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We study the vicinal surface with adsorption below the roughening temperature, using the restricted solid-on-solid model coupled with the Ising model. We calculate the step tension $\gamma$ and the step-interaction coefficient $B$ by…

Statistical Mechanics · Physics 2007-05-23 Noriko Akutsu , Yasuhiro Akutsu , Takao Yamamoto

We study the vicinal surface of the restricted solid-on-solid model coupled with the Langmuir adsorbates which we regard as two-dimensional lattice gas without lateral interaction. The effect of the vapor pressure of the adsorbates in the…

Statistical Mechanics · Physics 2009-11-07 Noriko Akutsu , Yasuhiro Akutsu , Takao Yamamoto

The wetting properties of solid substrates with customary (i.e., macroscopic) random roughness are considered as a function of the microscopic contact angle of the wetting liquid and its partial pressure in the surrounding gas phase.…

Soft Condensed Matter · Physics 2015-03-19 S. Herminghaus

The wetting of solid surfaces by fluids is a problem of great practical importance that has been extensively studied over the years. Most often, the experimental work has involved measurements of the contact angle made by a liquid on the…

Statistical Mechanics · Physics 2007-05-23 S. Curtarolo , M. J. Bojan , G. Stan , M. W. Cole , W. A. Steele

Here we present a structural study of pentacene (Pn) thin films on vicinal Ag(111) surfaces by He atom diffraction measurements and density functional theory (DFT) calculations supplemented with van der Waals (vdW) interactions. Our He atom…

Strongly Correlated Electrons · Physics 2012-11-19 E. Mete , I. Demiroglu , E. Albayrak , G. Bracco , S. Ellialtioglu , M. F. Danisman

Using a Monte Carlo method on a lattice model of a vicinal surface with short-range step-step attraction, we show that, at low temperature and near equilibrium, there is an inhibition of the motion of macro-steps. This inhibition leads to a…

Chemical Physics · Physics 2017-11-15 Noriko Akutsu

We present a density-functional theory study addressing the on-surface adsorption of oxygen at the Pd(11N) (N =3,5,7) vicinal surfaces, which exhibit (111) steps and (100) terraces of increasing width. We find the binding to be…

Materials Science · Physics 2007-05-23 Yongsheng Zhang , Jutta Rogal , Karsten Reuter

Relaxed atomic geometries and chemisorption energies have been calculated for the dissociative adsorption of molecular hydrogen on vicinal Si(001) surfaces. We employ density-functional theory, together with a pseudopotential for Si, and…

Condensed Matter · Physics 2009-10-31 E. Pehlke , P. Kratzer

A sublimating vicinal crystal surface can undergo a step bunching instability when the attachment-detachment kinetics is asymmetric, in the sense of a normal Ehrlich-Schwoebel effect. Here we investigate this instability in a model that…

Statistical Mechanics · Physics 2015-05-18 Marian Ivanov , Vladislav Popkov , Joachim Krug

A discrete version of deposition-diffusion equations appropriate for description of step flow on a vicinal surface is analyzed for a two-dimensional grid of adsorption sites representing the stepped surface and explicitly incorporating…

Mesoscale and Nanoscale Physics · Physics 2016-04-11 R. Zhao , J. W. Evans , T. J. Oliveira

We use a density functional approach to calculate the contact angle of the water model on a heterogeneous, graphite-like surface. The surface heterogeneity results from the pre-adsorption of a layer of spherical species. The pre-adsorbed…

Soft Condensed Matter · Physics 2022-10-04 K. Dąbrowska , O. Pizio , S. Sokołowski

The coverage of vicinal, stepped surfaces with molecules is simulated with the help of a two-dimensional Ising model including local distortions and an Ehrlich-Schwoebel barrier term at the steps. An effective two-spin model is capable to…

Statistical Mechanics · Physics 2015-06-25 K. Morawetz , C. Olbrich , S. Gemming , M. Schreiber

We propose a self-consistent model taking into account variations in adsorption properties of the adsorbent surface in the process of adsorption--desorption of molecules of gas on it. We introduce a dimensionless coupling parameter that…

Materials Science · Physics 2009-11-30 A. S. Usenko

A simple solid-on-solid model, proposed earlier to describe overlayer-induced faceting of bcc(111) surface, is applied to faceting of spherical surfaces covered by adsorbate monolayer. Monte Carlo simulation results show that morphology of…

Soft Condensed Matter · Physics 2009-11-11 Daniel Niewieczerzal , Czeslaw Oleksy

We perform the analysis of predictions of a classical density functional theory for associating fluids with different association strength concerned with wetting of solid surfaces. The four associating sites water-like models with…

Soft Condensed Matter · Physics 2024-04-01 A. Kozina , M. Aguilar , O. Pizio , S. Sokołowski

With a Si(001) vicinal surface in mind, we study step wandering instability on a vicinal surface with an anisotropic surface diffusion whose orientation dependence alternates on each consecutive terrace. In a conserved system step wandering…

Materials Science · Physics 2013-05-29 M. Sato , M. Uwaha , Y. Saito , Y. Hirose

A solid-on-solid growth model for dimer adsorption and desorption is introduced and studied numerically. The special property of the model is that dimers can only desorb at the edges of terraces. It is shown that the model exhibits a…

Statistical Mechanics · Physics 2009-10-31 Haye Hinrichsen , Geza Odor

Close to a solid surface, the properties of a fluid deviate significantly from their bulk values. In this context, we study the surface adsorption profiles of a symmetric binary liquid confined to a slit pore by means of molecular dynamics…

Soft Condensed Matter · Physics 2025-01-15 Sutapa Roy , Felix Höfling

In this work we report studies of nitrogen adsorption and desorption onto solid surfaces using computer simulations of the three dimensional Ising model, for systems with complex porous structures at the mesoscopic and microscopic levels. A…

Soft Condensed Matter · Physics 2015-03-17 M. A. Balderas Altamirano , S. Cordero , G. Roman , A. Gama Goicochea

We examine the reversible adsorption of spherical solutes on a random site surface in which the adsorption sites are uniformly and randomly distributed on a substrate. Each site can be occupied by one solute provided that the nearest…

Soft Condensed Matter · Physics 2008-05-23 J. Talbot , G. Tarjus , P. Viot
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