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The distance-resolved effective interaction between two star polymers in a good solvent is calculated by Molecular Dynamics computer simulations. The results are compared with a pair potential proposed recently by Likos et al. [Phys. Rev.…

Soft Condensed Matter · Physics 2009-10-31 A. Jusufi , M. Watzlawek , H. Loewen

We derive the short distance interaction of star polymers in a colloidal solution. We calculate the corresponding force between two stars with arbitrary numbers of legs f_1 and f_2. We show that a simple scaling theory originally derived…

By employing monomer-resolved computer simulations and analytical considerations based on polymer scaling theory, we analyze the conformations and interactions of multiarm star polymers strongly adsorbed on a smooth, two-dimensional plane.…

Soft Condensed Matter · Physics 2015-06-15 S. A. Egorov , J. Paturej , C. N. Likos , A. Milchev

We consider a coarse-grained (CG) model with pairwise interactions, suitable to describe low-density solutions of star-branched polymers of functionality $f$. Each macromolecule is represented by a CG molecule with $(f+1)$ interaction…

Soft Condensed Matter · Physics 2017-08-02 Roberto Menichetti , Andrea Pelissetto , Ferdinando Randisi

We analyze the effect of polydispersity in the arm number on the effective interactions, structural correlations and the phase behavior of star polymers in a good solvent. The effective interaction potential between two star polymers with…

Soft Condensed Matter · Physics 2009-10-31 Christian von Ferber , Arben Jusufi , Martin Watzlawek , Christos N. Likos , Hartmut Lowen

Understanding the dynamics of soft colloids, such as star polymers, dendrimers, and microgels, is of scientific and practical importance. It is known that the excluded volume effect plays a key role in colloidal dynamics. Here, we propose a…

Soft Condensed Matter · Physics 2019-09-17 Zhe Wang , Antonio Faraone , Panchao Yin , Lionel Porcar , Yun Liu , Changwoo Do , Kunlun Hong , Wei-Ren Chen

Simulations and Mode-Coupling Theory calculations, for a large range of the arm number $f$ and packing fraction $\eta$ have shown that the structural arrest and the dynamics of star polymers in a good solvent are extremely rich: the systems…

Soft Condensed Matter · Physics 2009-11-10 F. Lo Verso , L. Reatto , G. Foffi , P. Tartaglia , K. A. Dawson

We analyze the effective triplet interactions between the centers of star polymers in a good solvent. Using an analytical short distance expansion inspired by scaling theory, we deduce that the triplet part of the three-star force is…

Soft Condensed Matter · Physics 2015-06-24 Christian von Ferber , Arben Jusufi , Christos N. Likos , Hartmut Lowen , Martin Watzlawek

The phase diagram of star polymer solutions in a good solvent is obtained over a wide range of densities and arm numbers by Monte Carlo simulations. The effective interaction between the stars is modeled by an ultrasoft pair potential which…

Soft Condensed Matter · Physics 2009-10-31 M. Watzlawek , C. N. Likos , H. Loewen

PEP-PEO block copolymer micelles offer the possibility to investigate phase behaviour and interactions of star polymers (ultra-soft colloids). A star-like architecture is achieved by an extremely asymmetric block ratio (1:20). Micellar…

Soft Condensed Matter · Physics 2009-11-11 M. Laurati , J. Stellbrink , R. Lund , L. Willner , D. Richter , E. Zaccarelli

In this work, we consider a semi-dilute solution of identical star-polymers, made of attached flexible long polymer chains of the same polymerization degree N. We first compute the effective pair-potential between star-polymers. Such a…

Soft Condensed Matter · Physics 2007-05-23 F. Benzouine , M. Yassine , A. Derouiche , A. Bettachy , M. Benhamou

Star-like microgels have recently emerged as a promising class of thermoresponsive soft colloids, that have an internal architecture similar to that of star polymers. Here, we perform extensive monomer-resolved simulations to theoretically…

Soft Condensed Matter · Physics 2026-04-29 Tommaso Papetti , Elisa Ballin , Francesco Brasili , Emanuela Zaccarelli

We report on the linear viscoelastic properties of mixtures comprising multiarm star (as model soft colloids) and long linear chain homopolymers in a good solvent. In contrast to earlier works, we investigated symmetric mixtures (with a…

Soft Condensed Matter · Physics 2020-07-01 Daniele Parisi , Domenico Truzzolillo , Vishnu D. Deepak , Mario Gauthier , Dimitris Vlassopoulos

Star polymer undergoes a transformation from a group of loosely coupled chains at low number of arms to a dense hairy colloid at their high number. This change affects solubility, aggregation and rheological behavior and is of much…

Soft Condensed Matter · Physics 2019-06-20 Ostap Kalyuzhnyi , Khristine Haidukivska , Viktoria Blavatska , Jaroslav Ilnytskyi

We study numerically the effective pair potential between star polymers with equal arm lengths and equal number $f$ of arms. The simulations were done for the soft core Domb-Joyce model on the simple cubic lattice, to minimize corrections…

Soft Condensed Matter · Physics 2009-11-10 Hsiao-Ping Hsu , Peter Grassberger

The surface tension of interacting polymers in a good solvent is calculated theoretically and by computer simulations for a planar wall geometry and for the insertion of a single colloidal hard-sphere. This is achieved for the planar wall…

Soft Condensed Matter · Physics 2016-08-31 A. A. Louis , P. G. Bolhuis , E. J. Meijer , J. P. Hansen

The structural and dynamical properties of ultra-soft colloids - star polymers - exposed to a uniform external force field are analyzed applying the multiparticle collision dynamics approach, a hybrid coarse-grain mesoscale simulation…

Soft Condensed Matter · Physics 2018-03-09 Sunil P. Singh , Gerhard Gompper , Roland G. Winkler

We derive effective interaction potentials between hard, spherical colloidal particles and star-branched polyelectrolytes of various functionalities and smaller size than the colloids. The effective interactions are based on a…

Soft Condensed Matter · Physics 2007-05-23 M. Konieczny , C. N. Likos

We consider a model of star copolymers, based on self-avoiding walks, where the arms of the star can be chemically distinct. The copolymeric star is attached to an impenetrable surface at a vertex of unit degree and the different monomers…

Statistical Mechanics · Physics 2022-06-22 EJ Janse van Rensburg , SG Whittington

Polymeric films with greater impact and ballistic resistance are highly desired for numerous applications, but molecular configurations that best address this need remain subject to debate. We study the resistance to ballistic impact of…

Soft Condensed Matter · Physics 2020-09-28 Andrea Giuntoli , Nitin K. Hansoge , Sinan Keten
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