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We investigate electronic transport through two types of conjugated molecules. Mechanically controlled break-junctions are used to couple thiol endgroups of single molecules to two gold electrodes. Current-voltage characteristics (IVs) of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Reichert , R. Ochs , D. Beckmann , H. B. Weber , M. Mayor , H. v. Loehneysen

We simulate bulk materials under strong currents by following in real-time the dynamics of the electrons under an electric field. By changing the intensity of the electric field, our method can model, for the first time, non-linear effects…

Materials Science · Physics 2017-02-03 Xavier Andrade , Sebastien Hamel , Alfredo A. Correa

We analyze changes of the electronic structure of a triangular molecule under the influence of an electric field (i.e., the Stark effect). The effects of the field are shown to be anisotropic and include both a linear and a nonlinear part.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Bogdan R. Bulka , Tomasz Kostyrko , Jakub Luczak

We propose a simple scheme that describes accurately essential non-equilibrium effects in nanoscale electronics devices using equilibrium transport theory. The scheme, which is based on the alignment and dealignment of the junction…

Mesoscale and Nanoscale Physics · Physics 2012-10-01 V. M. García-Suárez , J. Ferrer

Nonequilibrium quantum transport is of central importance in nanotechnology. Its description requires the understanding of strong electronic correlations, which couple atomic-scale phenomena to the nanoscale. So far, research in correlated…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 A. Erpenbeck , E. Gull , G. Cohen

We analyze the effect of electron-phonon coupling on the full counting statistics of a molecular junction beyond the lowest order perturbation theory. Our approach allows to take into account analytically the feedback between the…

Mesoscale and Nanoscale Physics · Physics 2010-10-14 D. F. Urban , R. Avriller , A. Levy Yeyati

A minimal model for coherent transport through a donor/acceptor molecular junction is presented. The two donor and acceptor sites are described by single levels energetically separated by an intramolecular tunnel barrier. In the limit of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Florian Pump , Gianaurelio Cuniberti

Electron transport through a single-level quantum dot weakly coupled to Luttinger liquid leads is considered in the master equation approach. It is shown that for a weak or moderately strong interaction the differential conductance…

Strongly Correlated Electrons · Physics 2013-02-06 G. A. Skorobagatko , I. V. Krive

We discuss the conductance of a molecular bridge between mesoscopic electrodes supporting low-dimensional transport and bearing an internal structure. As an example for such nanoelectrodes we assume semi-infinite (carbon) nanotubes. In the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 G. Fagas , G. Cuniberti , K. Richter

We derive a master equation for the electron transport through molecular wires in the limit of strong Coulomb repulsion. This approach is applied to two typical situations: First, we study transport through an open conduction channel for…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Franz J. Kaiser , Michael Strass , Sigmund Kohler , Peter Hänggi

Colloidal nanoparticles developed as interesting objects to establish two- or three-dimensional super-structures with properties not known from conventional bulk materials. Beyond, the properties can be tuned and quantum effects can be…

Materials Science · Physics 2017-10-30 Christian Klinke

A theoretical model of a single molecule coupled to many vibronic modes is presented. At low energies, transport is dominated by electron-vibron processes where transfer of an electron through the dot is accompanied by the…

Mesoscale and Nanoscale Physics · Physics 2011-08-19 Abdullah Yar , Andrea Donarini , Sonja Koller , Milena Grifoni

A theoretical model of a single molecule coupled to many vibronic modes is presented. At low energies, transport is dominated by electron-vibron processes where transfer of an electron through the dot is accompanied by the…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Abdullah Yar , Andrea Donarini , Sonja Koller , Milena Grifoni

We present an atomistic self-consistent study of the electronic and transport properties of semiconducting carbon nanotube in contact with metal electrodes of different work functions, which shows simultaneous electron and hole doping…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yongqiang Xue , Mark A. Ratner

It is demonstrated that non-equilibrium vibrational effects are enhanced in molecular devices for which the effective potential for vibrations is sensitive to the charge state of the device. We calculate the electron tunneling current…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Maarten R. Wegewijs , Katja C. Nowack

Weakly coupled molecular junctions are an active and important field of research as they exhibit various non-linear transport phenomena. We have investigated the carrier transport through weakly coupled B2C2N2H6 molecules using quantum…

Mesoscale and Nanoscale Physics · Physics 2020-03-09 Dibyajyoti Ghosh , Prakash Parida , Swapan K. Pati

We performed studies of coherent electronic transport through a single walled carbon nanotube. In the calculations multiple scattering on the contacts and interference processes were taken into account. Conductance is a composition of…

Materials Science · Physics 2016-08-31 W. Iwo Babiaczyk , Bogdan. R. Bulka

One of the ultimate goals of molecular electronics is to create technologies that will complement - and eventually supersede - Si-based microelectronics technologies. To reach this goal, electronic properties that mimic at least some of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-26 Bingqian Xu , Yonatan Dubi

We study charge and energy transfer in two-site molecular electronic junctions in which electron transport is assisted by a vibrational mode. To understand the role of mode harmonicity/anharmonicity on transport behavior, we consider two…

Mesoscale and Nanoscale Physics · Physics 2015-09-01 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal

We analyze the effect of a gate on the conductance of molecules by separately evaluating the gate-induced polarization and the potential shift of the molecule relative to the leads. The calculations use ab initio density functional theory…

Materials Science · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang