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Using first-principles calculations, we systematically study the adsorption behavior of a single molecular H$_{2}$O on the Be(0001) surface. We find that the favored molecular adsorption site is the top site with an adsorption energy of…

Materials Science · Physics 2015-05-27 Shuang-Xi Wang , Peng Zhang , Jian Zhao , Shu-Shen Li , Ping Zhang

A comparative first principles pseudopotential study of the adsorption and migration profiles of single Pt and Au atoms on the stoichiometric and reduced TiO2 rutile (110) surfaces is presented. Pt and Au behave similarly with respect to…

Materials Science · Physics 2009-11-10 Hakim Iddir , Serdar Ogut , Nigel D. Browning , Mark M. Disco

The adsorption of rare gases on metal surfaces serve as the paradigm of weak adsorption where it is typically assumed that the adsorbate occupies maximally coordinated hollow sites. Density-functional theory calculations using the…

Materials Science · Physics 2009-11-07 Juarez L. F. Da Silva , Catherine Stampfl , Matthias Scheffler

In order to investigate the orientational ordering of molecular dipoles and the associated electronic properties, we studied the adsorption of chlorogallium phthalocyanine molecules (GaClPc, Pc=C_32N_8H_16) on Cu(111) using the X-ray…

Materials Science · Physics 2015-03-19 A. Gerlach , T. Hosokai , S. Duhm , S. Kera , O. T. Hofmann , E. Zojer , J. Zegenhagen , F. Schreiber

We report an experimental and theoretical analysis of the sqrt(3)x sqrt(3)-R30 and 2x2 reconstructions on the NiO (111) surface combining transmission electron microscopy, x-ray photoelectron spectroscopy, and reasonably accurate density…

Materials Science · Physics 2015-05-13 J. Ciston , A. Subramanian , D. M. Kienzle , L. D. Marks

Atomic oxygen adsorption on the Mo(112) surface has been investigated by means of first-principles total energy calculations. Among the variety of possible adsorption sites it was found that the bridge sites between two Mo atoms of the…

Materials Science · Physics 2007-05-23 Adam Kiejna , R. M. Nieminen

Electronic structure calculations are performed to obtain the As-exposed Si(211) and the Te adsorbed As-exposed Si(211) surface. Arsenic-exposed Si(211) may be obtained by adsorbing As on Si(211) or by replacing surface Si atoms by As.…

Materials Science · Physics 2007-05-23 Bikash C Gupta , Inder P Batra , S. Sivananthan

We identify the atomic structure of the Au/Si(111)-5x2 surface by using density functional theory calculations. With seven Au atoms per unit cell, our model forms a bona fide 5x2 atomic structure, which is energetically favored over the…

Materials Science · Physics 2014-08-20 Se Gab Kwon , Myung Ho Kang

The geometrical structures of singlet or triplet NCH3 molecules adsorbing on Cu(110) surface with presence of Cu adatoms have been determined by first-principle calculation method. The two distinguishable structures match the patterns of…

Materials Science · Physics 2016-06-28 Po-Tuan Chen

A comprehensive phase diagram of lowest-energy structures and compositions of the rutile TiO_2(110) surface in equilibrium with a surrounding gas phase at finite temperatures and pressures has been determined using density functional theory…

Materials Science · Physics 2009-11-13 Piotr M. Kowalski , Bernd Meyer , Dominik Marx

We present a first-principles study of the atomic hydrogen adsorption onto the Be(10\={1}0) thin film. There are two types of Be(10\={1}0) surfaces according to the interlayer spacing between the surface and its nearest-neighbor layer. We…

Materials Science · Physics 2007-05-23 Ping Zhang , Hong-Zhou Song

We study the binding pattern of the amino acid alanine on the naturally chiral Pt surfaces Pt(531), Pt(321) and Pt(643). These surfaces are all vicinal to the {111} direction but have different local environments of their kink sites and are…

Materials Science · Physics 2015-06-23 J. -H. Franke , D. S. Kosov

In our theoretical study where we combine a nonequilibrium Green's function (NEGF) approach with density functional theory (DFT) we investigate compounds containing a ferrocene moiety which is connected to i) thiol anchor groups on both…

Chemical Physics · Physics 2019-01-30 Xin Zhao , Robert Stadler

The first principles density functional theory (DFT) is applied to study effects of molecular adsorption on optical losses of silver (111) surface. The ground states of the systems including water, methanol, and ethanol molecules adsorbed…

Materials Science · Physics 2015-05-14 Alexander V. Gavrilenko , Carla S. McKinney , Vladimir I. Gavrilenko

The local adsorption geometries of the (2x2)-N and the (sqrt(3)x sqrt(3))R30^o -N phases on the Ru(0001) surface are determined by analyzing low-energy electron diffraction (LEED) intensity data. For both phases, nitrogen occupies the…

Materials Science · Physics 2009-10-28 S. Schwegmann , A. P. Seitsonen , H. Dietrich , H. Bludau , H. Over , K. Jacobi , G. Ertl

By means of density functional theory we have undertaken a structural, electronic and magnetic survey of the adsorption of the Fe_xPt_y(x,y=<4) clusters on MgO (001) surface under the generalized gradient approximation. We have tested…

Materials Science · Physics 2015-06-23 Ramon Cuadrado , Roy W. Chantrell

The spin-density functional theory (DFT) and DFT+$U$ with Hubbard $U$ term accounting for on-site Coulomb interactions were applied to investigate structure, stability, and electronic properties of different terminations of the…

Materials Science · Physics 2015-06-03 Adam Kiejna , Tomasz Ossowski , Tomasz Pabisiak

A metastable {\epsilon}-Al60Sm11 phase appears during the initial devitrification of as-quenched Al-10.2 at.% Sm glasses. The {\epsilon} phase is nonstoichiometric in nature since Al occupation is observed on the 16f Sm lattice sites.…

We have studied the adsorption of bisphenol-A-polycarbonate (BPA-PC) on the alpha-Al2O3(0001) surface using density-functional theory (DFT) with van der Waals (vdW) corrections. The BPA-PC polymer can be divided into its chemical fragments…

Materials Science · Physics 2012-05-30 Janne Blomqvist , Petri Salo

Adsorption of acetylene on Si(100) is studied from first principles. We find that, among a number of possible adsorption configurations, the lowest-energy structure is a ``bridge'' configuration, where the C$_2$H$_2$ molecule is bonded to…

Condensed Matter · Physics 2009-10-31 Pier Luigi Silvestrelli , Flavio Toigo , Francesco Ancilotto
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