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We investigate the frustrated magnetic interactions in cubic transition metal oxides with orbital degeneracy. The $e_g$ orbitals order easier and their ordering explains the $A$-type antiferromagnetic phase in KCuF$_3$ and LaMnO$_3$. In…

Strongly Correlated Electrons · Physics 2016-08-31 Andrzej M. Oles

Evolution of composite spin-orbital order and coupled spin-orbital excitations is studied in a variety of $d^4$ systems with $n$=$4$ electrons in the $t_{2g}$ orbital sector using the generalised self-consistent + fluctuations approach for…

Strongly Correlated Electrons · Physics 2025-04-30 Shahid Ahmad , Harshvardhan Parmar , Shubhajyoti Mohapatra , Avinash Singh

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

Strongly Correlated Electrons · Physics 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

We study the effective spin-orbital model derived for the d9 ions in a three-dimensional perovskite lattice, as in KCuF_3, where at each site the doubly degenerate eg orbitals contain a single hole. The model describes the superexchange…

Strongly Correlated Electrons · Physics 2009-10-31 Andrzej M. Oles , Louis Felix Feiner , Jan Zaanen

Basic mechanisms controlling orbital order and orbital fluctuations in transition metal oxides are discussed. The lattice driven classical orbital picture, e.g. like in manganites LaMnO$_3$, is contrasted to the quantum behavior of orbitals…

Strongly Correlated Electrons · Physics 2009-11-11 Giniyat Khaliullin

The interactions between charge and orbitally ordered $d$-electrons are important in many transition metal oxides. We propose an effective energy model for such interactions, parameterized with DFT+U calculations, so that energy…

Strongly Correlated Electrons · Physics 2015-11-17 Fei Zhou , Gerbrand Ceder

We summarize some characteristic features of the frustrated magnetic interactions in spin-orbital models adequate for cubic transition metal oxides with orbital degeneracy. A generic tendency towards dimerization, found already in the…

Strongly Correlated Electrons · Physics 2015-06-24 Andrzej M. Oles

The exchange interactions and magnetic structure in layered system CuMnO2 (mineral crednerite) and in nonstoichiometric system Cu1.04Mn0.96O2, with triangular layers distorted due to orbital ordering of the Mn3+ ions, are studied by…

Strongly Correlated Electrons · Physics 2014-01-21 A. V. Ushakov , S. V. Streltsov , D. I. Khomskii

The magnetic excitations of the iron pnictides are explained within a degenerate double-exchange model. The local-moment spins are coupled by superexchanges $J_1$ and $J_2$ between nearest and next-nearest neighbors, respectively, and…

Strongly Correlated Electrons · Physics 2015-05-18 Weicheng Lv , Frank Krüger , Philip Phillips

The magnetic and orbital orders for the bilayer manganites in the doping region $0.5 < x <1.0$ have been investigated from a model that incorporates the two $e_g$ orbitals at each Mn site, the inter-orbital Coulomb interaction and lattice…

Strongly Correlated Electrons · Physics 2009-11-10 Tulika Maitra , A. Taraphder

The magnon dispersion in the charge, orbital and spin ordered phase in La(0.5)Sr(1.5)MnO(4) has been studied by means of inelastic neutron scattering. We find an excellent agreement with a magnetic interaction model basing on the CE-type…

Strongly Correlated Electrons · Physics 2009-11-11 D. Senff , F. Krueger , S. Scheidl , M. Benomar , Y. Sidis , F. Demmel , M. Braden

Spin-charge-orbital ordered structures in doped layered manganites are investigated using an orbital-degenerate double-exchange model tightly coupled to Jahn-Teller distortions. In the ferromagnetic phase, unexpected diagonal stripes at…

Strongly Correlated Electrons · Physics 2009-10-31 Takashi Hotta , Adrian Feiguin , Elbio Dagotto

A short introduction to the complex phenomena encountered in transition metal oxides with either charge or orbital or joint charge-and-orbital order, usually accompanied by magnetic order, is presented. It is argued that all the types of…

Strongly Correlated Electrons · Physics 2022-01-27 Andrzej M. Oles

We consider a model of strongly correlated $e_g$ electrons interacting by superexchange orbital interactions in the ferromagnetic phase of LaMnO$_3$. It is found that the classical orbital order with alternating occupied $e_g$ orbitals has…

Strongly Correlated Electrons · Physics 2009-10-31 Jeroen van den Brink , Peter Horsch , Frank Mack , Andrzej M. Oles

We derive a spin-orbital model for insulating LaMnO_3 which fulfills the SU(2) symmetry of S=2 spins at Mn^{3+} ions. It includes the complete e_g and t_{2g} superexchange which follows from a realistic Mn^{2+} multiplet structure in cubic…

Strongly Correlated Electrons · Physics 2009-10-31 Louis Felix Feiner , Andrzej M. Oles

The two-orbital double-exchange model is employed for the study of the magnetic and orbital orders in ($R$MnO$_3$)$_n$/($A$MnO$_3$)$_{2n}$ ($R$: rare earths; $A$: alkaline earths) superlattices. The A-type antiferromagnetic order is…

Strongly Correlated Electrons · Physics 2012-12-11 Shuai Dong , Qinfang Zhang , Seiji Yunoki , J. -M. Liu , Elbio Dagotto

We report the magnetic properties of $A$-site spinel compound MnSc$_2$Se$_4$. The macroscopic magnetic measurements uncovers successive magnetic transitions at $T_{\rm{N1}}$= 2.04 K, followed by two further transitions at $T_{\rm{N2}}$=1.8…

Strongly Correlated Electrons · Physics 2022-06-01 K. Guratinder , V. Tsurkan , L. Prodan , L. Keller , J. P. Embs , F. Juranyi , M. Medarde , Ch. Rüegg , O. Zaharko

Mott insulators based on $4d$ and $5d$ transition-metal ions, where spin-orbit interaction plays a key role, can exhibit various forms of unusual magnetism. A particular example is the antiferromagnet Ca$_2$RuO$_4$ containing $d^4$…

Strongly Correlated Electrons · Physics 2025-05-16 Jan Revenda , Krzysztof Wohlfeld , Jiří Chaloupka

We study theoretically the phase diagram of the double-layered perovskite manganites taking into account the orbital degeneracy, the strong Coulombic repulsion, and the coupling with the lattice deformation. Observed spin structural changes…

Strongly Correlated Electrons · Physics 2009-10-31 Ryo Maezono , Naoto Nagaosa

We review some aspects related to orbital degrees of freedom in manganites. The Mn$^{3+}$ ions in these compounds have double orbital degeneracy and are strong Jahn-Teller ions, causing structural distortions and orbital ordering. We…

Strongly Correlated Electrons · Physics 2007-05-23 Jeroen van den Brink , Giniyat Khaliullin , Daniel Khomskii
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