magnon modes of the Ni$^{2+}$ ions. The fitting of…

Strongly Correlated Electrons · Physics 2016-06-01 S. Toth , W. Wu , D. T. Adroja , S. Rayaprol , E. V. Sampathkumaran