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The resonant inelastic x-ray scattering spectrum in insulating cuprates is examined by using the exact diagonalization technique on small clusters in the two-dimensional Hubbard model with second and third neighbor hopping terms. When the…

Strongly Correlated Electrons · Physics 2009-10-31 K. Tsutsui , T. Tohyama , S. Maekawa

The electronic structure of Mott insulators continues to be a major unsolved problem in physics despite more than half-century of intense research efforts. Well-developed momentum-resolved spectroscopies such as photoemission or neutron…

Strongly Correlated Electrons · Physics 2009-11-07 M. Z. Hasan , E. D. Isaacs , Z-X. Shen , L. L. Miller , K. Tsutsui , T. Tohyama , S. Maekawa

We report a Cu K-edge resonant inelastic x-ray scattering (RIXS) study of high-Tc cuprates. Momentum-resolved charge excitations in the CuO2 plane are examined from parent Mott insulators to carrier-doped superconductors. The Mott gap…

We report momentum resolved charge excitations in a one dimensional (1-D) Mott insulator studied using high resolution (~ 325 meV) inelastic x-ray scattering over the entire Brillouin zone for the first time. Excitations at the insulating…

Strongly Correlated Electrons · Physics 2007-05-23 M. Z. Hasan , P. A. Montano , E. D. Isaacs , Z-X. Shen , H. Eisaki , S. K. Sinha , Z. Islam , N. Motoyama , S. Uchida

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

Strongly Correlated Electrons · Physics 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

We report the first measurement of collective charge modes of insulating Sr14Cu24O41 using inelastic resonant x-ray scattering over the complete Brillouin zone. Our results show that the intense excitation modes at the charge gap edge…

Strongly Correlated Electrons · Physics 2008-01-10 L. Wray , D. Qian , D. Hsieh , Y. Xia , H. Eisaki , M. Z. Hasan

We theoretically examine the momentum dependence of resonant inelastic x-ray scattering (RIXS) spectrum for one-dimensional and two-dimensional cuprates based on the single-band Hubbard model with realistic parameter values. The spectrum is…

Strongly Correlated Electrons · Physics 2007-05-23 T. Tohyama , K. Tsutsui , S. Maekawa

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

Collective excitations contain rich information about photoinduced transient states in correlated systems. In a Mott insulator, charge degrees of freedom are frozen, but can be activated by photodoping. The energy-momentum distribution of…

Strongly Correlated Electrons · Physics 2020-04-23 Yao Wang , Yuan Chen , Chunjing Jia , Brian Moritz , Thomas P. Devereaux

The recent development of x-ray scattering techniques revealed the charge-excitation spectrum in high-$T_c$ cuprate superconductors. While the presence of a dispersive signal in the high-energy charge-excitation spectrum is well accepted in…

Superconductivity · Physics 2019-01-09 Andrés Greco , Hiroyuki Yamase , Matías Bejas

Predictions are made for the momentum- and carrier-dependent degradation of the Mott gap upon doping in high-Tc cuprates as would be observed in Cu K-edge resonant inelastic x-ray scattering (RIXS). The two-dimensional Hubbard model with…

Strongly Correlated Electrons · Physics 2009-11-10 K. Tsutsui , T. Tohyama , S. Maekawa

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to…

Superconductivity · Physics 2015-06-15 S. Wakimoto , K. Ishii , H. Kimura , K. Ikeuchi , M. Yoshida , T. Adachi , D. Casa , M. Fujita , Y. Fukunaga , T. Gog , Y. Koike , J. Mizuki , K. Yamada

Momentum dependent charge excitations of a two-leg ladder are investigated by resonant inelastic x-ray scattering of (La,Sr,Ca)14Cu24O41. In contrast to the case of a square lattice, momentum dependence of the Mott gap excitation of the…

Strongly Correlated Electrons · Physics 2007-08-02 K. Ishii , K. Tsutsui , T. Tohyama , T. Inami , J. Mizuki , Y. Murakami , Y. Endoh , S. Maekawa , K. Kudo , Y. Koike , K. Kumagai

We calculate the inelastic light scattering from X-rays, which allows the photon to transfer both energy and momentum to the strongly correlated charge excitations. We find that the charge transfer peak and the low energy peak both broaden…

Strongly Correlated Electrons · Physics 2009-11-07 T. P. Devereaux , G. E. D. McCormack , J. K. Freericks

We investigate electronic excitations in La2-x(Br,Sr)xCuO4 using resonant inelastic x-ray scattering (RIXS) at the oxygen K edge. RIXS spectra of the hole-doped cuprates show clear momentum dependence below 1 eV. The spectral weight…

Strongly Correlated Electrons · Physics 2017-09-26 K. Ishii , T. Tohyama , S. Asano , K. Sato , M. Fujita , S. Wakimoto , K. Tustsui , S. Sota , J. Miyawaki , H. Niwa , Y. Harada , J. Pelliciari , Y. Huang , T. Schmitt , Y. Yamamoto , J. Mizuki

We investigate the problem of inelastic x-ray scattering in the spin$-{1/2}$ Heisenberg model on the square lattice. We first derive a momentum dependent scattering operator for the $A_{1g}$ and $B_{1g}$ polarization geometries. On the…

Strongly Correlated Electrons · Physics 2009-11-13 F. H. Vernay , M. J. P. Gingras , T. P. Devereaux

Recent experiments on inelastic light scattering in a number of insulating cuprates [1] revealed a new excitation appearing in the case of crossed polarizations just below the optical absorption threshold. This observation suggests that…

Condensed Matter · Physics 2009-10-22 D. V. Khveshchenko , P. B. Wiegmann

Resonant inelastic x-ray scattering (RIXS) tuned for the Cu L edge is a possible tool to detect charge excitations in cuprate superconductors. We theoretically investigate the possibility for observing a collective charge excitation by the…

Strongly Correlated Electrons · Physics 2015-08-03 Takami Tohyama , Kenji Tsutsui , Michiyasu Mori , Shigetoshi Sota , Seiji Yunoki

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

Momentum-resolved resonant inelastic x-ray scattering (RIXS) spectroscopy has been carried out at the Fe K edge, successfully for the first time. The RIXS spectra of a FeBO3 single crystal reveal a wealth of information on 1-10 eV…

Strongly Correlated Electrons · Physics 2015-05-14 Jungho Kim , Yuri Shvyd'ko
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