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It is well known that conventional harmonic lattice dynamics cannot be applied to energetically unstable crystals at 0 K, such as high temperature body centered cubic (BCC) phase of crystalline Zr. Predicting phonon spectra at finite…

Materials Science · Physics 2019-01-02 Xin Qian , Ronggui Yang

The electronic behavior of various solid metals (Al, Ni, Cu, Au, Ti, and W) under ultrashort laser irradiation is investigated by means of density functional theory. Successive stages of extreme nonequilibrium on picosecond time scale…

Materials Science · Physics 2014-04-04 Emile Bévillon , Jean-Philippe Colombier , Vanina Recoules , Razvan Stoian

We report an experimental and theoretical investigation of the lattice dynamics and thermal properties of the actinide dioxide NpO$_2$. The energy-wavevector dispersion relation for normal modes of vibration propagating along the $[001]$,…

We report on the dynamics of coherent phonons in semimetal 1T'-MoTe2 using femtosecond pump-probe spectroscopy. On an ultrafast sub-picosecond time scale at room temperature, a low frequency and long-lifetime shear phonon mode was observed…

Materials Science · Physics 2020-03-09 T. Fukuda , K. Makino , Y. Saito , P. Fons , A. V. Kolobov , K. Ueno , M. Hase

We present numerical simulations of the acoustic-phonon-limited mobility, $\mu_{ac}$, and phonon-drag thermopower, $S^{g}$, in two-dimensional electron gases confined in MgZnO/ZnO heterostructures. The calculations are based on the…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Margarita Tsaousidou

We investigate shock-compressed copper in the warm dense matter regime by means of density functional theory molecular dynamics simulations. We use neural-network-driven interatomic potentials to increase the size of the simulation box and…

Other Condensed Matter · Physics 2022-12-07 Maximilian Schörner , Bastian B. L. Witte , Andrew D. Baczewski , Attila Cangi , Ronald Redmer

Accurately modeling dense plasmas over wide ranging conditions of pressure and temperature is a grand challenge critically important to our understanding of stellar and planetary physics as well as inertial confinement fusion. In this work,…

First-principles investigation within the density functional theory is utilized to explore the physical properties of a superconducting topological semimetal Sn4Au under pressure within the range of 0-5 GPa. According to the computed…

Materials Science · Physics 2024-08-15 M. Abdul Hadi Shah , M. I. Naher , S. H. Naqib

This paper studies thermal transport in nanoporous silicon with a significant specific surface area. First, the equilibrium molecular dynamics approach was used to obtain the dependence of thermal conductivity on a specific surface area.…

Mesoscale and Nanoscale Physics · Physics 2023-05-15 Mykola Isaiev , Yuliia Mankovska , Vasyl Kuryliuk , David Lacroix

We present a phenomenological force-constant model developed for the description of lattice dynamics of sp2 hybridized carbon networks. Within this model approach, we introduce a new set of parameters to calculate the phonon dispersion of…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Zimmermann , P. Pavone , G. Cuniberti

The thermal properties of silver are calculated within the quasi-harmonic approximation, by using phonon dispersions from density-functional perturbation theory, and the pseudopotential plane-wave method. The resulting free energy provides…

Materials Science · Physics 2009-10-31 Jianjun Xie , Stefano de Gironcoli , Stefano Baroni , Matthias Scheffler

We present here a theoretical method to determine the phononic contribution to the thermal conductance of nanoscale systems in the phase-coherent regime. Our approach makes use of classical molecular dynamics (MD) simulations to calculate…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Fabian Müller , Peter Nielaba , Juan Carlos Cuevas , Fabian Pauly

The phonon-assisted sticking rate of slow moving atoms impinging on an elastic membrane at nonzero temperature is studied analytically using a model with linear atom-phonon interactions, valid in the weak coupling regime. A perturbative…

Mesoscale and Nanoscale Physics · Physics 2017-12-06 Dennis P. Clougherty

Using ab initio method we have studied the structural, elastic, electronic, optical and thermodynamic properties of AlB2 and TaB2. We have used plane wave pseudopotential with generalised gradient approximation as implemented in CASTEP…

Materials Science · Physics 2015-05-26 N. Jahan , M. A. Ali

Using a large scale molecular dynamics computer simulation we investigate the dynamics of a supercooled melt of SiO_2. We find that with increasing temperature the temperature dependence of the diffusion constants crosses over from an…

Statistical Mechanics · Physics 2009-10-31 Walter Kob , Jurgen Horbach , Kurt Binder

Using molecular dynamics (MD) with classical interaction potentials we present calculations of thermal conductivity and heat transport in crystals and glasses. Inducing shock waves and heat pulses into the systems we study the spreading of…

Materials Science · Physics 2009-10-31 C. Oligschleger , J. C. Sch"on

Understanding ballistic phonon transport effects in transient thermoreflectance experiments and explaining the observed deviations from classical theory remains a challenge. Diffusion equations are simple and computationally efficient but…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Jesse Maassen , Mark Lundstrom

We report an ab initio molecular dynamics simulation study of several static and dynamic properties of the liquid 3d transition metals. The calculated static structure factors show qualitative agreement with the available experimental data,…

Soft Condensed Matter · Physics 2020-05-27 B. G. del Rio , C. Pascual , O. Rodriguez , L. E. González , D. J. González

Density functional molecular dynamics simulations have been carried out to understand the finite temperature behavior of Au$_{19}$ and Au$_{20}$ clusters. Au$_{20}$ has been reported to be a unique molecule having tetrahedral geometry, a…

Statistical Mechanics · Physics 2016-09-28 Sailaja Krishnamurty , Ghazal Shafai , D. G. Kanhere , B. Soulé de Bas , M. J. Ford

We study the bonding and diffusion of Au in graphene vacancies using density-functional theory. Energetics show that Au adsorbs preferably to double vacancies, steadily in-plane with graphene. All diffusion barriers for the complex of Au in…

Materials Science · Physics 2009-02-16 S. Malola , H. Häkkinen , P. Koskinen