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We present magnetodielectric measurements in single crystals of the cubic spin-1/2 compound Cu$_2$OSeO$_3$. A magnetic field-induced electric polarization ($\vec{P}$) and a finite magnetocapacitance (MC) is observed at the onset of the…

Strongly Correlated Electrons · Physics 2012-06-14 M. Belesi , I. Rousochatzakis , M. Abid , U. K. Rößler , H. Berger , J. -Ph. Ansermet

We report the observation of a frequency shift and splitting of the electron spin resonance (ESR) mode of the low-dimensional S=1/2 frustrated antiferromagnet Cs2CuCl4 in the spin-correlated state below the Curie-Weiss temperature 4 K but…

Strongly Correlated Electrons · Physics 2015-03-18 K. Yu. Povarov , A. I. Smirnov , O. A. Starykh , S. V. Petrov , A. Ya. Shapiro

We investigated magnetization, muon spin rotation ($\mu$SR), and $^{119}Sn$ M\"{o}ssbauer spectroscopy on Sn substituted $CuCr_{2-x}Sn_xS_4$ (x=0.03 and 0.08) spinel compounds. The magnetization and $\mu$SR results reveal similar additional…

We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field…

Strongly Correlated Electrons · Physics 2013-06-25 Y. Tokiwa , T. Radu , R. Coldea , H. Wilhelm , Z. Tylczynski , F. Steglich

Magnetization maesurements under hydrostatic pressure were performed on an S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic field H parallel to the [2,0,1] direction. With increasing applied pressure P, the gap…

Statistical Mechanics · Physics 2009-11-10 Kenji Goto , Masashi Fujisawa , Toshio Ono , Hidekazu Tanaka , Yoshiya Uwatoko

We study the high magnetic field regime of the antiferromagnetic insulator Cs$_2$CuCl$_4$ by expressing the spin-1/2 operators in the relevant Heisenberg model in terms of hard-core bosons and implementing the hard-core constraint via an…

Strongly Correlated Electrons · Physics 2015-10-01 Simon Streib , Peter Kopietz

Motivated by the discovery of multiferroicity in the geometrically frustrated triangular antiferromagnet CuCrO$_2$ below its N\'eel temperature $T_N$, we investigate its magnetic and ferroelectric properties using ab initio calculations and…

Materials Science · Physics 2017-10-23 Ahmed Albaalbaky , Yaroslav Kvashnin , Denis Ledue , Renaud Patte , Raymond Frésard

We use series expansion methods to study ground- and excited-state properties in the helically ordered phase of spin-1/2 frustrated antiferromagnets on an anisotropic triangular lattice. We calculate the ground state energy, ordering…

Strongly Correlated Electrons · Physics 2009-11-13 John O. Fjaerestad , Weihong Zheng , Rajiv R. P. Singh , Ross H. McKenzie , Radu Coldea

We report $^{133}$Cs nuclear magnetic resonance (NMR) measurements on the 2D frustrated Heisenberg antiferromagnet Cs$_2$CuCl$_4$ down to 2 K and up to 15 T. We show that $^{133}$Cs NMR is a good probe of the magnetic degrees of freedom in…

Strongly Correlated Electrons · Physics 2009-11-11 M. -A. Vachon , W. Kundhikanjana , A. Straub , V. F. Mitrović , A. P. Reyes , P. Kuhns , R. Coldea , Z. Tylczynski

Geometrical frustration and the enhancement of strong quantum fluctuations in two-dimensional triangular antiferromagnets can lead to various intriguing phenomena. Here, we studied the spin-1/2 triangular lattice antiferromagnet…

Isotropic and anisotropic magnetic behavior of the frustrated spin chain compound $\beta$-TeVO$_4$ is reported. Three magnetic transitions observed in zero magnetic field are tracked in fields applied along different crystallographic…

We have studied the influence of the magnetization on the superconducting transition temperature ($T_c$) in bi- and trilayers consisting of the half-metallic ferromagnet La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) and the high-temperature…

Superconductivity · Physics 2009-04-15 M. van Zalk , M. Veldhorst , A. Brinkman , J. Aarts , H. Hilgenkamp

The 3$d$-electronic spin dynamics and the magnetic order in Fe$_3$PO$_4$O$_3$ were investigated by muon spin rotation and relaxation ($\mu$SR) and $^{57}$Fe M\"ossbauer spectroscopy. Zero-field (ZF)-$\mu$SR and $^{57}$Fe M\"ossbauer studies…

We have investigated the magnetic ground state properties of the quantum spin trimer compound strontium hydroxy copper chloride SrCu(OH)$_3$Cl using bulk magnetization, specific heat measurements, nuclear magnetic resonance (NMR), and…

In this letter we describe the ground-state magnetic structure of the highly anisotropic helimagnet Cr$_{1/3}$NbS$_2$ in a magnetic field. A Heisenberg spin model with Dyzaloshinkii-Moriya interactions and magne- tocrystalline anisotropy…

Strongly Correlated Electrons · Physics 2015-06-22 Benjamin J. Chapman , Alexander C. Bornstein , Nirmal J. Ghimire , David Mandrus , Minhyea Lee

We report first-principles all-electron density-functional based studies of the electronic structure, magnetic ordering and anisotropy for the V$_{15}$ molecular magnet. From these calculations, we determine a Heisenberg Hamiltonian with…

Materials Science · Physics 2009-11-07 Jens Kortus , C. Stephen Hellberg , Mark R. Pederson

The spin-1 anisotropic antiferromagnet NiCl_2-4SC(NH2)_2 exhibits a field-induced quantum phase transition that is formally analogous to Bose-Einstein condensation. Here we present results of systematic high-field electron spin resonance…

Strongly Correlated Electrons · Physics 2012-02-27 C. Psaroudaki , S. A. Zvyagin , J. Krzystek , A. Paduan-Filho , X. Zotos , N. Papanicolaou

The mechanisms of thermally activated magnetization switching in small ferromagnetic particles driven by an external magnetic field are investigated. For low uniaxial anisotropy the spins rotate coherently while for sufficiently large…

Statistical Mechanics · Physics 2009-10-31 U. Nowak , D. Hinzke

The magnetic properties of Cs$_2$Cu$_3$CeF$_{12}$ were investigated through magnetization and specific heat measurements. Cs$_2$Cu$_3$CeF$_{12}$ is composed of a buckled kagome lattice of Cu$^{2+}$, which is stacked along the b axis. The…

Strongly Correlated Electrons · Physics 2015-06-04 Taiki Amemiya , Izumi Umegaki , Hidekazu Tanaka , Toshio Ono , Akira Matsuo , Koichi Kindo

We investigate the magnetic properties of the multiferroic quantum-spin system LiCu$_2$O$_2$ by electron spin resonance (ESR) measurements at $X$- and $Q$-band frequencies in a wide temperature range $(T_{\rm N1} \leq T \leq 300$\,K). The…