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The electrostatic complexation between DOTAP-DOPC unilamellar liposomes and an oppositely charged polyelectrolyte (NaPA) has been investigated in a wide range of the liposome surface charge density. We systematically characterized the…

Soft Condensed Matter · Physics 2015-03-11 Simona Sennato , Laura Carlini , Domenico Truzzolillo , Federico Bordi

We present results of molecular dynamics simulations of strong, flexible polyelectrolyte chains in solution with added salt. The effect of added salt on the polyelectrolyte chain structure is fully treated for the first time as a function…

Soft Condensed Matter · Physics 2008-02-03 Mark J. Stevens , Steve Plimpton

A simple model is presented to calculate the potential of mean force between a polyion and a multivalent counterion inside a polyelectrolite solution. We find that under certain conditions the electrostatic interactions can lead to a strong…

Statistical Mechanics · Physics 2009-11-11 Jürgen F. Stilck , Yan Levin

Phase transitions in polar binary mixtures can be drastically altered even by a small amount of salt. This is because the preferential solvation strongly depends on the ambient composition. Together with a summary of our research in this…

Soft Condensed Matter · Physics 2015-05-20 Akira Onuki , Takeaki Araki , Ryuichi Okamoto

The kinetics of phase transition processes often governs the resulting material microstruc-ture. Using optical microscopy, we here investigate the formation and stabilization of a po-rous crystalline microstructure forming in low-salt…

Soft Condensed Matter · Physics 2023-06-23 Nina Lorenz , Christopher Wittenberg , Thomas Palberg

Efficient mixing of colloids, particles or molecules is a central issue in many processes. It results from the complex interplay between flow deformations and molecular diffusion, which is generally assumed to control the homogenization…

The charge inversion phenomenon is studied by molecular dynamics simulations, focusing on size and valence asymmetric salts, and a threshold of surface charge density for charge inversion. The charge inversion criteria by the…

Soft Condensed Matter · Physics 2009-11-10 Motohiko Tanaka

In nanoparticle haloing, charged nanoparticles have been found to enhance the stability of colloidal suspensions by forming a non-adsorbing layer surrounding neutral colloids which induces an electrostatic repulsion between them. However,…

Soft Condensed Matter · Physics 2019-12-18 Marzieh Moradi , Qingwen He , Gerold A. Willing

In this paper, some equations are derived to describe the out-of-equilibrium thermodynamics of colloidal suspensions. These results are obtained assuming that the properties of the colloids essentially come from their surfaces which are…

Soft Condensed Matter · Physics 2013-03-29 Pierre de Thier

The distribution of counterions and the electrostatic interaction between two similarly charged dielectric slabs is studied in the strong coupling limit. Dielectric inhomogeneities and discreteness of charge on the slabs have been taken…

Biological Physics · Physics 2015-06-12 Weria Pezeshkian , Narges Nikoofard , Davood Norouzi , Farshid Mohammad-Rafiee , Hossein Fazli

Colloidal particles are often seen as big atoms that can be directly observed in real space. They are therefore playing an increasingly important role as model systems to study processes of interest in condensed matter physics such as…

The effect of fixed discrete colloidal charges in the primitive model is investigated for spherical macroions. Instead of considering a central bare charge, as it is traditionally done, we distribute \textit{discrete} charges randomly on…

Soft Condensed Matter · Physics 2009-10-31 Rene Messina , Christian Holm , Kurt Kremer

We study the electrophoretic flow of suspensions of charged colloids with a mesoscopic method that allows to model generic experimental conditions. We show that for highly charged colloids their electrophoretic mobility increases…

Soft Condensed Matter · Physics 2015-05-28 Giovanni Giupponi , Ignacio Pagonabarraga

The effects of image charges (i.e., induced surface charges of polarization) in spherical geometry and their implication for charged colloidal systems are investigated. We study analytically and exactly a single microion interacting with a…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina

Aggregation of two oppositely charged colloids in salty water is studied. We focus on the role of Coulomb interaction in strongly asymmetric systems in which the charge and size of one colloid is much larger than the other one. In the…

Soft Condensed Matter · Physics 2009-11-10 R. Zhang , B. I. Shklovskii

The solid-liquid phase-diagram of charge-stabilized colloidal suspensions is calculated using a technique that combines a continuous Poisson-Boltzmann description for the microscopic electrolyte ions with a molecular-dynamics simulation for…

Soft Condensed Matter · Physics 2009-11-07 J. Dobnikar , R. Rzehak , H. H. von Gruenberg

We review recent experimental, numerical, and analytical results on active suspensions of self-propelled colloidal beads moving in (quasi) two dimensions. Active colloids form part of the larger theme of active matter, which is noted for…

Soft Condensed Matter · Physics 2014-09-03 Julian Bialké , Thomas Speck , Hartmut Löwen

Colloidal suspensions with free polymer coils which are larger than the colloidal particles are considered. The polymer-colloid interaction is modeled by an extension of the Asakura-Oosawa model. Phase separation occurs into dilute and…

Soft Condensed Matter · Physics 2009-10-31 Richard P. Sear

We investigate numerically and on the scaling level the adsorption of a charged colloid on an oppositely charged flexible membrane. We show that the long ranged character of the electrostatic interaction leads to a wrapping reentrance of…

Biological Physics · Physics 2009-11-10 Christian C. Fleck , Roland R. Netz

We study the thermodynamic behavior of nonpolar liquid mixtures in the vicinity of curved charged objects, such as electrodes or charged colloids. For small enough charge on the object, or equivalently, small potential, the…

Statistical Mechanics · Physics 2009-11-13 Gilad Marcus , Sela Samin , Yoav Tsori