Related papers: Electron and Nuclear Spin Dynamics in Antiferromag…
We study theoretically the thermodynamic properties and spin dynamics of a class of magnetic rings closely related to ferric wheels, antiferromagnetic ring systems, in which one of the Fe (III) ions has been replaced by a dopant ion to…
We present detailed calculations of low-energy spin dynamics in the ``ferric wheel'' systems Na:Fe_6 and Cs:Fe_8 in a magnetic field. We compute by exact diagonalisation the low-energy spectra and matrix elements for total-spin and…
The Li-centered "ferric wheel" molecules with six oxo-bridged iron atoms form molecular crystals. We probed their electronic structure by X-ray photoelectron (XPS) and soft X-ray emission spectroscopy (XES), having calculated in parallel…
We consider fluctuations of the electronic spin due to coupling to nuclear spin. Noise spectroscopy of an electronic spin can be revealed in the Scanning Tunnelling Microscope (STM). We argue that the noise spectroscopy of electronic spin…
From inelastic neutron scattering experiments, we demonstrate quantum tunneling of the Neel vector in the antiferromagnetic molecular ferric wheel CsFe8. Analysis of the linewidth of the tunneling transition evidences coherent tunneling.
We present the appearance of negative differential resistance (NDR) in spin-dependent electron transport through a few-atom spin-chain. A chain of three antiferromagnetically coupled Fe atoms(Fe trimer) was positioned on a Cu2N/Cu(100)…
Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…
Coherent control of individual molecular spins in nano-devices is a pivotal prerequisite for fulfilling the potential promised by molecular spintronics. By applying electric field pulses during time-resolved electron spin resonance…
The antiferromagnetic molecular wheel Fe18 of eighteen exchange-coupled Fe(III) ions has been studied by measurements of the magnetic torque, the magnetization, and the inelastic neutron scattering spectra. The combined data show that the…
The spin correlations \omega^z_r, r=1,2,3, and the probability p_N$ of finding a system in the Neel state for the antiferromagnetic ring Fe(III)6 (the so-called `small ferric wheel') are calculated. States with magnetization M=0, total spin…
Spin dynamics is considered in ferromagnets consisting of electron and nuclear subsystems interacting with each other through hyperfine forces. In addition, the ferromagnetic sample is coupled with a resonance electric circuit. Under these…
The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…
The electron-nuclear hyperfine interaction shows up in a variety of phenomena including e.g. NMR studies of correlated states and spin decoherence effects in quantum dots. Here we focus on the hyperfine coupling and the NMR spin relaxation…
The one-dimensional homonuclear periodic array of nuclear spins I = 1/2, owing to hyperfine interaction of nuclear spins with electronic magnetic moments in antiferromagnetic structure, is considered. The neighbor nuclear spins in such…
Nonlinear spin motion in ferromagnets is considered with nonlinearity due to three factors: (i) the sample is prepared in a strongly nonequilibrium state, so that evolution equations cannot be linearized as would be admissible for spin…
Molecular nanomagnets are among the first examples of spin systems of finite size and have been test-beds for addressing a range of elusive but important phenomena in quantum dynamics. In fact, for short-enough timescales the spin…
The interaction between electronic and nuclear spins in the presence of external magnetic fields can be described by a spin Hamiltonian, with parameters obtained from first principles, electronic structure calculations. We describe an…
We develop a theory for spin transported by coherent Neel dynamics through an antiferromagnetic insulator coupled to a ferromagnetic insulator on one side and a current-carrying normal metal with strong spin-orbit coupling on the other. The…
The detailed theoretical understanding of quantum spin dynamics in various molecular magnets is an important step on the roadway to technological applications of these systems. Quantum effects in both ferromagnetic and antiferromagnetic…
High-frequency electron paramagnetic resonance (EPR) studies of the antiferromagnetic Mn-$[3\times 3]$ molecular grid clearly reveal a breaking of the $\Delta S = 0$ selection rule, providing direct evidence for the mixing of spin…