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Simulations of five different coarse-grained models of symmetric diblock copolymer melts are compared to demonstrate a universal (i.e., model-independent) dependence of the free energy on the invariant degree of polymerization…

Soft Condensed Matter · Physics 2015-06-18 Jens Glaser , Pavani Medapuram , Thomas M. Beardsley , Mark W. Matsen , David C. Morse

We study the microstructural glass transitions in diblock-copolymer melts using a thermodynamic replica approach. Our approach performs an expansion in terms of the natural smallness parameter -- the inverse of the scaled degree of…

Soft Condensed Matter · Physics 2009-11-11 C. -Z. Zhang , Z. -G. Wang

We present several ordering mechanisms in diblock copolymers. For temperatures above the order-disorder temperature and in the weak segregation regime, a linear response theory is presented which gives the polymer density in the vicinity of…

Soft Condensed Matter · Physics 2007-05-23 Yoav Tsori , David Andelman

We present a model addressing the orientation transition of symmetric block copolymers such as PS/PMMA on smooth and rough surfaces. The distortion free energy of parallel and perpendicular lamellar phases in contact with a rough solid…

Soft Condensed Matter · Physics 2012-01-31 Yoav Tsori , Easan Sivaniah , David Andelman , Takeji Hashimoto

We investigate the effect of chemically patterned surfaces on the morphology of diblock copolymers below the order-disorder transition. Profiles for lamellar phases in contact with one surface, or confined between two surfaces are obtained…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , David Andelman

We present results of temperature resolved scattering studies of a liquid crystalline block copolymer undergoing an order-disorder transition (ODT) in the presence of magnetic fields and time-resolved measurements during isothermal field…

Soft Condensed Matter · Physics 2013-03-06 Manesh Gopinadhan , Pawel W. Majewski , Youngwoo Choo , Chinedum O. Osuji

In this work we investigated the phase behavior of melts of block-copolymers with one charged block by means of dissipative particle dynamics with explicit electrostatic interactions. We assumed that all the Flory-Huggins \c{hi} parameters…

Soft Condensed Matter · Physics 2019-06-12 Alexey A. Gavrilov , Alexander V. Chertovich , Igor I. Potemkin

The Leibler weak segregation theory in molten diblock copolymers is generalized with due regard for the 2nd shell harmonics contributions defined in the paper and the phase diagrams are built for the linear and miktoarm ternary ABC triblock…

Soft Condensed Matter · Physics 2009-11-11 Igor Ya. Erukhimovich

We present numerical calculations of lamellar phases of block copolymers at patterned surfaces. We model symmetric di-block copolymer films forming lamellar phases and the effect of geometrical and chemical surface patterning on the…

Soft Condensed Matter · Physics 2016-02-18 Xingkun Man , David Andelman , Henri Orland

We present few ordering mechanisms in block copolymer melts in the coarse-graining approach. For chemically homogeneous or modulated confining surfaces, the surface ordering is investigated above and below the order-disorder temperature. In…

Soft Condensed Matter · Physics 2012-01-31 Yoav Tsori , David Andelman

The dynamics of microphase separation and the orientation of lamellae in diblock copolymers is investigated in terms of a mean-field model. The formation of lamellar structures and their stable states are explored and it is shown that…

Soft Condensed Matter · Physics 2015-06-15 Vanessa Weith , Alexei Krekhov , Walter Zimmermann

We study morphologies of thin-film diblock copolymers between two flat and parallel walls. The study is restricted to the weak segregation regime below the order-disorder transition temperature. The deviation from perfect lamellar shape is…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , David Andelman

We study a model of flexible block copolymers (BCPs) in which there is an enlthalpic preference for local alignment, among like-block segments. We describe a generalization of the self-consistent field theory (SCFT) of flexible BCPs to…

Soft Condensed Matter · Physics 2018-05-23 Christopher J. Burke , Gregory M. Grason

We derive the mean-field theory of disordered block-copolymers composed of two monomeric species, combining Edwards' functional method with the replica technique of disordered systems. In the absence of disorder we recover the canonical…

Soft Condensed Matter · Physics 2011-01-17 Gabriele Migliorini

We investigate symmetric grain boundaries in a lamellar diblock copolymer system. The form of the interface between two grains strongly depends on the angle $\theta$, between the normals of the grains. When this angle is small, the lamellae…

Statistical Mechanics · Physics 2009-10-31 Yoav Tsori , David Andelman , Michael Schick

In the present paper, the connection between surface order-disorder phase transitions and the percolating properties of the adsorbed phase has been studied. For this purpose, four lattice-gas models in presence of repulsive interactions…

Computational Physics · Physics 2009-11-13 M. Cecilia Gimenez , Felix Nieto , Antonio J. Ramirez-Pastor

A mixture of hard squares, dimers and vacancies on a square lattice is known to undergo a transition from a low-density disordered phase to high-density columnar ordered phase. Along the fully packed square-dimer line, the system undergoes…

Statistical Mechanics · Physics 2017-07-26 Dipanjan Mandal , R. Rajesh

We consider the fundamental problem of high temperature phase transitions in the system of high density two-level atoms off-resonantly interacting with a pump field in the presence of optical collisions (OCs) and placed in the cavity. OCs…

Quantum Physics · Physics 2015-06-17 I. Yu. Chestnov , A. P. Alodjants , S. M. Arakelian

X-ray diffraction, UV-vis absorption and photoluminescence (PL) spectroscopy have been used to study the well-known order-disorder transition (ODT) to the beta phase in poly(9,9-(di n,n-octyl)fluorene)) (PF8) thin film samples through…

Materials Science · Physics 2009-11-07 M. J. Winokur , J. Slinker , D. L. Huber

We overview the concept of dynamical phase transitions in isolated quantum systems quenched out of equilibrium. We focus on non-equilibrium transitions characterized by an order parameter, which features qualitatively distinct temporal…

Statistical Mechanics · Physics 2022-10-25 Jamir Marino , Martin Eckstein , Matthew S. Foster , Ana Maria Rey
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