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Optical transmission spectra of YAl3(BO3)4 crystals doped with the Pr3+ ions in concentrations 1 and 2.5 at. % were studied by high-resolution (up to 0.05 cm-1) Fourier spectroscopy, including in magnetic field parallel to the trigonal c…

We report on the synthesis and spectroscopic characterization of Sm$^{3+}$-doped K$_2$YF$_5$ microparticles. The particles were synthesized via the hydrothermal technique, yielding a particle size of approximately 20 $\mu$m in length.…

Materials Science · Physics 2025-10-15 Pakwan Chanprakhon , Michael F. Reid , and Jon-Paul R. Wells

Erbium ions in crystals show considerable promise for the technologies that will form the backbone of future networked quantum information technology. Despite advances in leveraging erbium's fibre-compatible infrared transition for…

High-resolution absorption and laser spectroscopy are used to determine electronic energy levels for Ho$^{3+}$ ions in K$_2$YF$_5$ microparticles. A total of 72 crystal-field energy levels, distributed among 8 multiplets, are assigned. This…

Materials Science · Physics 2025-10-21 Pakwan Chanprakhon , Michael F. Reid , Jon-Paul R. Wells

Parametrized crystal-field analyses are presented for both the six and seven fold coordinated, C$_{1}$ symmetry Sm$^{3+}$ centers in Y$_{2}$SiO$_{5}$, based on extensive spectroscopic data spanning the infrared to optical regions. Laser…

Materials Science · Physics 2022-06-29 N. L. Jobbitt , J. -P. R. Wells , M. F. Reid

High-resolution absorption spectra of \NH\ in the region 2100 - 5500 \cm\ at 1027 $^{\circ}$C and atmospheric pressure (1045 $\pm$ 3 mbar) are measured. An \NH\ concentration of 10\% in volume fraction is used in the measurements. Spectra…

Optical absorption spectra of Cr$^{3+}$-Cr$^{2+}$ pair center in KZnF$_{3}$:Cr$^{3+}$,Cr$^{2+}$ crystal were investigated in wide temperature range. Broad band at 30800 cm$^{-1}$ is attributed to cation-cation (e_g)-electron transfer…

Strongly Correlated Electrons · Physics 2009-10-31 M. V. Eremin , S. I. Nikitin , S. Yu. Prosvirnin , N. I. Silkin , R. V. Yusupov

In single crystals of SrTiO_3, a paramagnetic center, characterized by S = 3/2 and hyperfine interaction with an I = 5/2 nuclear spin has been observed in the temperature range 4.2K-77K by means of EPR. The impurity center is attributed to…

Materials Science · Physics 2010-03-09 Th. W. Kool

We report high-resolution optical absorption spectra for NdFe3(BO3)4 trigonal single crystal which is known to exhibit a giant magnetoelectric effect below the temperature of magnetic ordering TN = 33 K. The analysis of the…

Laser site-selective spectroscopy and high-resolution absorption measurements have been used to determine 51 crystal-field energy levels for one of the Ho$^{3+}$ centres in Y$_{2}$SiO$_{5}$. This centre is denoted as Site 2 and has been…

We report growth of high-quality single crystals of CeCl3 using a modified Bridgman Stockbarger method in an infrared image furnace. The grown crystals are characterized using single-crystal/powder X-ray diffraction, Laue X-ray diffraction,…

Strongly Correlated Electrons · Physics 2024-07-03 Nashra Pistawala , Suman Karmakar , Rajeev Rawat , Surjeet Singh

Photoluminescence, thermally stimulated luminescence (TSL) and EPR characteristics of the Ce3+ doped single crystals of multicomponent Y1Lu2GaxAl5-xO12 and Lu3GaxAl5-xO12 garnets with different Ga contents (x = 0, 1, 2, 3, 4, 5) excited in…

Low-temperature electronic properties of rare-earth intermetallics are substantially influenced by the symmetry and magnitude of the crystal electric field. The direct spectroscopic analysis of crystal field splitting can be challenging,…

Strongly Correlated Electrons · Physics 2017-04-19 B. Halbig , U. Bass , J. Geurts , M. Zinner , K. Fauth

The nonproportional scintillation response of LaBr3 doped with 5% Ce3+ and of LaCl3 doped with 10% Ce3+ was measured using highly monochromatic synchrotron irradiation. To estimate the photon response, pulse height spectra at many finely…

Materials Science · Physics 2011-03-18 Ivan V. Khodyuk , Pieter Dorenbos

Absorption, excitation and emission spectra of cadmium fluoride crystals doped with rare-earth ions were investigated. In contrast to alkaline-earth fluorides the absorption spectra due to 4f - 5d transitions of Ce$^{3+}$, Pr$^{3+}$ and…

Materials Science · Physics 2015-06-17 Evgeny Radzhabov , Roman Shendrik

The local environment of Gd3+ (4f7 S=7/2) ions in single crystals of Ca1-xGdxB6 (0.0001 < x < 0.01) is studied by means of Electron Spin Resonance (ESR). The spectra for low concentration samples (x < 0.001) show a split spectrum due to…

We show that crystal-field calculations for $C_1$ point-group symmetry are possible, and that such calculations can be performed with sufficient accuracy to have substantial utility for rare-earth based quantum information applications. In…

K$_2$YF$_5$ crystals doped with lanthanide ions have a variety of possible optical applications. Owing to the low symmetry of the system, the crystal structure cannot be unambiguously determined by x-ray diffraction. However,…

Materials Science · Physics 2024-09-27 Pratik S. Solanki , Michael F. Reid , Jon-Paul R. Wells

Group IV color centers in diamond are among the most promising optically active spin systems with strong optical transitions and long spin coherences. The ground-state splitting of the center is particularly important to suppress the…

We present a comprehensive spectroscopic study of C$_{2v}$ point-group symmetry sites in Sm$^{3+}$:CaF$_2$/SrF$_2$ codoped with either NaF or LiF. Data includes electron paramagnetic resonance measurements of Zeeman and hyperfine…

Materials Science · Physics 2018-12-05 Sebastian P Horvath , Jon-Paul R Wells , Michael F Reid , Mitsuo Yamaga , Makoto Honda
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