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We report accurate quantum calculations of the sieving of Helium atoms by two-dimensional (2D) graphtriyne layers with a new interaction potential. Thermal rate constants and permeances in an ample temperature range are computed and…

Mesoscale and Nanoscale Physics · Physics 2021-04-19 Marta I. Hernández , Massimiliano Bartolomei , José Campos-Martínez

The ground and excited state properties of small helium clusters, 4He_N, containing nanoscale (~3-10 Angstroms) planar aromatic molecules have been studied with quantum Monte Carlo methods. Ground state structures and energies are obtained…

Chemical Physics · Physics 2016-09-08 Patrick Huang , Heather D. Whitley , K. Birgitta Whaley

The adsorption of a single multi-block $AB$-copolymer on a solid planar substrate is investigated by means of computer simulations and scaling analysis. It is shown that the problem can be mapped onto an effective homopolymer adsorption…

Soft Condensed Matter · Physics 2008-06-27 Swati Bhattacharya , Hsiao-Ping Hsu , Andrey Milchev , Vakhtang G. Rostiashvili , Thomas A. Vilgis

The conformational behavior of a coarse-grained finite polymer chain near an attractive spherical surface was investigated by means of multicanonical Monte Carlo computer simulations. In a detailed analysis of canonical equilibrium data…

Soft Condensed Matter · Physics 2018-01-03 Handan Arkin , Wolfhard Janke

We investigate deuterium atoms adsorbed on the surface of liquid helium in equilibrium with a vapor of atoms of the same species. These atoms are studied by a sensitive optical method based on spectroscopy at a wavelength of 122 nm,…

Condensed Matter · Physics 2009-10-31 A. P. Mosk , M. W. Reynolds , T. W. Hijmans

The ability of atomic hydrogen to chemisorb on graphene makes the latter a promising material for hydrogen storage. Based on scanning tunneling microscopy techniques, we report on site-selective adsorption of atomic hydrogen on convexly…

The density functional approach for classical associating fluids is used to explore the wetting phase diagrams for model systems consisting of water and graphite-like solid surfaces chemically modified by a small amount of grafted chain…

Soft Condensed Matter · Physics 2025-06-26 O. Pizio

Path-integral Monte Carlo calculations have been performed to study the $^4$He adsorption on $\gamma$-graphyne, a planar network of benzene rings connected by acetylene bonds. Assuming the $^4$He-substrate interaction described by a…

Materials Science · Physics 2014-09-05 Jeonghwan Ahn , Hoonkyung Lee , Yongkyung Kwon

Path Integral Monte Carlo calculations of the superfluid density throughout ^4He droplets doped with linear impurities (HCN)_n are presented. After deriving a local estimator for the superfluid density distribution, we find a decreased…

Condensed Matter · Physics 2009-11-07 E. W. Draeger , D. M. Ceperley

Helium films show various quantum phases that undergo quantum phase transitions by changing coverage n. We found anomalous elastic phenomena in bosonic 4He and fermionic 3He films adsorbed on a glass substrate. The films stiffen under AC…

Strongly Correlated Electrons · Physics 2018-12-12 T. Makiuchi , M. Tagai , Y. Nago , D. Takahashi , K. Shirahama

A lattice gas model of adsorption inside cylindrical pores is evaluated with Monte Carlo simulations. The model incorporates two kinds of site: (a line of) ``axial'' sites and surrounding ``cylindrical shell'' sites, in ratio 1:7. The…

Statistical Mechanics · Physics 2009-11-10 Raluca A. Trasca , M. Mercedes Calbi , Milton W. Cole , Jose L. Riccardo

Graphite is a ubiquitous electrode material with particular promise for use in e.g., energy storage and desalination devices, but very little is known about the properties of the graphite-electrolyte double layer at technologically relevant…

Materials Science · Physics 2021-09-03 Aaron R. Finney , Ian J. McPherson , Patrick R. Unwin , Matteo Salvalaglio

We study the three-dimensional structure formation when atoms are deposited onto a substrate with a decagonal quasicrystalline order. Molecular-dynamicscalculations show that the adsorbate layer consists of ordered nano-scale domains with…

Materials Science · Physics 2007-11-29 Muhittin Mungan , Yves Weisskopf , Mehmet Erbudak

We demonstrate the temperature-mediated and completely reversible process of desorption-readsorption of water on a few layers of epitaxial graphene on a 4H-SiC(0001) substrate. We show that under ambient conditions water forms solid…

Mesoscale and Nanoscale Physics · Physics 2012-04-17 Tim L. Burnett , Jack Patten , Olga Kazakova

Molecular hydrogen is at the core of hydrogen energy applications and has the potential to significantly reduce the use of carbon dioxide emitting energy processes. However, hydrogen gas storage is a major bottleneck for its large-scale use…

Materials Science · Physics 2025-01-22 Yasmine S. Al-Hamdani , Andrea Zen , Dario Alfé

$^4$He nanodroplets doped with an alkali ion feature a snowball of crystallized layers surrounded by superfluid helium. For large droplets, we predict that a transitional supersolid layer can form, bridging between the solid core and the…

Quantum Gases · Physics 2025-03-12 Juan Carlos Acosta Matos , Panos Giannakeas , Matteo Ciardi , Thomas Pohl , Jan M. Rost

We examine the hydrodynamic phonon spectrum of a monolayer film adsorbed on the wall of a spherical pore. Due to the boundary conditions, the monolayer film exhibits a discrete phonon spectrum. The corresponding density of states per unit…

Statistical Mechanics · Physics 2009-11-07 R. A. Trasca , A. M. Vidales , M. W. Cole

The flat metasurfaces described by tensor surface conductivity, the transverse size of which is small compared to the wavelength, are considered. In this case, we introduce two-dimensional surface conductivity for them, as well as for…

Mesoscale and Nanoscale Physics · Physics 2025-02-28 Michael V. Davidovich

A recent claim of possible superfluid behaviour of parahydrogen films intercalated within a crystalline matrix of Na atoms is examined. Quantum Monte Carlo simulations at finite temperature yield strong numerical evidence that the system…

Other Condensed Matter · Physics 2016-02-10 Massimo Boninsegni

A flux liquid can condense into a smectic crystal in a pure layered superconductor with the magnetic field oriented nearly parallel to the layers. Similar order can arise in low temperature $^4$He films with a highly anisotropic periodic…

Condensed Matter · Physics 2016-08-31 Leon Balents , David R. Nelson
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