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The osmotic coefficient of B-DNA in water may, in moderately dilute solutions, deviate as much as 100 % from predictions based on a simple 'counterion condensation' theory. We determine the results for osmotic properties via a cell model…

Soft Condensed Matter · Physics 2019-05-15 Per Lyngs Hansen , Rudi Podgornik , V. Adrian Parsegian

Electrostatics plays a key role in biomolecular assembly. Oppositely charged biomolecules, for instance, can co-assembled into functional units, such as DNA and histone proteins into nucleosomes and actin-binding protein complexes into…

Materials Science · Physics 2009-11-11 Y. S. Velichko , M. Olvera de la Cruz

Based on a reconsideration of the Gibbs paradox, we show that a residual, non-extensive term in entropy turns up upon mixing identical particles, whether they are indistinguishable or not. The positive contribution from this residual…

Soft Condensed Matter · Physics 2012-01-04 Chi-Lun Lee , Yiing-Rei Chen

Structuring of DNA counterions around the double helix has been studied by the molecular dynamics method. A DNA dodecamer d(CGCGAATTCGCG) in water solution with the alkali metal counterions Na$^{+}$, K$^{+}$, and Cs$^{+}$ has been…

Biomolecules · Quantitative Biology 2015-03-19 O. O. Liubysh , A. V. Vlasiuk , S. M. Perepelytsya

A theory is presented for the effective charge of colloidal particles in suspensions containing multivalent counterions. It is shown that if colloids are sufficiently strongly charged, the number of condensed multivalent counterion can…

Soft Condensed Matter · Physics 2009-11-11 S. Pianegonda , Marcia C. Barbosa , Yan Levin

Aggregation of two oppositely charged colloids in salty water is studied. We focus on the role of Coulomb interaction in strongly asymmetric systems in which the charge and size of one colloid is much larger than the other one. In the…

Soft Condensed Matter · Physics 2009-11-10 R. Zhang , B. I. Shklovskii

We consider the effect of strong electron-electron attraction on superconductivity in the dilute system of the negative U-centers. They couple to the conducting electronic states and mediate attraction between electrons. We predict the…

Superconductivity · Physics 2020-12-24 Alexander Yu. Zyuzin

We explore, using the recently developed efficient Monte Carlo simulation method, the interaction of an anionic polyelectrolyte solution with a like-charged dielectric surface. In addition to polyions, the solution also contains salt with…

Soft Condensed Matter · Physics 2018-01-12 Alexandre P. dos Santos , Matheus Girotto , Yan Levin

A nonlinear response theory is developed and applied to electrostatic interactions between spherical macroions, screened by surrounding microions, in charge-stabilized colloidal suspensions. The theory describes leading-order nonlinear…

Soft Condensed Matter · Physics 2009-11-10 A. R. Denton

The nature of electrostatic interaction between like-charged particles at water-air interface is analyzed in this paper. We show that long-ranged electrostatic dipolar attraction between these objects generally exists. Our result provides a…

Soft Condensed Matter · Physics 2007-05-23 Yi Zhou , Tai-Kai Ng

The free energy of ion solvation can be decomposed into enthalpic and entropic contributions. This helps to understand the connection between the dielectric properties and the underlying forces. We present a simple linear-response model of…

Soft Condensed Matter · Physics 2024-06-24 Alec Wills , Anthony Mannino , Isidro Losada , Sara G. Mayo , Jose M. Soler , Marivi Fernandez-Serra

Adsorption of multivalent counterions on the charged surface of a macroion is known to lead to inversion of the macroion charge due to the strong lateral correlations of counterions. We consider a nontrivial role of the excluded volume of…

Soft Condensed Matter · Physics 2009-11-07 Toan T. Nguyen , Boris I. Shklovskii

The structure of polyelectrolytes is highly sensitive to small changes in the interactions between its monomers. In particular, interactions mediated by counterions play a significant role, and are affected by both specific molecular…

Soft Condensed Matter · Physics 2020-02-03 Pauline Bacle , Marie Jardat , Virginie Marry , Guillaume Mériguet , Guillaume Batôt , Vincent Dahirel

Electronic charge carriers in ionic materials can self-trap to form large polarons. Interference between the ionic displacements associated with oppositely charged large polarons increases as they approach one another. Initially this…

Other Condensed Matter · Physics 2018-02-05 David Emin

Bending rigidity of a charged membrane or a charged polyelectrolyte screened by monovalent counterions is known to be enhanced by electrostatic effects. We show that in the case of screening by multivalent counterions the electrostatic…

Soft Condensed Matter · Physics 2009-10-31 T. T. Nguyen , I. Rouzina , B. I. Shklovskii

We examine the force between two charged surfaces immersed in aqueous mixtures having a coexistence curve. For a homogeneous water-poor phase, as the distance between the surfaces is decreased, a water-rich phase condenses at a distance…

Statistical Mechanics · Physics 2015-05-27 Sela Samin , Yoav Tsori

Global transverse-momentum conservation induces correlations between any number of particles, which contribute in particular to the two- and three-particle correlations measured in heavy-ion collisions. These correlations are examined in…

Nuclear Theory · Physics 2008-11-26 Nicolas Borghini

When an ionic liquid adsorbs onto a porous electrode, its ionic arrangement is deeply modified due to a screening of the Coulombic interactions by the metallic surface and by the confinement imposed upon it by the electrode's morphology. In…

We study macroion correlation effects on the thermodynamics of highly charged colloidal suspensions using a mean-field theory and primitive model computer simulations. We suggest a simple way to include the macroion correlations into the…

Soft Condensed Matter · Physics 2009-11-11 Ramon Castaneda-Priego , Luis F. Rojas-Ochoa , Vladimir Lobaskin , J. C. Mixteco-Sanchez

The dynamical response of a tethered semiflexible polymer with self-attractive interactions and subjected to an external force field is numerically investigated by varying stiffness and self-interaction strength. The chain is confined in…

Soft Condensed Matter · Physics 2022-11-09 A. Lamura
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