Related papers: Response theory for time-resolved second-harmonic …
Ideally, strong non-linearities could be used to implement quantum gates for photonic qubits by well controlled two photon interactions. However, the dependence of the non-linear interaction on frequency and time makes it difficult to…
The theory for time-resolved photoemission spectroscopy as applied to pump-probe experiments is developed and solved for the generic case of a strongly correlated material. The formal development incorporates all of the nonequilibrium…
We experimentally demonstrate coherent control of the nonlinear response of optical second harmonic generation in resonant nanostructures beyond the weak-field regime. Contrary to common perception, we show that maximizing the intensity of…
We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…
The nonlinear photon-photon interaction mediated by a single two-level atom is studied theoretically based on a one-dimensional model of the field-atom interaction. This model allows us to determine the effects of an atomic nonlinearity on…
Head-on collision of laser-induced plasma wakefields with differing profiles of electrostatic potential has been recently found to be an efficient mechanism for generating high-power electromagnetic emission at the second harmonic of the…
A systematic study of the nonlinear response of Silicon Photomultipliers (SiPMs) has been conducted through Monte Carlo simulations. SiPMs have been proven to show a universal nonlinear response when it is expressed in terms of relative…
Time-resolved angle-resolved photoemission spectroscopy is one of the most powerful pump-probe measurements of materials driven far from equilibrium. Unlike the linear-response regime, where the frequency-dependent response function is…
Rapid modulation of the electromagnetic response in both time and space creates temporal boundaries in the medium and leads to time-reflection and time-refraction of light and to the eventual formation of the photonic time crystal within…
The theory of Bloembergen and Pershan for the light waves at the boundary of nonlinear media is extended to a nonlinear two-dimensional atomic crystal, i.e. a single planar atomic lattice, placed in between linear bulk media. The crystal is…
Second-order nonlinear optical responses, including photogalvanic effect (PGE) and second harmonic generation (SHG), are important physical phenomena in nonlinear optics. The PGE (SHG) related to linearly and circularly polarized light are…
We derive the two-time linear response theory for out-of-equilibrium pumped systems, generic pump-probe delays and probe frequencies. Such a theory enormously simplifies the numerical calculations, for instance, of the optical conductivity…
We develop a microscopic large-$N$ theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory, which reduces to the well-known random…
We study the interaction of Gaussian one- and two-photon pulses with a single two-level atom based on a one-dimensional model of pulse propagation to and from the atom. The characteristic time scale of the atomic response is the dipole…
The bulk photovoltaic effect is an example of a non-linear optical response that leads to a DC current that is relevant for photo-voltaic applications. In this work, we theoretically study this effect in the presence of electron-phonon…
Nonlinear phenomena are inherent in most systems in nature. Second or higher-order harmonic generations, three-wave and four-wave mixing are typical phenomena in nonlinear optics. To obtain a nonzero signal for second-harmonic generation in…
We derive general formulas for photon and dilepton production rates from an arbitrary non-equilibrated medium from first principles in quantum field theory. At lowest order in the electromagnetic coupling constant, these relate the rates to…
We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier…
For light in a single temporal mode, the time dependence is associated entirely with the deterministic pulse shape rather than the quantum state. This means the second order coherence of light can no longer be understood as the temporal…
Nonlinear responses in crystalline solids are attracting a great deal of attention because of exciting phenomena, such as the bulk photovoltaic effect in noncentrosymmetric crystals and the third harmonic generation related to Higgs modes…