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Adsorption of benzene on the Si(100) surface is studied from first principles. We find that the most stable configuration is a tetra-$\sigma$-bonded structure characterized by one C-C double bond and four C-Si bonds. A similar structure,…

Condensed Matter · Physics 2009-10-31 Pier Luigi Silvestrelli , Francesco Ancilotto , Flavio Toigo

Adsorption of acetylene on Si(100) is studied from first principles. We find that, among a number of possible adsorption configurations, the lowest-energy structure is a ``bridge'' configuration, where the C$_2$H$_2$ molecule is bonded to…

Condensed Matter · Physics 2009-10-31 Pier Luigi Silvestrelli , Flavio Toigo , Francesco Ancilotto

Several dissociated and two non-dissociated adsorption structures of the phenol molecule on the Si(001)-(2 \times 1) surface are studied using density functional theory with various exchange and correlation functionals. The relaxed…

Computational Physics · Physics 2015-05-19 Karen Johnston , Andris Gulans , Tuukka Verho , Martti J. Puska

First-principles density-functional theory and supercell models are employed to calculate the adsorption of water molecules on the Cu(100) surface. In agreement with the experimental observations, the calculations show that a H2O molecule…

Materials Science · Physics 2009-09-29 Sanwu Wang , Yanzhao Cao , P. A. Rikvold

We investigate the chemical and structural configuration of acetophenone on Si(001) using synchrotron radiation core-level spectroscopy techniques and density functional theory calculations. Samples were prepared by vapour phase dosing of…

Materials Science · Physics 2015-06-22 Kane M. O'Donnell , Oliver Warschkow , Asif Suleman , Adam Fahy , Lars Thomsen , Steven R. Schofield

We present a systematic study of the atomic and electronic structure of the Si(111)-(5x2)-Au reconstruction using first-principles electronic structure calculations based on the density functional theory. We analyze the structural models…

Materials Science · Physics 2009-11-11 Sampsa Riikonen , Daniel Sanchez-Portal

The structures and energetics of organic molecules adsorbed onto clean and H-passivated Si(001)-(2$\times$1) surfaces have been calculated using density functional theory. For benzene adsorbed on the clean Si surface the tight-bridge…

Materials Science · Physics 2009-11-13 Karen Johnston , Risto M. Nieminen

This paper focuses on the performance of the storage of Li and the stability of the hybrid structure of different lattice planes of the silicon clusters and graphene by the first-principle theory. In this paper, we calculate the binding…

Mesoscale and Nanoscale Physics · Physics 2012-03-01 Wu Jiangbin , Qian Yao , Guo Xiaojie , Cui Xianhui , Miao Ling , Jiang Jianjun

We study adsorption sites of a single Xe adatom on Nb(110) surface using a density functional theory approach: The on-top site is the most favorable position for the adsorption. We compare the binding features of the present study to…

Materials Science · Physics 2015-06-03 S. Dag , M. Shaughnessy , C. Y. Fong , X. D. Zhu , L. H. Yang

The simulations of field-evaporation processes for silicon atoms on various Si(001) surfaces are implemented using the first-principles calculations based on the real-space finite-difference method. We find that the atoms which locate on…

Condensed Matter · Physics 2009-11-10 Tomoya Ono , Kikuji Hirose

We recently proposed a new structural model for the Si(331)-(12x1) surface reconstruction containing silicon pentamers as elementary structural building blocks. Using first-principles density-functional theory we here investigate the…

Materials Science · Physics 2010-01-31 Corsin Battaglia , Katalin Gaal-Nagy , Giovanni Onida , Philipp Aebi

We have performed a density functional study of fifteen different structural models of the Si(557)-Au surface reconstruction. Here we present a brief summary of the main structural trends obtained for the more favourable models, focusing…

Materials Science · Physics 2007-05-23 Daniel Sanchez-Portal , Richard M. Martin

The relaxed geometries and electronic properties of the hydrogenated phases of the Si(111)-7$\times$7 surface are studied using first-principles molecular dynamics. A monohydride phase, with one H per dangling bond adsorbed on the bare…

Condensed Matter · Physics 2009-10-28 D. R. Alfonso , C. Noguez , D. A. Drabold , S. E. Ulloa

Extensive density-functional calculations are performed for chemisorption of atoms in the three first periods (H, B, C, N, O, F, Al, Si, P, S, and Cl) on the polar TiC(111) surface. Calculations are also performed for O on TiC(001), for…

Materials Science · Physics 2007-05-23 Carlo Ruberto , Bengt I. Lundqvist

We simulate the liquid silicon surface with first-principles molecular dynamics in a slab geometry. We find that the atom-density profile presents a pronounced layering, similar to those observed in low-temperature liquid metals like Ga and…

Soft Condensed Matter · Physics 2009-10-31 G. Fabricius , E. Artacho , D. Sanchez-Portal , P. Ordejon , D. A. Drabold , J. M. Soler

Structural and charge relaxation of nanoclusters of CdSe of diameter 1-2 nm are studied with first principle calculations. The relaxations cause significant distortions of smaller systems of ~ 1 nm in diameter and have very minimal effect…

Materials Science · Physics 2014-05-09 Anteneh G Tefera , Mogus D Mochena , Elijah Johnson , James Dickerson

First-principles calculations using density functional theory based on norm-conserving pseudopotentials have been performed to investigate the Mg adsorption on the Si(001) surface for 1/4, 1/2 and 1 monolayer coverages. For both 1/4 and 1/2…

Soft Condensed Matter · Physics 2007-05-23 R. Shaltaf , E. Mete , Ş. Ellialtıoğlu

Localized basis ab initio molecular dynamics simulation within the density functional framework has been used to generate realistic configurations of amorphous silicon carbide (a-SiC). Our approach consists of constructing a set of smart…

Disordered Systems and Neural Networks · Physics 2015-05-13 Raymond Atta-Fynn , Parthapratim Biswas

Surface adsorption of C$_{60}$ affects its chemical and electronic properties. Numerous studies have reported observation of bright and dark fullerenes on metal surfaces that suggest extensive surface reconstruction, however, the…

Materials Science · Physics 2021-12-01 Leonardo Forcieri , Simon Taylor , Philip Moriarty , Samuel P Jarvis

Silicon is viewed as an excellent electrode material for lithium batteries due to its high lithium storage capacity. Various Si nano-structures, such as Si nanowires, have performed well as lithium battery anodes and have opened up exciting…

Materials Science · Physics 2015-06-15 Qianfan Zhang , Yi Cui , Enge Wang
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